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arXiv:1102.0088 · Physical Review B

Time-optimal rotation of a spin 12 : Application to the NV center spin in diamond

Zhi-Hui Wang, V. V. Dobrovitski

Published Jul 6, 2011• 20 citations
arXivHTMLPDF

Abstract

We study the applicability of the time-optimal bang-bang control designed for spin $\frac{1}{2}$ [Boscain and Mason, J. Math. Phys. 47, 062101 (2006)] to the rotation of the electron spin of a nitrogen-vacancy (NV) center in diamond. The spin of the NV center is a three-level system, with two levels forming a relevant qubit subspace where the time-varying magnetic control field performs rotation, and the third level being idle. We find that the bang-bang control protocol decreases the rotation time by 20%--25% in comparison with the traditional oscillating sinusoidal driving. We also find that for most values of the bias field, the leakage to the idle level is very small, so that the NV center is a suitable testbed for experimental study of the time-optimal protocols. For some special values of the bias field, however, the unwanted leakage is greatly increased. We demonstrate that this is caused by the resonance with higher-order Fourier harmonics of the bang-bang driving field.

DOI
10.1103/physrevb.84.045303

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We study the applicability of the time-optimal bang-bang control designed for spin 12\frac{1}{2}21​ [Boscain and Mason, J. Math. Phys. 47, 062101 (2006)] to the rotation of the electron spin of a nitrogen-vacancy (NV) center in diamond. The spin of the NV center is a three-level system, with two levels forming a relevant qubit subspace where the time-varying magnetic control field performs rotation, and the third level being idle. We find that the bang-bang control protocol decreases the rotation time by 20%--25% in comparison with the traditional oscillating sinusoidal driving. We also find that for most values of the bias field, the leakage to the idle level is very small, so that the NV center is a suitable testbed for experimental study of the time-optimal protocols. For some special values of the bias field, however, the unwanted leakage is greatly increased. We demonstrate that this is caused by the resonance with higher-order Fourier harmonics of the bang-bang driving field.
Among the possible defects that can occur in diamonds, one that draws attention is the nitrogen-vacancy (NV) center.Studied since the early 90s, in recent years, they became one of the most promising platforms for field applications of quantum technology at room temperature, especially for quantum sensing.They are sensitive to electric and magnetic fields, temperature, and strain, making these nanosensors a versatile platform for many applications.The NV center's spin state is easy to read and manipulate by optical means, and, most interestingly, it works well at room temperature, which facilitates its use.The great challenge to implement quantum protocols and quantum algorithms is the coherence time of the quantum states.The NV center stands out for having relatively high coherence times at room temperature.This dissertation presents measurements to characterize the electron spin coherence of NV centers in an ultrapure sample of diamond designed for quantum sensing applications.These measurements combine optical e magnetic resonance techniques.For that, a method was implemented using a conventional CCD camera and a clever imaging protocol, making it possible to perform various pulsed microwave experiments on the electron spin, such as Rabi oscillations and Hahn spin-echo, which were used for determining the characteristic relaxation times (T 1 and T 2 ).Results show that this system provides at least two readily accessible qubits that can be used in quantum protocols even at room temperature.
Coupling-selective quantum optimal control in weak-coupling NV-13^{13}13C system
Abstract Quantum systems are under various unwanted interactions due to their coupling with the environment. Efficient control of quantum system is essential for quantum information processing. Weak-coupling interactions are ubiquitous, and it is very difficult to suppress them using optimal control method, because the control operation is at a time scale of the coherent life time of the system. Nitrogen-vacancy (NV) center of diamond is a promising platform for quantum information processing. The 13^{13}13 13 C nuclear spins in the bath are weakly coupled to the NV, rendering the manipulation extremely difficulty. Here, we report a coupling selective optimal control method that selectively suppresses unwanted weak coupling interactions and at the same time greatly prolongs the life time of the wanted quantum system. We applied our theory to a 3 qubit system consisting of one NV electron spin and two 13^{13}13 13 C nuclear spins through weak-coupling with the NV center. In the experiments, the iSWAP †^{\dagger }† † gate with selective optimal quantum control is implemented in a time-span of TctrlT_{ctrl}Tctrl​ T ctrl = 170.25 μ\muμ μ s, which is comparable to the phase decoherence time T2T_2T2​ T 2 = 203 μs\mu sμs μ s . The two-qubit controlled rotation gate is also completed in a strikingly 1020(80) μ\muμ μ s, which is five times of the phase decoherence time. These results could find important applications in the NISQ era.
The negatively charged nitrogen-vacancy (NV) center spin in diamond can be used to realize quantum computation and to sense magnetic fields. Its spin triplet consists of three levels labeled with its spin zzz-components of +1, 0, and \ensuremath{-}1. Without external field, the +1 and \ensuremath{-}1 states are degenerate and higher than the 0 state due to the zero-field splitting. By taking the symmetrical and antisymmetrical superpositions of the +1 and \ensuremath{-}1 states as our qubit basis, we obtain the exact evolution operator of the NV center spin under time-dependent magnetic field by mapping the three-level system on time-dependent quantum two-level systems with exact analytical solutions. With our exact evolution operator of the NV center spin including three levels, we show that arbitrary qubits can be prepared from the starting 0 state, and arbitrary rapid quantum logic gates of these qubits can be realized with magnetic fields. In addition, it is made clear that the typical quantum logic gates can be accomplished within a few nanoseconds and the fidelity can be very high because only magnetic field strength needs to be controlled in this approach. These results should be useful to realizing quantum computing with the NV center spin systems in diamond and exploring other effects and applications.
Abstract A nitrogen-vacancy (NV) center in a diamond enables the access to an electron spin, which is expected to present highly sensitive quantum sensors. Although exploiting a nitrogen nuclear spin improves the sensitivity, manipulating it using a resonant pulse requires a long gate time owing to its small gyromagnetic ratio. Another technique to control nuclear spins is a conditional rotation gate based on dynamical decoupling, which is faster but unavailable for nitrogen spins owing to the lack of transverse hyperfine coupling with the electron spin. In this study, we generated effective transverse coupling by applying a weak off-axis magnetic field. An effective coupling depends on the off-axis field; the conditional rotation gate on the nitrogen-14 spins of an NV center was demonstrated within 4.2 μs under an 1.8% off-axis field and a longitudinal field of approximately 280 mT. We estimated that a population transfer from the electron to nitrogen spins can be implemented with 8.7 μs. Our method is applicable to an ensemble of NV centers, in addition to a single NV center.
The NV-center in diamond is a promising system for quantum information processing. The typical qubits are the electron spin in the NV-center and the surrounding 13C nuclear spins. Fast and precise control of many 13C spins is desirable but challenging due to crosstalk. Crosstalk is the unwanted effect of a control pulse on the other qubits. The coupled NV-13C system is explored, and numerical techniques to optimize the control of multiple and single qubits are used. In this report the effect of the Bloch-Siegert shift in the weak driving regime is investigated first. This is done by studying the effect of a π-pulse when two carbon qubits are driven at the same time on resonance. It turns out that in this weak driving regime the effect of the off resonance is very small, and changes the fidelity not more than 0.3%. Furthermore the effect of a square πpulse on 4 nearby qubits is studied. If the pulse is not optimized (thus square), the pulse cannot be done in less than 100µs while retaining at least 99% fidelity. By optimizing the envelope of the driving field using constrained optimization the pulse can be done in 22µs while retaining at least 99% fidelity.
Nitrogen-vacancy (NV) centers in diamond are a promising platform for ambient, high-spatial resolution magnetometry relevant to biological signals such as cardiac and muscle activity. One of the challenges is the development of pulse sequences tailored to biological signals in the near DC-range. The spatial environment of NV centers within the diamond lattice is highly complex, e.g. due to magnetic field inhomogeneities, limiting the sensors performance. To overcome these experimental constraints, quantum optimal control (QOC) aims at a precise manipulation of the systems dynamics via optimally shaped microwave pulses increasing the overall robustness of spin-based quantum sensors.