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arXiv:1101.4692 · Physical Review Letters

Decoupling a Cooper-Pair Box to Enhance the Lifetime to 0.2 ms

Z. Kim, Baladitya Suri, V. Zaretskey, S P Novikov, Kevin D. Osborn, Ari Mizel, F. C. Wellstood, B. S. Palmer

Published Mar 22, 2011• 70 citations
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Abstract

We present results on a circuit QED experiment in which a separate transmission line is used to address a quasilumped element superconducting microwave resonator which is in turn coupled to an $\mathrm{Al}/{\mathrm{AlO}}_{x}/\mathrm{Al}$ Cooper-pair box charge qubit. With our device, we find a strong correlation between the lifetime of the qubit and the inverse of the coupling between the qubit and the transmission line. At the smallest coupling we measured, the lifetime of the Cooper-pair box was ${T}_{1}=200\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$, which represents more than a twentyfold improvement in the lifetime of the Cooper-pair box compared with previous results. These results imply that the loss tangent in the ${\mathrm{AlO}}_{x}$ junction barrier must be less than about $4\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}$ at 4.5 GHz, about 4 orders of magnitude less than reported in larger area $\mathrm{Al}/{\mathrm{AlO}}_{x}/\mathrm{Al}$ tunnel junctions.

DOI
10.1103/physrevlett.106.120501

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We present results on a circuit QED experiment in which a separate transmission line is used to address a quasilumped element superconducting microwave resonator which is in turn coupled to an Al/AlOx/Al\mathrm{Al}/{\mathrm{AlO}}_{x}/\mathrm{Al}Al/AlOx​/Al Cooper-pair box charge qubit. With our device, we find a strong correlation between the lifetime of the qubit and the inverse of the coupling between the qubit and the transmission line. At the smallest coupling we measured, the lifetime of the Cooper-pair box was T1=200  \ensuremathμs{T}_{1}=200\text{ }\text{ }\ensuremath{\mu}\mathrm{s}T1​=200  \ensuremathμs, which represents more than a twentyfold improvement in the lifetime of the Cooper-pair box compared with previous results. These results imply that the loss tangent in the AlOx{\mathrm{AlO}}_{x}AlOx​ junction barrier must be less than about 4\ifmmode×\else\texttimes\fi10\ensuremath−84\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}8}4\ifmmode×\else\texttimes\fi10\ensuremath−8 at 4.5 GHz, about 4 orders of magnitude less than reported in larger area Al/AlOx/Al\mathrm{Al}/{\mathrm{AlO}}_{x}/\mathrm{Al}Al/AlOx​/Al tunnel junctions.
The quantum states of an Al/AlOx/Al Cooper pair box (CPB) qubit were measured at temperatures below 100 mK. Detailed spectroscopic measurements of the excited state of the CPB were made along with detailed measurements of the lifetime T1 of the first excited state. The CPB states were probed using radio-frequency (rf) techniques to read out using either an rf - single-electron transistor (rf-SET) or a low-loss superconducting resonator. Using an rf-SET, I measured the excited state spectrum of a CPB from 15 to 50 GHz. In this spectrum, a few anomalous avoided level crossings (ALC) were observed. These ALCs exhibited a strong gate voltage dependence and Josephson energy (Ej) dependence, consistent with a charge fluctuator coupled to the CPB island. A model Hamiltonian was used to fit the measured spectrum. Fitting parameters such as the charging energy Ec/h = 12.1 GHz and the Josephson energy Ej/h tuned between 2 GHz and 21 GHz for the CPB, and the well asymmetry, tunneling amplitude, and the minimum hopping distance for each fluctuator were extracted. The tunneling rates ranged from less than 3.5 to 13 GHz, i.e. values between 5 % and 150 % of the well asymmetry, and the dipole moments yield a minimum hopping distance of 0.3 to 0.8 Angstroms. I also made detailed measurements of the lifetime of the first excited state away from the CPB charge degeneracy point and found that the lifetime varied from less than 50 ns up to a few us as the Josephson energy Ej decreased, consistent with a charge noise (Sq~10-11 e2/Hz around 37 GHz to Sq~10-12 e2/Hz around 27 GHz) coupled to the qubit. I also found that at frequencies where an ALC was observed in the spectrum, a decrease in T1 occurred, suggesting that the discrete charge defects are a significant source of dissipation in the CPB. I also designed and fabricated a quasi-lumped element thin-film superconducting Al microwave resonator on sapphire to be used for a dispersive read-out of the CPB. The resonator consists of a meandering inductor and an interdigitated capacitor coupled to a transmission line. At T = 30 mK and on resonance at 5.578 GHz, the transmission through the transmission line decreased by 15 dB and the loaded quality factor was 60,000. I measured the temperature dependence of the resonator frequency and loss at temperatures as high as 500 mK and found reasonable agreement with the Mattis-Bardeen theory. Finally, I coupled a quasi-lumped element microwave resonator (f0~5.443 GHz), made of superconducting Al on sapphire, to an Al/AlOx/Al CPB qubit. Most of my measurements were made in the dispersive regime where Ej-hf0 is much larger than the coupling strength. In this case, the qubit causes a small state-dependent frequency shift in the resonator's resonant frequency. By sending down a second microwave tone (the pump), I was able to excite the CPB qubit. In zero magnetic field with the CPB far detuned from the resonator, I measured a 50 kHz decrease in f0 with the qubit in the ground state and biased near the degeneracy point of the CPB. The charging energy and Josephson energy of the CPB were determined from spectroscopy taken by saturating the CPB with a second microwave tone and measuring the transmission through the resonator. The first device had Ec/h = 12.5 GHz and maximum Ej/h = 9 GHz. The second device had Ec/h = 6.24 GHz and Ej/h tuned between 4 GHz and 8 GHz. By changing the external magnetic field, I could decrease the effective Ej of the CPB. From modeling, I extracted coupling strengths g/2&pi = 11 MHz and 5 MHz for the first and second device, respectively. Finally I did single and two-tone spectroscopy, and measured the relaxation and Rabi oscillations of the CPB. From the first device, I was able to obtain relaxation times T1 of 10.3 us at Ej/h = 7 GHz on the CPB degeneracy point and spectroscopic coherence times T2 *~ 100 ns. From the second device, I found relaxation times T1 of 200 us at Ej/h = 4 GHz to 4.5 GHz decreasing down to 4 us around 8 GHz. There was also a depression in T1 around the resonant frequency of the resonator. The Rabi decay times were found to be up to T'~ 330 ns.
We have investigated the decoherence of quantum states in two Al/AlOx/Al Cooper-pair boxes coupled to lumped element superconducting inductor-capacitor resonators. At 25 mK, the first qubit had an energy relaxation time T1 that varied from 30 μs to 200 μs between 4 and 8 GHz and displayed an inverse correlation between T1 and the coupling to the microwave drive line. The Ramsey fringe decay times T2* were in the [200–500] ns range while the spin echo envelope decay times Techo varied from 2.4–3.3 μs, consistent with 1/f charge noise with a high frequency cutoff of 0.2 MHz. A second Cooper-pair box qubit with similar parameters showed T1=4−30 μs between 4 and 7.3 GHz, and that the T1 and the coupling were again inversely correlated. Although the lifetime of the second device was shorter than that of the first device, the dependence on coupling in both devices suggests that further reduction in coupling should lead to improved qubit performance.
This dissertation describes my detailed investigation of decoherence and defects in two Al/AlOx/Al Cooper-pair box (CPB) charge qubits. Both devices were coupled to thin-film lumped-element superconducting aluminum LC resonators at a temperature of 25 mK. Device 1 was previously found to have an exceptionally long energy relaxation time of T1=205 μs and a strong correlation between the lifetime T1 and the decoupling from the microwave drive line dVg,rms/dΩR,0. I determined the dephasing properties of this CPB though a series of experiments. I measured Ramsey fringes, extracted dephasing times Tφ in the range200-500 ns, and determined a corresponding bound of Sq(f=1 Hz)≤(3×10-3)2 e2/Hz on the amplitude of the 1/f charge noise affecting the qubit. I then carried out a spin echo experiment and found echo decay times Techo in the 2.4-3.3 μs range, implying a high frequency 1/f charge noise cutoff of ωc/2π≈0.2 MHz. I followed this up by fabricating and characterizing a nearly identical Device 2. This CPB had a reasonably long relaxation time T1≈4-30 μs and again the lifetime T1 and decoupling dVg,rms/dΩR,0 were correlated. Although the lifetime of Device 2 was shorter than that of Device 1, the results suggest that the exceptional relaxation time was somewhat reproducible and that this approach may lead to further improvements in qubit coherence. During my initial characterization of Device 2, I discovered that it displayed an anomalously twinned transition spectrum. I studied this feature in detail in parallel with my decoherence experiments. I found that above the resonator resonance at ω/2π=5.472 GHz the system spectrum was twinned but below it was quadrupled. This behavior was consistent with a pair of two-level systems (TLS) coupled non-resonantly to the CPB via both charge and critical current. I developed a model that matched this scenario and successfully fit the predicted spectrum to my data. Both the coherent non-resonant interaction and joint charge and critical current CPB-TLS coupling are novel observations. From the fits I extracted microscopic parameters of the fluctuators including the well asymmetry, tunneling rate, and a minimum hopping distance of 0.2-0.45 Å. I also found a large fractional change of the Josephson energy ΔEJ,k/EJ≈30-40%, consistent with a non-uniform tunnel barrier containing a few dominant conduction channels and a defect that modulates one of them.
We report on the quadrupling of the transition spectrum of an Al/AlOx{}_{x}x​/Al Cooper-pair box (CPB) charge qubit in the 4.0−−7.34.0--7.34.0−−7.3 GHz frequency range. The qubit was coupled to a quasilumped-element Al superconducting resonator and measured at a temperature of 25 mK. We obtained good matches between the observed spectrum and the spectra calculated from a model Hamiltonian containing two distinct low-excitation energy two-level systems (TLS) coupled to the CPB. In our model, each TLS has a charge that tunnels between two sites in a local potential and induces a change in the CPB critical current. By fitting the model to the spectrum, we have extracted microscopic parameters of the fluctuators including the well asymmetry, tunneling rate, and a surprisingly large fractional change (3030%--40%30) in the critical current (12 nA). This large change is consistent with a Josephson junction with a nonuniform tunnel barrier containing a few dominant conduction channels and a TLS that modulates one of them.
We study theoretically the parametric down-conversion and squeezing of microwaves using cavity quantum electrodynamics of a superconducting Cooper-pair box (CPB) qubit located inside a transmission line resonator. The nonlinear susceptibility chi2 describing three-wave mixing can be tuned by dc gate voltage applied to the CPB and vanishes by symmetry at the charge degeneracy point. We show that the coherent coupling of different cavity modes through the qubit can generate a squeezed state. Based on parameters realized in recent successful circuit QED experiments, squeezing of 95% approximately 13 dB below the vacuum noise level should be readily achievable.
I report an investigation into using an rf Single Electron Transistor (rf-SET) to implement single shot readout of the quantum state of a Cooper pair box. I fabricated Al/AlOx/Al SETs and Cooper pair boxes using e-beam lithography and double-angle evaporation. The devices had typical charging energies of about 1 K and were measured at 30 mK in a dilution refrigerator. I built rf-SETs with an LC resonant circuit integrated on the chip and operating frequencies of 650 MHz and 1.5 GHz. The rf-SETs had a typical bandwidth of 30 MHz and the best achieved charge sensitivity was 8X10-6 erms/(Hz)1/2 at 1.5 GHz. The rf-SETs were used to measure the Coulomb staircase on the Cooper pair box. Measurements of the staircase show features due to quasiparticle poisoning that are dependent on temperature and SET bias. The data was compared to a theory I developed to extend existing theories of quasiparticle poisoning. My model is based on the calculation of tunneling rates to explain observations of parity effects in the Cooper pair box over a wide temperature range. Quantum state control of the Cooper pair box was demonstrated by using fast voltage pulses applied to the gate. Temporal oscillations of charge states and spectroscopy measurements reveal a dephasing time T2=200 ps at 30 mK, for a drive frequency of 30 GHz. The energy relaxation time T1=140 ns was determined from time domain measurements of the decay of the Cooper pair box charge. The fidelity of single shot measurements and the feasibility of this quantum readout scheme based on the results are discussed.