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arXiv:1011.1275 · Physical Review B

Scaling properties of the Anderson model in the Kondo regime studied by σGσW formalism

Catalin D. Spataru

Published Nov 10, 2010• 7 citations
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Abstract

The symmetric Anderson model for a single impurity coupled to two leads is studied at strong interaction using the GW approximation within the $\ensuremath{\sigma}G\ensuremath{\sigma}W$ formalism. We find that the low-energy properties show universal scaling behavior in the asymptotic regime. While the GW scaling functions are similar in form to the scaling functions known from the numerically exact solution, they are characterized by a different parameter value indicating that GW fails to describe correctly spin correlations between the impurity and lead electrons. We also compare the GW and exact Kondo scales for a broad range of the interaction strength. In contrast to the exponential behavior shown by the exact solution, the GW Kondo scale depends algebraically on the interaction strength.

DOI
10.1103/physrevb.82.195111

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The symmetric Anderson model for a single impurity coupled to two leads is studied at strong interaction using the GW approximation within the \ensuremathσG\ensuremathσW\ensuremath{\sigma}G\ensuremath{\sigma}W\ensuremathσG\ensuremathσW formalism. We find that the low-energy properties show universal scaling behavior in the asymptotic regime. While the GW scaling functions are similar in form to the scaling functions known from the numerically exact solution, they are characterized by a different parameter value indicating that GW fails to describe correctly spin correlations between the impurity and lead electrons. We also compare the GW and exact Kondo scales for a broad range of the interaction strength. In contrast to the exponential behavior shown by the exact solution, the GW Kondo scale depends algebraically on the interaction strength.
The impurity Green function and dynamical susceptibilities for the two-channel Anderson impurity model are calculated. An exact expression for the self-energy of the impurity Green function as ratio of two correlation functions is given. The imaginary part of the self-energy scales as $\sqrt{\ensuremath{\mid}\ensuremath{\omega}∕{T}_{K}\ensuremath{\mid}}$ for $T\ensuremath{\rightarrow}0$, serving as a hallmark for non-Fermi behavior. The many-body resonance is pinned to a universal value of $1∕(2\ensuremath{\pi}\ensuremath{\Delta})$ at $\ensuremath{\omega}=0$ for arbitrary local occupation in contrary to the single-channel Anderson impurity model. Its shape becomes increasingly more symmetric for the Kondo regimes of the model. The dynamical spin and channel susceptibilities are governed by two energy scales TK{T}_{K}TK​ and Th{T}_{h}Th​, and their ${\ensuremath{\chi}}^{\ensuremath{''}}(\ensuremath{\omega})$ approach a constant value for $\ensuremath{\omega}\ensuremath{\rightarrow}0$.
The local moment approach is extended to the orbitally degenerate (SU(2N)) Anderson impurity model (AIM). Single-particle dynamics are obtained over the full range of energy scales, focusing on particle-hole symmetry in the strongly-correlated regime where the onsite Coulomb interaction leads to many-body Kondo physics with entangled spin and orbital degrees of freedom. The approach captures many-body broadening of the Hubbard satellites and recovers the correct exponential vanishing of the Kondo scale for all N, and its universal scaling spectra are found to be in very good agreement with numerical renormalization group (NRG) results. In particular the high-frequency logarithmic decays of the scaling spectra, obtained here in closed form for arbitrary N, coincide essentially perfectly with available numerics from the NRG. A particular case of an anisotropic Coulomb interaction, in which the model represents a system of N 'capacitively coupled' SU(2) AIMs, is also discussed. Here the model is generally characterized by two low-energy scales, the crossover between which is seen directly in its dynamics.
We reinvestigate the large degeneracy solution of the multichannel Kondo problem, and show how in the universal regime the complicated integral equations simplifying the problem can be mapped onto a first-order differential equation. This leads to an explicit expression for the full zero-temperature scaling functions at---and away from---the intermediate non-Fermi-liquid fixed point, providing complete analytic information on the universal low---and intermediate---energy properties of the model. These results also apply to the widely used noncrossing approximation of the Anderson model, taken in the Kondo regime. An extension of this formalism for studying finite-temperature effects is also proposed and offers a simple approach to solve models of strongly correlated electrons with relevance to the physics of heavy fermion compounds.
Single-particle dynamics of the Anderson impurity model in the presence of a magnetic field H are considered, using a recently developed local moment approach that encompasses all energy scales, field and interaction strengths. For strong coupling in particular, the Kondo scaling regime is recovered. Here the frequency (ω/ω K ) and field ( H /ω K ) dependence of the resultant universal scaling spectrum is obtained in large part analytically, and the field-induced destruction of the Kondo resonance investigated. The scaling spectrum is found to exhibit the slow logarithmic tails recently shown to dominate the zero-field scaling spectrum. At the opposite extreme of the Fermi level, it gives asymptotically exact agreement with results for statics known from the Bethe ansatz. Good agreement is also found with the frequency and field-dependence of recent numerical renormalization group calculations. Differential conductance experiments on quantum dots in the presence of a magnetic field are likewise considered, and appear to be well accounted for by the theory. Some new exact results for the problem are also established.
We generalize Nozi\`eres' Fermi-liquid theory for the low-energy behavior of the Kondo model to that of the single-impurity Anderson model. In addition to the electrons' phase shift at the Fermi energy, the low-energy Fermi-liquid theory is characterized by four Fermi-liquid parameters: the two given by Nozi\`eres that enter to first order in the excitation energy, and two additional ones that enter to second order and are needed away from particle-hole symmetry. We express all four parameters in terms of zero-temperature physical observables, namely the local charge and spin susceptibilities and their derivatives with respect to the local level position. We determine these in terms of the bare parameters of the Anderson model using Bethe ansatz and numerical renormalization group (NRG) calculations. Our low-energy Fermi-liquid theory applies throughout the crossover from the strong-coupling Kondo regime via the mixed-valence regime to the empty-orbital regime. From the Fermi-liquid theory, we determine the conductance through a quantum dot symmetrically coupled to two leads in the regime of small magnetic field, low temperature, and small bias voltage, and compute the coefficients of the $\ensuremath{\sim}{B}^{2}, \ensuremath{\sim}{T}^{2}$, and $\ensuremath{\sim}{V}^{2}$ terms exactly in terms of the Fermi-liquid parameters. The coefficients of T2,V2{T}^{2}, {V}^{2}T2,V2, and B2{B}^{2}B2 are found to change sign during the Kondo to empty-orbital crossover. The crossover becomes universal in the limit that the local interaction is much larger than the level width. For completeness, we also compute the shot noise and discuss the resulting Fano factor.
The Kondo scale TK{T}_{\mathrm{K}}TK​ for impurity systems is expected to guarantee universal scaling of physical quantities. However, in practice, not every definition of TK{T}_{\mathrm{K}}TK​ necessarily supports this notion away from the strict scaling limit. Specifically, this paper addresses the role of finite bandwidth DDD in the strongly correlated Kondo regime. For this, various theoretical definitions of TK{T}_{\mathrm{K}}TK​ are analyzed based on the inverse magnetic impurity susceptibility at zero temperature. While conventional definitions in that respect quickly fail to ensure universal Kondo scaling for a large range of DDD, this paper proposes an altered definition of TKsc{T}_{\mathrm{K}}^{\mathrm{sc}}TKsc​ that allows universal scaling of dynamical or thermal quantities for a given fixed Hamiltonian. If the scaling is performed with respect to an external parameter that directly enters the Hamiltonian, such as magnetic field, the corresponding TKsc,B{T}_{\mathrm{K}}^{\mathrm{sc}},\mathrm{B}TKsc​,B for universal scaling differs, yet becomes equivalent to TKsc{T}_{\mathrm{K}}^{\mathrm{sc}}TKsc​ in the scaling limit. The only requirement for universal scaling in the full Kondo parameter regime with a residual error of less than 1% is a well-defined isolated Kondo feature with ${T}_{\mathrm{K}}\ensuremath{\lesssim}0.01\phantom{\rule{0.16em}{0ex}}D$ irrespective of specific other impurity parameter settings. By varying DDD over a wide range relative to the bare energies of the impurity, for example, this allows a smooth transition from the Anderson to the Kondo model.