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arXiv:1010.1520 · Physical Review Letters

Differential Light-Shift Cancellation in a Magnetic-Field-Insensitive Transition of Rb87

Radu Chicireanu, K. D. Nelson, Steven Olmschenk, Nathan E. Lundblad, Andrei Derevianko, J. V. Porto

Published Feb 8, 2011• 41 citations
arXivHTMLPDF

Abstract

The precise measurement of transition frequencies of trapped atomic samples is susceptible to inaccuracy arising from the inhomogeneous differential shift of the relevant energy levels in the presence of the trapping fields. We demonstrate near-complete cancellation of the differential ac Stark shift ("light shift") of a two-photon magnetic-field-insensitive microwave hyperfine (clock) transition in ^{87}Rb atoms trapped in an optical lattice. Up to 95(2)% of the differential light shift is cancelled while maintaining magnetic-field insensitivity. This technique should have applications in quantum information and frequency metrology.

DOI
10.1103/physrevlett.106.063002

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The precise measurement of transition frequencies of trapped atomic samples is susceptible to inaccuracy arising from the inhomogeneous differential shift of the relevant energy levels in the presence of the trapping fields. We demonstrate near-complete cancellation of the differential ac Stark shift ("light shift") of a two-photon magnetic-field-insensitive microwave hyperfine (clock) transition in ^{87}Rb atoms trapped in an optical lattice. Up to 95(2)% of the differential light shift is cancelled while maintaining magnetic-field insensitivity. This technique should have applications in quantum information and frequency metrology.
We demonstrate the cancellation of the differential ac Stark shift of the microwave hyperfine clock transition in trapped 87Rb^{87}\mathrm{Rb}87Rb atoms. Recent progress in metrology exploits so-called magic wavelengths, whereby an atomic ensemble can be trapped with laser light whose wavelength is chosen so that both levels of an optical atomic transition experience identical ac Stark shifts. Similar magic-wavelength techniques are not possible for the microwave hyperfine transitions in the alkali metals due to their simple electronic structure. We show, however, that ac Stark shift cancellation is indeed achievable for certain values of wavelength, polarization, and magnetic field. The cancellation comes at the expense of a small magnetic-field sensitivity. The technique demonstrated here has implications for experiments involving the precise control of optically trapped neutral atoms.
We demonstrate the cancellation of the differential ac Stark shift of the microwave hyperfine clock transition in trapped 87 Rb atoms. Recent progress in metrology exploits so-called “magic wavelengths,” whereby an atomic ensemble can be trapped with laser light whose wavelength is chosen so that both levels of an optical atomic transition experience identical ac Stark shifts. Similar magic-wavelength techniques are not possible for the microwave hyperfine transitions in the alkalis, due to their simple electronic structure. We show, however, that ac Stark shift cancellation is indeed achievable for certain values of wavelength, polarization, and magnetic field. The cancellation comes at the expense of a small magnetic-field sensitivity. The technique demonstrated here has implications for experiments involving the precise control of optically-trapped neutral atoms.
Differential light shifts (DLS) induced by optical trapping fields fundamentally limit the stability and accuracy of trapped-atom microwave clocks. We demonstrate an in-situ method to cancel DLS by simultaneously interrogating multiple spatially separated atomic ensembles at different trap intensities generated from a common light source. By operating the ensembles at set intensity ratios and performing Ramsey spectroscopy, the intensity-dependent frequency shifts are measured within each experimental cycle and extrapolated to the zero-intensity limit. This approach effectively enables shot-to-shot determination of a DLS-free frequency without requiring magic wavelengths or species-specific cancellation schemes. We validate the method for Rb atoms trapped in time-averaged potentials by introducing controlled variations of the total trap power and show that the extrapolated frequency remains insensitive to these fluctuations. The technique is general and can be extended to other systematic shifts, providing a scalable route toward improved stability and accuracy in compact trapped-atom clocks and related quantum sensors relying on optical dipole traps
We report on a precision measurement of the DDD line tune-out wavelength of 87Rb^{87}\text{Rb}87Rb in the hyperfine ground state $\left|F=1,{m}_{F}=0,\ifmmode\pm\else\textpm\fi{}1\right\ensuremath{\rangle}$ manifold at 790nm790\phantom{\rule{0.16em}{0ex}}\mathrm{nm}790nm, where the scalar ac Stark shifts of the D1{D}_{1}D1​ and the D2{D}_{2}D2​ lines cancel. This wavelength is sensitive to usually neglected contributions from vector and tensor ac Stark shifts, transitions to higher principle quantum numbers, and core electrons. The ac Stark shift is probed by Kapitza-Dirac scattering of a rubidium Bose-Einstein condensate in a one-dimensional optical lattice in free space and controlled magnetic environment. The tune-out wavelength of the magnetically insensitive mF=0{m}_{F}=0mF​=0 state was determined to 790.01858(23)nm790.01858(23)\phantom{\rule{0.16em}{0ex}}\mathrm{n}\mathrm{m}790.01858(23)nm with sub-pm accuracy. An in situ absolute polarization, and magnetic background field measurement is performed by employing the ac vector Stark shift for the ${m}_{F}=\ifmmode\pm\else\textpm\fi{}1$ states. Comparing our findings to theory, we get quantitative insight into atomic physics beyond commonly used two-level atom approximations or the neglect of inner shell contributions.
The dynamic Stark shift of an inhomogeneously broadened spectral transition has been studied. Our measurements show a shift in the observed 87 Rb ground-state hyperfine transition, which has a nonlinear dependence on light intensity when the conditions for inhomogeneous broadening are met. The nonlinearity is the result of light-intensity gradients in the signal volume, which produce an inhomogeneously broadened asymmetric microwave transition. We show that our measurements are in full agreement with the second-order perturbation-theory treatment of light-induced energy-level shifts when the effects of inhomogeneities are properly taken into consideration. The effects of inhomogeneous broadening must be carefully considered when one extracts oscillator strengths from light-shift data, or performs high-precision laser spectroscopy. Originator-supplied keywords include: AC stark effect, Atomic clocks, Atomic line shapes, Light shifts.
We propose a combination of electromagnetically induced transparency-Raman and pulsed spectroscopy techniques to accurately cancel frequency shifts arising from electromagnetically induced transparency fields in forbidden optical clock transitions of alkaline earth atoms. At appropriate detunings, time-separated laser pulses are designed to trap atoms in coherent superpositions while eliminating off-resonance ac Stark contributions, achieving efficient population transfer up to 60% with inaccuracy <10(-17). Results from the wave-function formalism are confirmed by the density matrix approach.