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arXiv:1008.2792 · Physical Review A

Heralding single photons without spectral factorability

Yu-Ping Huang, Joseph B. Altepeter, Prem Kumar

Published Oct 18, 2010• 29 citations
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Abstract

Recent efforts to produce single photons via heralding have relied on creating spectrally factorable two-photon states in order to achieve both high purity and high production rate. Through a careful multimode analysis, we find, however, that spectral factorability is not necessary. Utilizing single-mode detection, a similar or better performance can be achieved with nonfactorable states. This conclusion rides on the fact that even when using a broadband filter, a single-mode measurement can still be realized, as long as the coherence time of the triggering photons exceeds the measurement window of the on-off detector.

DOI
10.1103/physreva.82.043826

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Recent efforts to produce single photons via heralding have relied on creating spectrally factorable two-photon states in order to achieve both high purity and high production rate. Through a careful multimode analysis, we find, however, that spectral factorability is not necessary. Utilizing single-mode detection, a similar or better performance can be achieved with nonfactorable states. This conclusion rides on the fact that even when using a broadband filter, a single-mode measurement can still be realized, as long as the coherence time of the triggering photons exceeds the measurement window of the on-off detector.
A major obstacle to a practical, heralded source of single photons is the fundamental trade-off between high purity and high production rate. To overcome this difficulty, we propose applying sequential spectral and temporal filtering on the signal photons before they are detected for heralding. Based on a multimode theory that takes into account the effect of simultaneous multiple photon-pair emission, we find that these filters can be optimized to yield both high purity and a high production rate. While the optimization conditions vary depending on the underlying photon-pair spectral correlations, all correlation profiles can lead to similarly high performance levels when optimized filters are employed. This suggests that a better strategy for improving the performance of heralded single-photon sources is to adopt an appropriate measurement scheme for the signal photons, rather than tailoring the properties of the photon-pair generation medium.
Optical quantum protocols are reliant on the production of highly pure single photons. However, most parametric heralded single-photon sources possess spectral correlations, limiting the purity of the produced photon. The most common method for restoring the purity is with narrowband spectral filtering, which comes at the cost of reducing the rate of heralding detection. Here, we characterize this trade-off analytically for a large class of parametric sources. It is possible to achieve up to 20% heralding success probabilities with 90% heralded photon purities.
Quantum information processing requires techniques for the generation and transportation of quantum data. The use of photons as the carriers of that quantum information, with the data encoded as different polarization states of the light, is particularly appealing because photons are robust against decoherence effects and can be transported over long distances. The photons, however, need to be indistinguishable; i.e., identical and in a pure quantum state. Although techniques exist for the generation for single photons, determining whether they are in fact indistinguishable and pure has generally required a postselection or spectral filtering process that compromises their quantum utility. By careful design of the parametric downconversion process, in which a single photon is divided into two entangled photons, Mosley et al. show that restricting the optical modes into which the photon pairs emerge can provide a method for the generation of heralded (by measurement of one member of the pair) indistinguishable single photons of high purity. — ISO
We analyze the quantum-state purity of heralded single photons produced from frequency-anticorrelated biphotons. We find that the quantum-state purity in the time-frequency domain depends strongly on the response time uncertainty of the trigger-photon detector that heralds the generation of its paired photon. If the trigger response time is much shorter than the two-photon coherence time, the time-frequency quantum-state purity of heralded single photons approaches unity and the heralded single photon is in a nearly pure state. If the trigger response time is much longer than the two-photon coherence time, the heralded photon is then projected onto a mixed state. Making use of the time-frequency entanglement, heralded single photons with a well-defined temporal wave function or a frequency superposition state can be produced and engineered. This time-frequency entanglement allows for shaping heralded single photons through nonlocal spectral modulation.
Sources of single photons in pure quantum states are essential to many quantum optics applications. We explore a technique, known as group-velocity matching, that enables the heralded generation of pure single photons through nonlinear optical processes. It reduces or eliminates the requirement of spectral filtering that conventional sources rely on to achieve high purity, therefore increasing both heralding efficiency and photon flux. Implementation in both spontaneous parametric downconversion and spontaneous four-wave mixing is studied as we discuss several recent experimental realizations demonstrating purity of more than 0.84 for the heralded photons.
Photon pairs produced by parametric down-conversion or four-wave mixing can interfere with each other in multiport interferometers or carry entanglement between distant nodes for use in entanglement swapping. This requires the photons to be spectrally pure to ensure good interference and have high heralding efficiency to know accurately the number of photons involved and to maintain high rates as the number of photons grows. Spectral filtering is often used to remove noise and define spectral properties. For heralded single photons high purity and heralding efficiency are possible by filtering the heralding arm, but when both photons in typical pair sources are filtered, we show that the heralding efficiency of one or both of the photons is strongly reduced even by ideal spectral filters with 100% transmission in the passband: any improvement in reduced-state spectral purity from filtering comes at the cost of lowered heralding efficiency. We consider the fidelity to a pure, lossless single photon, symmetrize it to include both photons of the pair, and show this quantity is intrinsically limited for sources with spectral correlation. We then provide a framework for this effect for benchmarking common photon-pair sources and present an experiment where we vary the photon filter bandwidths and measure the increase in purity and corresponding reduction in heralding efficiency.