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arXiv:1008.1549 · Physical Review A

Stimulated Raman adiabatic passage in a Λ system in the presence of quantum noise

M. Scala, Benedetto Militello, ANTONINO MESSINA, Nikolay V. Vitanov

Published Jan 10, 2011• 29 citations
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Abstract

We exploit a microscopically derived master equation for the study of stimulated Raman adiabatic passage in the presence of spontaneous decay from the intermediate state toward the initial and final states and compare our results with the predictions obtained from a phenomenological model used previously [P. A. Ivanov, N. V. Vitanov, and K. Bergmann, Phys. Rev. A 72, 053412 (2005)]. It is shown that our approach predicts a much higher efficiency for counterintuitively ordered pulses, while no significant difference between the two approaches is found for intuitively ordered pulses. These features are readily explained in the dressed-state picture.

DOI
10.1103/physreva.83.012101

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We exploit a microscopically derived master equation for the study of stimulated Raman adiabatic passage in the presence of spontaneous decay from the intermediate state toward the initial and final states and compare our results with the predictions obtained from a phenomenological model used previously [P. A. Ivanov, N. V. Vitanov, and K. Bergmann, Phys. Rev. A 72, 053412 (2005)]. It is shown that our approach predicts a much higher efficiency for counterintuitively ordered pulses, while no significant difference between the two approaches is found for intuitively ordered pulses. These features are readily explained in the dressed-state picture.
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This paper begins with the premise that stimulated Raman adiabatic passage (STIRAP) from one state to another by coupling to an intermediate state necessarily requires some population of that intermediate state. The usual view of the process depends on having no population in the intermediate state, but a simple argument from the time-dependent Schr\"odinger equation shows that such adiabatic transfer cannot occur. From another perspective, removing the time dependence of the Hamiltonian by making the rotating frame transformation cancels the optical frequency oscillations but does not account for the envelopes of the pulses commonly used for STIRAP. By assuming a small but finite intermediate state amplitude ${\ensuremath{\varepsilon}}_{1}$ in the wave function, the propagator for the evolution between initial and final states is derived. Applying the propagator to the initial state produces a single compact formula for the final intermediate-state population that is readily evaluated for an arbitrary choice of laser pulse parameters. Several plots for various experimental conditions show that under the conditions normally used for STIRAP experiments the effects are typically a few percent or less, but in the end this effect puts an ultimate limit on total efficiency.
We propose a technique which produces nearly complete ionization of the population of a discrete state coupled to a continuum by a two-photon transition via a lossy intermediate state whose lifetime is much shorter than the interaction duration. We show that using counterintuitively ordered pulses, as in stimulated Raman adiabatic passage (STIRAP), wherein the pulse coupling the intermediate state to the continuum precedes and partly overlaps the pulse coupling the initial and intermediate states, greatly increases the ionization signal and strongly reduces the population loss due to spontaneous emission through the lossy state. For strong spontaneous emission from that state, however, the ionization is never complete because the dark state required for STIRAP does not exist. We demonstrate that this drawback can be eliminated almost completely by creating a laser-induced continuum structure (LICS) by embedding a third discrete state into the continuum with a third control laser. This LICS introduces some coherence into the continuum, which enables a STIRAP-like population transfer into the continuum. A highly accurate analytic description is developed and numerical results are presented for Gaussian pulse shapes.
We present an analytic description of the effects of dephasing processes on stimulated Raman adiabatic passage in a tripod quantum system. To this end, we develop an effective two-level model. Our analysis makes use of the adiabatic approximation in the weak dephasing regime. An effective master equation for a two-level system formed by two dark states is derived, where analytic solutions are obtained by utilizing the Demkov-Kunike model. From these, it is found that the fidelity for the final coherent superposition state decreases exponentially for increasing dephasing rates. Depending on the pulse ordering and for adiabatic evolution, the pulse delay can have an inverse effect.
Different adiabatic passage methods are applied as part of a state mapping scheme in multilevel trapped systems. The aim is to achieve full population transfer from the rotational states of a trapped molecular ion to its translational states. Our analysis is based on numerical simulations with the master equation. We discuss how the resolved sideband condition, and spontaneous emission have an adverse effect on the efficiency for stimulated Raman adiabatic passage. Use of adiabatic rapid passage techniques, with two-photon Raman transitions results in higher efficiencies that can exceed 97%.