We review the progress and main challenges in implementing large-scale quantum computing by optical control of electron spins in quantum dots (QDs). Relevant systems include self-assembled QDs of III–V or II–VI compound semiconductors (such as InGaAs and CdSe), monolayer fluctuation QDs in compound semiconductor quantum wells, and impurity centres in solids, such as P-donors in silicon and nitrogen-vacancy centres in diamond. The decoherence of the electron spin qubits is discussed and various schemes for countering the decoherence problem are reviewed. We put forward designs of local nodes consisting of a few qubits which can be individually addressed and controlled. Remotely separated local nodes are connected by photonic structures (microcavities and waveguides) to form a large-scale distributed quantum system or a quantum network. The operation of the quantum network consists of optical control of a single electron spin, coupling of two spins in a local nodes, optically controlled quantum interfacing between stationary spin qubits in QDs and flying photon qubits in waveguides, rapid initialization of spin qubits and qubit-specific single-shot non-demolition quantum measurement. The rapid qubit initialization may be realized by selectively enhancing certain entropy dumping channels via phonon or photon baths. The single-shot quantum measurement may be in situ implemented through the integrated photonic network. The relevance of quantum non-demolition measurement to large-scale quantum computation is discussed. To illustrate the feasibility and demand, the resources are estimated for the benchmark problem of factorizing 15 with Shor's algorithm.
We review the progress and main challenges in implementing large-scale quantum computing by optical control of electron spins in quantum dots (QDs). Relevant systems include self-assembled QDs of III–V or II–VI compound semiconductors (such as InGaAs and CdSe), monolayer fluctuation QDs in compound semiconductor quantum wells, and impurity centres in solids, such as P-donors in silicon and nitrogen-vacancy centres in diamond. The decoherence of the electron spin qubits is discussed and various schemes for countering the decoherence problem are reviewed. We put forward designs of local nodes consisting of a few qubits which can be individually addressed and controlled. Remotely separated local nodes are connected by photonic structures (microcavities and waveguides) to form a large-scale distributed quantum system or a quantum network. The operation of the quantum network consists of optical control of a single electron spin, coupling of two spins in a local nodes, optically controlled quantum interfacing between stationary spin qubits in QDs and flying photon qubits in waveguides, rapid initialization of spin qubits and qubit-specific single-shot non-demolition quantum measurement. The rapid qubit initialization may be realized by selectively enhancing certain entropy dumping channels via phonon or photon baths. The single-shot quantum measurement may be in situ implemented through the integrated photonic network. The relevance of quantum non-demolition measurement to large-scale quantum computation is discussed. To illustrate the feasibility and demand, the resources are estimated for the benchmark problem of factorizing 15 with Shor's algorithm.
Single spins in semiconductor quantum dots form a promising platform for solid-state quantum information processing. The spin-up and spin-down states of a single electron or hole, trapped inside a quantum dot, can represent a single qubit with a reasonably long decoherence time. The spin qubit can be optically coupled to excited (charged exciton) states that are also trapped in the quantum dot, which provides a mechanism to quickly initialize, manipulate and measure the spin state with optical pulses, and to interface between a stationary matter qubit and a 'flying' photonic qubit for quantum communication and distributed quantum information processing. The interaction of the spin qubit with light may be enhanced by placing the quantum dot inside a monolithic microcavity. An entire system, consisting of a two-dimensional array of quantum dots and a planar microcavity, may plausibly be constructed by modern semiconductor nano-fabrication technology and could offer a path toward chip-sized scalable quantum repeaters and quantum computers. This article reviews the recent experimental developments in optical control of single quantum dot spins for quantum information processing. We highlight demonstrations of a complete set of all-optical single-qubit operations on a single quantum dot spin: initialization, an arbitrary SU(2) gate, and measurement. We review the decoherence and dephasing mechanisms due to hyperfine interaction with the nuclear-spin bath, and show how the single-qubit operations can be combined to perform spin echo sequences that extend the qubit decoherence from a few nanoseconds to several microseconds, more than 5 orders of magnitude longer than the single-qubit gate time. Two-qubit coupling is discussed, both within a single chip by means of exchange coupling of nearby spins and optically induced geometric phases, as well as over longer-distances. Long-distance spin-spin entanglement can be generated if each spin can emit a photon that is entangled with the spin, and these photons are then interfered. We review recent work demonstrating entanglement between a stationary spin qubit and a flying photonic qubit. These experiments utilize the polarization- and frequency-dependent spontaneous emission from the lowest charged exciton state to single spin Zeeman sublevels.
Single electron spin in a semiconductor quantum dot (QD) and single photon wavepacket propagating in an optical waveguide are investigated as carriers of quantum bit (qubit) for information processing. Cavity quantum electrodynamics of the coupled system composed of charged QD, microcavity and waveguide provides a quantum interface for the interplay of stationary spin qubits and flying photon qubits via cavity assisted optical control. This interface forms the basis for a wide range of essential functions of a quantum network, including transferring, swapping, and entangling qubits at distributed quantum nodes as well as a deterministic source and an efficient detector of a single photon wavepacket with arbitrarily specified shape. The cavity assisted optical process also made possible ultrafast initialization and QND readout of the spin qubit in QD. In addition, the strong optical nonlinearity of dot-cavity-waveguide coupled system enables phase gate and entanglement operation for flying single photon qubits in waveguides. The coherence of the electron spin is the wellspring of these quantum applications being investigated. At low temperature and strong magnetic field, the dominant cause of electron spin decoherence is the coupling with the interacting lattice nuclear spins. We present a quantum solution to the coupled dynamics of the electron with the nuclear spin bath. The decoherence is treated in terms of quantum entanglement of the electron with the nuclear pair-flip excitations driven by the various nuclear interactions. A novel nuclear interaction, mediated by virtue spin-flips of the single electron, plays an important role in single spin free-induction decay (FID). The spin echo not only refocuses the dephasing by inhomogeneous broadening in ensemble dynamics but also eliminates the decoherence by electron-mediated nuclear interaction. Thus, the decoherence times for single spin FID and ensemble spin echo are significantly different. The quantum theory of decoherence also leads to a method of coherence recovery of the electron by disentanglement, realized through maneuvering the nuclear bath evolution by control of the electron spin-flip. The studies form the basis to outline the construction of a solid-state quantum network for scalable and distributed processing of quantum information
A fascinating dream in quantum information science is to build quantum computers with super-performance and quantum networks with unconditional security [1]. Quantum networks utilize static (matter) quantum bits (qubits) to store and process quantum information at local nodes, and photons as flying qubits for long-distance quantum state transmission between different nodes. To realize a quantum network, it is crucial to achieve light-matter entanglement and reversible quantum-state transfer between light and matter, i.e., the light-matter quantum interface, and the quantum repeater for large-scale quantum communications [2]. Recent experiments have shown that both electrons and holes confined in semiconductor quantum dots (QDs) have long spin relaxation time (T1e, T1h ~ ms) and long spin coherence time (T2e ~ microseconds, T2h > 100 ns). Moreover, fast spin cooling and ultra-fast spin manipulation as well as spin echoes to preserve the spin coherence have also been demonstrated. Undoubtedly these rapid progresses imply that the QD spin is a good candidate for matter qubit in quantum information processing. Furthermore, QD-based single photon sources have been also developed. Therefore, semiconductor QDs offer a good platform for solid-state quantum networking and quantum computation. Here we present two types of conditional quantum gates, i.e., the photon-spin entangling gates [3-4] using a single QD spin in a single-sided or double-sided optical microcavity. Both gates are universal and deterministic (if they are optimized). The spin-selective coherent photon-spin interaction enhanced by the cavity QED lead to giant circular birefringence, which allows us to build these gates. We will show the versatile spin-cavity systems can be applied in all aspects of quantum information science and technology, not only for large-scale quantum communication networks (solid-state quantum repeaters) [5], but also for scalable quantum computing with either photons or spins as qubits. We will also discuss other applications using these gates, such as photon-number resolving detection, quantum feed-back control, loss-resistant quantum metrology, and loophole-free Bell test [6], and other devices based on optical nonlinearity at single-photon levels in these gate structures. All these schemes are feasible with current semiconductor technology [7], and we have recently seen conditional phase shifts in uncharged QD-cavity systems [8]. References [1] H.J. Kimble, Nature (London) 453, 1023 (2008). [2] H.-J. Briegel et al., Phys. Rev. Lett. 81, 5932 (1998). [3] C.Y. Hu et al., Phys. Rev. B 78, 085307 (2008); ibid. 78, 125318 (2008). [4] C.Y. Hu et al., Phys. Rev. B 80, 205326 (2009). [5] C.Y. Hu and J.G. Rarity, Phys. Rev. B 83, 115303 (2011). [6] N. Brunner et al., Arxiv: quant-phys 1303.6522 (2013). [7] S. Reitzenstein et al., Appl. Phys. Lett. 90, 251109 (2007). [8] A.B. Young et al., Phys. Rev. A 84, 011803 (2011).
The ultimate goal of quantum information science is to build quantum networks for distributed quantum computing or for the secure sharing of information between spatially remote parties [1]. Quantum networks utilize static (matter) quantum bits (qubits) to store and process quantum information at local nodes, and photons as flying qubits for long-distance quantum state transmission between different nodes. To realize a quantum network, it is crucial to achieve light-matter entanglement and reversible quantum-state transfer between light and matter, i.e., the light-matter quantum interface, and the quantum repeater for large-scale quantum communications [2]. Recent experiments have shown that both electrons and holes confined in semiconductor quantum dots (QDs) have long spin relaxation time (T1e, T1h ~ ms) and long spin coherence time (T2e ~ s, T2h > 100 ns). Moreover, fast spin cooling and ultra-fast spin manipulation as well as spin echoes to preserve the spin coherence have also been demonstrated. Undoubtedly these rapid progresses imply that the QD spin is a good candidate for matter qubit in quantum information processing. Furthermore, QD-based single photon sources have been also developed. Therefore, semiconductor QDs offer a good platform for solid-state quantum networking. Here we present two types of conditional quantum gates, i.e., the photon-spin entangling gates [3-4] using a single QD spin in a single-sided or double-sided optical microcavity. Both gates are universal and deterministic (if they are optimized). The spin-selective coherent photon-spin interaction enhanced by the cavity QED lead to giant circular birefringence, which allows us to build these gates. We will show some of the key applications [3-5], including: (i) single-shot quantum non-demolition measurement of spin; (ii) single-photon based spin manipulations and spin echoes to preserve the spin coherence; (iii) photon-spin, spin-spin and photon-photon entanglement generation with high fidelity and high efficiency; (iv) deterministic photon-spin interface and perfect spin memory; (v) complete and loss-resistant Bell-state analyzer, which could increase the distance of state-of-the-art quantum communications by one order of magnitude (from current 100 km to over 1000 km) [5]; (vi) the full quantum repeater combining quantum memory, entanglement swapping and purifications for arbitrary long distance communications [5]; (vii) spin-controlled single photon sources. All these schemes are feasible with current semiconductor technology [6], and we have recently seen conditional phase shifts in uncharged QD-cavity systems [7]. The versatile spin-cavity systems can be applied in all aspects of quantum information science and technology, not only for large-scale quantum communication networks, but also for scalable quantum computing with either photons or spins as qubits. References [1] H.J. Kimble, Nature (London) 453, 1023 (2008). [2] H.-J. Briegel et al., Phys. Rev. Lett. 81, 5932 (1998). [3] C.Y. Hu et al., Phys. Rev. B 78, 085307 (2008); ibid. 78, 125318 (2008). [4] C.Y. Hu et al., Phys. Rev. B 80, 205326 (2009). [5] C.Y. Hu and J.G. Rarity, ArXiv: quant-ph 1005.5545 (2010). [6] S. Reitzenstein et al., Appl. Phys. Lett. 90, 251109 (2007). [7] A.B. Young et al., ArXiv: quant-ph 1011.0384 (2010).
The recent discovery of efficient quantum algorithms for factoring and database search has shown that quantum computing would allow to solve important problems which are intractable with conventional computers. In contrast to the very demanding task of building a large-scale quantum computer, there are quantum communication protocols, e.g. quantum key distribution for cryptography, which—though still difficult—require much less effort and can be implemented with current technology. Apart from the technological motivation, the study of quantum information offers (at least) two additional benefits. First, new insight into fundamental questions on quantum mechanics, e.g. concerning non-locality and entanglement, are gained from an information-theoretical approach. And second, investigating a particular physical implementation of quantum information can give rise to independent physical results. Spintronics, the use of spin as opposed to charge in (classical) electronics is a new field for which some results presented here could be relevant. In this dissertation we investigate several theoretical aspects of the physical implementation of quantum computation and communication in which the fundamental unit of quantum information, the qubit, is represented by the spin of electrons in semiconductor quantum dots. The required coupling between the spins can be obtained by allowing for tunneling of electrons between adjacent dots, leading to a Heisenberg exchange coupling J S1 · S2 between the spins, a scenario which we study for laterally coupled quantum dots in a two-dimensional electron system, and for a three-dimensional setup with vertically coupled quantum dots. Furthermore, an alternative scheme to couple the spins via the interaction with an optical cavity mode is presented. Quantum error correction represents one of the important ingredients for the physical implementation of a quantum computer by protecting \nit from the e�ects of a noisy environment. As a �rst test for errorcorrection \nin a solid-state device using spins, we propose an optimized \nimplementation of the most primitive error correction scheme (the threebit \ncode). In this context, we introduce parallel switching, allowing \nto operate a quantum computer more e�ciently than the usual serial \nswitching. \nCoupling spins with the exchange interaction J S1 �S2 is not su�cient \nfor quantum computation; the spins also have to be addressed individually \nusing controllable local magnetic �elds or g-factors giBi �Si in order \nto allow for single-qubit operations. On the one hand, we discuss several \nschemes for overcoming the di�culty of applying local magnetic �elds \n(requiring large gradients), e.g. g-factor engineering, which allows for \nall-electric operation of the device. On the other hand, we show that \nat the expense of additional devices (spins) and switching operations, \nsingle-spin rotations can be dispensed with completely. \nAddressing the feasibility of quantum communication with entangled \nelectrons in mesoscopic wires, i.e. interacting many-body environments, \nwe propose an interference experiment using a scattering set-up with an \nentangler and a beam splitter. The current noise for electronic singlet \nstates turns out to be enhanced (bunching), while it is reduced for triplets \n(antibunching). Due to interactions, the �delity of the entangled singlet \nand triplet states is reduced by z4F \nin a conductor described by Fermi \nliquid theory, zF being the quasiparticle weight factor. \nFinally, we study the related but more general problem of the noise of \nthe cotunneling current through one or several tunnel-coupled quantum \ndots in the Coulomb blockade regime. The various regimes of weak and \nstrong, elastic and inelastic cotunneling are analyzed for quantum-dot \nsystems (QDS) with few-level, nearly-degenerate, and continuous electronic \nspectra. In contrast to sequential tunneling, the noise in inelastic \ncotunneling can be super-Poissonian. In order to investigate strong cotunneling \nwe develop a microscopic theory of cotunneling based on the \ndensity-operator formalism and using the projection operator technique. \nWe have derived the master equation for the QDS and the current and \nnoise in cotunneling in terms of the stationary state of the QDS. These \nresults are then applied to QDS with a nearly degenerate and continuous \nspectrum.
Self-assembled quantum dots (QDs) containing a single electron are one of the leading candidate systems for the realization of a quantum computer. The spin states of charges confined in these dots have been shown to possess a number of qualities that are attractive for use as the quantum bits (qubits) in quantum computing implementations, particularly their long lifetimes and coherence times. In addition, these spin qubits may be controlled optically, offering the prospect of ultrafast qubit gate operations, a crucial necessity for the execution of quantum algorithms. Due to the weak interaction of self-assembled QDs with light, however, the coherent optical control and read-out of the spin states of charged self-assembled QDs has proven to be a considerable challenge. This thesis presents two sets of experiments demonstrating the coherent optical control and read-out of the quantum states of a self-assembled InAs QD containing a single electron. The first utilizes mode-locked picosecond optical pulses to control the optical transitions in the dot and to detect QD level occupations. These capabilities are used to observe transient phenomena in a singly charged InAs QD such as the generation and decay of excited state population and spin precession. Further, Rabi oscillations between the electron and the lowest-lying excited state are observed, demonstrating the ability to coherently control the optical transitions of the QD, a prerequisite for spin control. These results are built upon in the second set of experiments, in which a combination of optical pulses, an externally applied DC magnetic field and a continuous-wave (CW) optical field are employed to initialize and completely control the states of a QD confined electron spin. Spin control by the use of pulse-driven two-photon Raman processes, spin precession about the external magnetic field and geometric phases generated by CW-driven cyclic evolutions in the dot is demonstrated. A number of spin qubit gate operations are shown for these spin control mechanisms, forming a foundational set of single qubit gates required for the implementation of quantum computing with singly charged self-assembled QDs.