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arXiv:1005.2807 · Physical Review Letters

Quantum Nondemolition Measurement of Large-Spin Ensembles by Dynamical Decoupling

Marco Koschorreck, M. Napolitano, B. Dubost, Morgan W. Mitchell

Published Aug 25, 2010• 85 citations
arXivHTMLPDF

Abstract

Quantum nondemolition (QND) measurement of collective variables by off-resonant optical probing has the ability to create entanglement and squeezing in atomic ensembles. Until now, this technique has been applied to real or effective spin one-half systems. We show theoretically that the buildup of Raman coherence prevents the naive application of this technique to larger spin atoms, but that dynamical decoupling can be used to recover the ideal QND behavior. We experimentally demonstrate dynamical decoupling by using a two-polarization probing technique. The decoupled QND measurement achieves a sensitivity 5.7(6) dB better than the spin projection noise.

DOI
10.1103/physrevlett.105.093602

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At the beginning of the 20th century measurement precision was related exclusively to the capabilities of the experimenter and the apparatus. Any imprecision was attributed to imperfect devices for the measurement. Later on, when the quantumness of objects like photons, electrons, or atoms, was recognized, it became clear that the measurement and the object to be measured could no longer be separated. Both follow the laws of quantum physics which impose limits on the accuracy of any measurement. In the last three decades, a lot of research has been dedicated to find strategies to overcome these limitations. This new field of quantum metrology is where this work is placed. This thesis describes the generation of interparticle entanglement in form of a squeezed spin state in a cloud of cold 87Rb atoms by performing nondestructive spin measurements. Towards this goal, we have implemented a shot-noise limited polarization probing and detection system, atom counting by means of absorption imaging, spin state preparation via optical pumping and nondestructive spin state detection. The quantum noise limited spin readout with polarized light is characterized in two complementary ways in terms of sensitivity and all possible quantum and classical noise sources are measured. To address the rich opportunities provided in the multilevel structure of 87Rb with dispersive probing, we have developed and implemented a frequency offsetlock which allows a large tuning range of several GHz for the dispersive probing. Working with a magnetically sensitive atomic system triggered the development of a magnetic field imaging technique. This applies the elongated atomic sample and internal atomic states as a way of measuring magnetic fields over several millimeters with micrometer resolution and sensitivities down to a few tens of pT/ Hz. We developed a new method for tomographic measurements of the atomic density matrix. Based on our ability of shot noise limited detection of polarization rotations we can in principle, characterize the whole atomic spin state. First, measurements are shown and possible improvements are discussed. An in depth characterization of the light-atom interaction between polarized pulses of light and collective atomic states are the basis for measurements at the quantum level. On one side, we apply classical measurements of spin polarized atoms to measure the strength of the lightatom interaction. On the other side, we use quantum measurements of unpolarized atomic states to characterize all noise sources both technical and quantum. One of the major results of this thesis is the realization of quantum nondemolition measurements in a largespin system. We realized limitations to the performance of the QND measurement implied by higher order light shifts in multilevel atoms, which are often neglected for these kind of systems. We develop a technique which suppresses the detrimental effects of higher order light shifts and recovers an ideal QND measurement. The thesis culminates in the demonstration of spin squeezing in the magnetically sensitive ground state of 87Rb. We achieve a quantum noise reduction by 3 dB, where metrological sensitivity is improved by 2 dB beyond the standard quantum limit of a coherent spin state with the same spin polarization. We address the question how spatial and temporal inhomogeneities both in light and atoms influence the preparation of nonclassical states. An existing covariance matrix approach is extended and we apply it to study effects of detector time resolution, spatial inhomogeneities and atomic motion.

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Quantum nondemolition (QND) measurement of collective variables by off-resonant optical probing has the ability to create entanglement and squeezing in atomic ensembles. Until now, this technique has been applied to real or effective spin one-half systems. We show theoretically that the buildup of Raman coherence prevents the naive application of this technique to larger spin atoms, but that dynamical decoupling can be used to recover the ideal QND behavior. We experimentally demonstrate dynamical decoupling by using a two-polarization probing technique. The decoupled QND measurement achieves a sensitivity 5.7(6) dB better than the spin projection noise.
We demonstrate spin squeezing and entanglement in a large-spin system via quantum non-demolition measurement. We make non-destructive, projection-noise-limited collective spin measurements on an ensemble of up to in 8.4 × 105 laser-cooled 87Rb atoms in the f = 1 hyperfine ground state. A dynamically-decoupled probing scheme [Phys. Rev. Lett. 105, 093602 (2010)] prevents probe-induced decoherence. Repeated measurements show correlations beyond the standard quantum limit, indicating generation of a spin-squeezed state with up to −3.6 dB of noise reduction and −2.6 dB of metrologically-relevant squeezing.
Large ensembles of uncorrelated atoms are extensively used as precise sensors of time, rotation, and gravity, and for tests of fundamental physics. The quantum nature of the sensors imposes a limit on their ultimate precision. Larger ensembles of N atoms can be used to average the quantum noise as 1/√N, a scaling known as the standard quantum limit. However, the ensemble size may be limited by technical constraints and/or atom-atom collisions -- a fundamental distinction from photon-based sensors. Learning to prepare entangled states of large ensembles with noise properties below the standard quantum limit will be key to extending both the precision and/or bandwidth of atomic sensors. More broadly, the generation and application of entanglement to solve problems is a core goal of quantum information science being pursued in both atomic and solid state systems.\nIn this thesis, we utilize the tools of cavity-QED to prepare entangled spin-squeezed states with 3.4(6) dB improvement in spectroscopic sensitivity over the standard quantum limit. The collective atomic spin is composed of the two-level clock states of 87Rb confined in a medium finesse F = 710 optical cavity. We employ cavity-aided quantum non-demolition measurements of the vacuum Rabi splitting to measure and subtract out the quantum projection noise of the collective spin state, preparing states with collective atomic spin projection noise 4.9(6) dB below the projection noise level. The conditionally reduced spin noise combined with the measured 1.5(3) dB reduction in the mean spin length implies a net 3.4(6) dB spectroscopic enhancement or conditional squeezing as defined by the Wineland criterion. Our method does not require single particle addressability and is applied to a spectroscopically large ensemble of N = 7 x 105 atoms using two collective population measurements, with the whole squeezing operation taking ~ 150 μs. The gain in sensitivity is spectroscopically equivalent to the enhancement obtained had we created > 105 pairs of maximally entangled qubits, demonstrating the power of a top-down approach for entangling large ensembles. The nondemolition probing of atomic populations via the vacuum Rabi splitting is also of broad interest for non-destructively reading out a wide variety of both atomic and solid state qubits.
Ultimate quantum fluctuations which limit the fundamental precision in metrology can be only reduced by entanglement of particles. In particular, squeezing of the fluctuations called the spin projection noise by means of generation of entanglement in an ensemble of atoms can improve the precision of spectroscopy and of atomic clocks. A powerful tool for generation of multiparticle entanglement is a quantum nondemolition measurement (QND). We will describe the fundamentals of QND measurement of atomic collective state with light and present a recent experiment [1] where this method has been used to reduce the projection noise on the clock transition in an ensemble of 105 cold and trapped Cesium atoms. Another method for generation of spin squeezing via electron-nucleus entanglement applicable only for atoms with angular momentum higher than ½ will be also discussed [2].
Squeezing of collective atomic spins has been shown to improve the sensitivity of atomic clocks and magnetometers to levels significantly below the standard quantum limit. In most cases the requisite atom-atom entanglement has been generated by dispersive interaction with a quantized probe field or by state-dependent collisions in a quantum gas. Such experiments typically use complex multilevel atoms like Rb or Cs, with the relevant interactions designed so that atoms behave like pseudospin-12\frac{1}{2}21​ particles. We demonstrate the viability of spin squeezing for collective spins composed of the physical angular momenta of 106{10}^{6}106 Cs atoms, each in an internal spin-4 hyperfine state. A peak metrological squeezing of at least 5dB is generated by quantum backaction from a dispersive quantum nondemolition (QND) measurement, implemented using a two-color optical probe that minimizes tensor light shifts without sacrificing measurement strength. Other significant developments include the successful application of composite pulse techniques for accurate dynamical control of the collective spin, enabled by broadband suppression of background magnetic fields inside a state-of-the-art magnetic shield. The absence of classical noise allows us to compare the observed quantum projection noise and squeezing to a theoretical model that properly accounts for both the relevant atomic physics and the spatial mode of the collective spin, finding good quantitative agreement and thereby validating its use in other contexts. Our work sets the stage for experiments on quantum feedback, deterministic squeezing, and closed-loop magnetometry. The implementation of real-time feedback may also create an opportunity for new types of quantum simulation, wherein the evolution of a quantum system is conditioned on the outcome of a time-continuous QND measurement. Such a scheme has the potential to access new regimes near the quantum-classical boundary, with opportunities to study long-standing issues related to quantum-classical correspondence in chaotic systems.
Quantum nondemolition (QND) measurement enhances the detection efficiency and measurement fidelity, and is highly desired for its applications in precision measurements and quantum information processing. We propose and demonstrate a QND measurement scheme for the spin states of laser-trapped atoms. On 171Yb{}^{171}\mathrm{Yb}171Yb atoms held in an optical dipole trap, a transition that is simultaneously cycling, spin-selective, and spin-preserving is created by introducing a circularly polarized beam of a control laser to optically dress the spin states in the excited level, while leaving the spin states in the ground level unperturbed. We measure the phase of spin precession of $5\ifmmode\times\else\texttimes\fi{}{10}^{4}$ atoms in a bias magnetic field of 20 mG. This QND approach reduces the optical absorption detection noise by $\ensuremath{\sim}19\phantom{\rule{0.2em}{0ex}}\mathrm{dB}$, to an inferred level of 2.3 dB below the atomic quantum projection noise. In addition to providing a general approach for efficient spin-state readout, this all-optical technique allows quick switching and real-time programming for quantum sensing and quantum information processing.
At the beginning of the 20th century measurement precision was related exclusively to the capabilities of the experimenter and the apparatus. Any imprecision was attributed to imperfect devices for the measurement. Later on, when the quantumness of objects like photons, electrons, or atoms, was recognized, it became clear that the measurement and the object to be measured could no longer be separated. Both follow the laws of quantum physics which impose limits on the accuracy of any measurement. In the last three decades, a lot of research has been dedicated to find strategies to overcome these limitations. This new field of quantum metrology is where this work is placed. This thesis describes the generation of interparticle entanglement in form of a squeezed spin state in a cloud of cold 87Rb atoms by performing nondestructive spin measurements. Towards this goal, we have implemented a shot-noise limited polarization probing and detection system, atom counting by means of absorption imaging, spin state preparation via optical pumping and nondestructive spin state detection. The quantum noise limited spin readout with polarized light is characterized in two complementary ways in terms of sensitivity and all possible quantum and classical noise sources are measured. To address the rich opportunities provided in the multilevel structure of 87Rb with dispersive probing, we have developed and implemented a frequency offsetlock which allows a large tuning range of several GHz for the dispersive probing. Working with a magnetically sensitive atomic system triggered the development of a magnetic field imaging technique. This applies the elongated atomic sample and internal atomic states as a way of measuring magnetic fields over several millimeters with micrometer resolution and sensitivities down to a few tens of pT/ Hz. We developed a new method for tomographic measurements of the atomic density matrix. Based on our ability of shot noise limited detection of polarization rotations we can in principle, characterize the whole atomic spin state. First, measurements are shown and possible improvements are discussed. An in depth characterization of the light-atom interaction between polarized pulses of light and collective atomic states are the basis for measurements at the quantum level. On one side, we apply classical measurements of spin polarized atoms to measure the strength of the lightatom interaction. On the other side, we use quantum measurements of unpolarized atomic states to characterize all noise sources both technical and quantum. One of the major results of this thesis is the realization of quantum nondemolition measurements in a largespin system. We realized limitations to the performance of the QND measurement implied by higher order light shifts in multilevel atoms, which are often neglected for these kind of systems. We develop a technique which suppresses the detrimental effects of higher order light shifts and recovers an ideal QND measurement. The thesis culminates in the demonstration of spin squeezing in the magnetically sensitive ground state of 87Rb. We achieve a quantum noise reduction by 3 dB, where metrological sensitivity is improved by 2 dB beyond the standard quantum limit of a coherent spin state with the same spin polarization. We address the question how spatial and temporal inhomogeneities both in light and atoms influence the preparation of nonclassical states. An existing covariance matrix approach is extended and we apply it to study effects of detector time resolution, spatial inhomogeneities and atomic motion.