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arXiv:1002.4746 · Physical Review A

Quantum-information-processing architecture with endohedral fullerenes in a carbon nanotube

W. L. Yang, Zhen Xu, H. Wei, Mang Feng, Dieter Suter

Published Mar 5, 2010• 46 citations
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Abstract

A potential quantum-information processor is proposed using an array of the endohedral fullerenes $^{15}\mathrm{N}@{\mathrm{C}}_{60}$ or $^{31}\mathrm{P}@{\mathrm{C}}_{60}$ contained in a single walled carbon nanotube (SWCNT). The qubits are encoded in the nuclear spins of the doped atoms, while the electronic spins are used for initialization and readout, as well as for two-qubit operations.

DOI
10.1103/physreva.81.032303

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A potential quantum-information processor is proposed using an array of the endohedral fullerenes 15N@C60^{15}\mathrm{N}@{\mathrm{C}}_{60}15N@C60​ or 31P@C60^{31}\mathrm{P}@{\mathrm{C}}_{60}31P@C60​ contained in a single walled carbon nanotube (SWCNT). The qubits are encoded in the nuclear spins of the doped atoms, while the electronic spins are used for initialization and readout, as well as for two-qubit operations.
We propose a scheme to implement the two-qubit gates between the nuclear spins of the encapsulated atoms in endohedral fullerenes 15N@C60^{15}\mathrm{N}@{\mathrm{C}}_{60}15N@C60​ or 31P@C60^{31}\mathrm{P}@{\mathrm{C}}_{60}31P@C60​, within today's magnetic resonance techniques. Since there is no interaction between the nuclear spins, this scheme employs the electronic spins as medium and two swap operations are proposed to transfer the information between the nuclear spin 12\frac{1}{2}21​ and the electronic spin 32\frac{3}{2}23​, and between two electronic spins 32\frac{3}{2}23​. These two-qubit gates, along with the single-qubit rotation gates, compose a universal set of quantum gates in fullerene-based quantum computation.
We propose to carry out two-qubit quantum gates with only one-step operations on endohedral fullerenes N@C60N@C_{60}N@C60​ or P@C60P@C_{60}P@C60​. The qubits are stored in electronic spin degrees of freedom of the doped atom NNN or PPP. By means of the magnetic dipolar coupling between two neighboring fullerenes, the two-qubit controlled-NOT gate is performed by a selective microwave pulse, and the two-qubit conditional phase gate is done by simultaneous radiation by two detuned microwaves. We will show that our proposal is useful for both quantum gating and the readout of quantum information from the spin-based qubit state.
We present a scheme to perform universal quantum computation using global addressing techniques as applied to a physical system of endohedrally doped fullerenes. The system consists of an ABAB\mathcal{ABAB}ABAB linear array of group-V endohedrally doped fullerenes. Each molecule spin site consists of a nuclear spin coupled via a hyperfine interaction to an electron spin. The electron spin of each molecule is in a quartet ground state S=3/2.S=3/2.S=3/2. Neighboring molecular electron spins are coupled via a magnetic dipole interaction. We find that an all-electron construction of a quantum cellular automaton is frustrated due to the degeneracy of the electronic transitions. However, we can construct a quantum-cellular-automata quantum computing architecture using these molecules by encoding the quantum information on the nuclear spins while using the electron spins as a local bus. We deduce the NMR and ESR pulses required to execute the basic cellular automaton operation and obtain a rough figure of merit for the number of gate operations per decoherence time. We find that this figure of merit compares well with other physical quantum computer proposals. We argue that the proposed architecture meets well the first four DiVincenzo criteria and we outline various routes toward meeting the fifth criterion: qubit readout.
We propose a potentially practical scheme for quantum-information processing (QIP) with spatially distributed fullerene-caged electron spins using optical and microwave manipulations. Each doped fullerene located in a semiconducting single-walled carbon nanotube is embedded in a two-mode optical cavity. The caged spins have long decoherence time and the optical manipulation makes sure short operational time. Compared to the conventional QIP proposals involving an array of fullerene-caged electron spins based on nearest-neighbor coupling, our scheme corresponds to a network which could much reduce overhead in implementing distant qubits. We discuss the experimental feasibility and challenge based on currently available techniques and we show the possibility of high-fidelity operations.
We propose two potentially practical schemes to carry out two-qubit quantum gates on endohedral fullerenes N@C60\mathrm{N}@{\mathrm{C}}_{60}N@C60​ or P@C60\mathrm{P}@{\mathrm{C}}_{60}P@C60​. The qubits are stored in electronic spin degrees of freedom of the doped atom N or P. By means of the magnetic dipolar coupling between two neighboring fullerenes, the two-qubit controlled-NOT gate and the two-qubit conditional phase gate are performed by selective microwave pulses assisted by the refocusing technique. We will discuss the necessary additional steps for the universality of our proposal. We will also show that our proposal is useful for both quantum gating and the readout of quantum information from the spin-based qubit state.
We propose a scalable design for a solid-state spin-based quantum computer. It uses endohedral fullerenes like N@C60\mathrm{N}@{\mathrm{C}}_{60}N@C60​ or P@C60,\mathrm{P}@{\mathrm{C}}_{60},P@C60​, which can be positioned on Si surfaces with a scanning tunneling microscope. Each logical qubit is stored in two physical qubits, corresponding to the nuclear and electronic spins. We discuss the addressing of individual qubits by a magnetic field gradient, and the implementation of one- and two-qubit quantum gates by sequences of radio-frequency and microwave pulses.