The influence of pure dephasing on the dynamics of the coupling between a two-level atom and a cavity mode is systematically addressed. We have derived an effective atom-cavity coupling rate that is shown to be a key parameter in the physics of the problem, allowing to generalize the known expression for the Purcell factor to the case of broad emitters, and to define strategies to optimize the performances of broad emitter-based single-photon sources. Moreover, pure dephasing is shown to be able to restore lasing in presence of detuning, a further demonstration that decoherence can be seen as a fundamental resource in solid-state cavity quantum electrodynamics, offering appealing perspectives in the context of advanced nanophotonic devices. We propose experimental strategies to develop a versatile device that can be operated either as a single-photon source or as a laser, based on the control by decoherence of the coupling between a single quantum dot and a solid-state cavity.
The influence of pure dephasing on the dynamics of the coupling between a two-level atom and a cavity mode is systematically addressed. We have derived an effective atom-cavity coupling rate that is shown to be a key parameter in the physics of the problem, allowing to generalize the known expression for the Purcell factor to the case of broad emitters, and to define strategies to optimize the performances of broad emitter-based single-photon sources. Moreover, pure dephasing is shown to be able to restore lasing in presence of detuning, a further demonstration that decoherence can be seen as a fundamental resource in solid-state cavity quantum electrodynamics, offering appealing perspectives in the context of advanced nanophotonic devices. We propose experimental strategies to develop a versatile device that can be operated either as a single-photon source or as a laser, based on the control by decoherence of the coupling between a single quantum dot and a solid-state cavity.
We have computed the spectrum emitted spontaneously by a quantum dot coupled to an arbitrarily detuned single mode cavity, taking into account pure dephasing processes. We show that if the emitter is incoherent, the cavity can efficiently emit photons with its own spectral characteristics. This effect opens unique opportunities for the development of devices exploiting both cavity quantum electrodynamic effects and pure dephasing, such as wavelength-stabilized single-photon sources robust against spectral diffusion.
The quantum dot-cavity system was investigated using a quantum master equation that took incoherent pumping,stimulated emission and pure dephasing into consideration,and analytical emission spectra at cavity and dot were presented.The theoretical analysis results show that the pure dephasing shifts the emission intensity towards the cavity frequency in non-resonant coupling system and thus can be a very good explanation of the non-resonantly coupled cavity effective emission effect.In order to further study the application of pure dephasing in the quantum dot-cavity coupled systems,the effective quantum dot-cavity coupling rate and the efficiency of the single photon source for detuned systems were introduced,and good cavity and bad ragime were able to be defined through comparing the effective quantum dot-cavity coupling rate and the cavity decay rate.Influence of the pure dephasing on the efective coupling rate and the efficiency of the single photon source were investigated in resonance and detuning selected two set of theoretical parameters according to the experimental data.The results show that the pure dephasing can increase the efftive quantum dot-cavity coupling and the efficiency of single photon source for detuned system and thus may make a transition from bad cavity to good cavity ragime;a set of parameters having larger coupling efficiency in a certain range can meet good cavity ragime that its single photon sources efficiency is obviously better than the other set.Compared with bad cavity regime laser in non-resonant coupling system,the good cavity regime is a necessary condition to achieve single quantum dot lasers;the Fano function shows no evidence of a maximum in the non-resonant coupling system and thus there is no laser threshold in this system.
Solid-state emitters are excellent candidates for developing integrated sources of single photons. Yet, phonons degrade the photon indistinguishability both through pure dephasing of the zero-phonon line and through phonon-assisted emission. Here, we study theoretically and experimentally the indistinguishability of photons emitted by a semiconductor quantum dot in a microcavity as a function of temperature. We show that a large coupling to a high quality factor cavity can simultaneously reduce the effect of both phonon-induced sources of decoherence. It first limits the effect of pure dephasing on the zero-phonon line with indistinguishabilities above 97% up to 18 K. Moreover, it efficiently redirects the phonon sidebands into the zero-phonon line and brings the indistinguishability of the full emission spectrum from 87% (24%) without cavity effect to more than 99% (76%) at 0K (20K). We provide guidelines for optimal cavity designs that further minimize the phonon-induced decoherence.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
We investigate the dynamical behavior of entanglement in a system made of two solid-state emitters, as two quantum dots, embedded in two separated microcavities. In these solid-state systems, in addition to the coupling with the cavity mode, the emitter is coupled to a continuum of leaky modes providing additional losses and is also subjected to a phonon-induced pure dephasing mechanism. We model this physical configuration as a multipartite system composed of two independent parts each containing a qubit embedded in a single-mode cavity, exposed to cavity losses, spontaneous emission and pure dephasing. We study the time evolution of entanglement of this multipartite open system, finally applying this theoretical framework to the case of currently available solid-state quantum dots in microcavities.
Multi-photon lasing has been realized in systems with strong nonlinear interactions between emitters and cavity modes, where single-photon processes are suppressed. Coherence between the internal states of a quantum emitter, or among multiple emitters, plays a key role. Such continuous nonclassical sources of light can find applications in quantum computation, quantum sensing, quantum metrology, and quantum communication.
This thesis explores the multi-photon lasing phenomena in various quantum dot-photonic crystal cavity quantum electrodynamic (QED) setups. Exciton-phonon interactions are inevitable in such systems and are incorporated using the polaron-transformed master equation. The Born-Markov approximation is employed to obtain the reduced density matrix rate equation. Using quantum laser theory, we derived the Scully-Lamb laser rate equations and evaluated the single- and multi-photon excess emission rates defined as the difference between emission and absorption rates into the cavity mode without mean-field approximations. We investigated cooperative two-photon lasing, correlated emission lasing, hyperradiant lasing, non-degenerate two-mode two-photon lasing, and continuous variable entanglement in open quantum systems with single or multiple semiconductor quantum dots (two-level, three-level, and four-level) driven coherently/incoherently and coupled to single/ bimodal cavities.