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arXiv:1002.2663 · Physical Review A

Local-field excitations in two-dimensional lattices of resonant atoms

S. N. Volkov, A. E. Kaplan

Published Apr 1, 2010• 6 citations
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Abstract

We study excitations of the local field (locsitons) in nanoscale two-dimensional (2D) lattices of strongly interacting resonant atoms and various unusual effects associated with them. Locsitons in low-dimensional systems and the resulting spatial strata and more complex patterns on a scale of just a few atoms were predicted by us earlier [A. E. Kaplan and S. N. Volkov, Phys. Rev. Lett. 101, 133902 (2008)]. These effects present a radical departure from the classical Lorentz-Lorenz theory of the local field (LF), which assumes that the LF is virtually uniform on this scale. We demonstrate that the strata and patterns in the 2D lattices may be described as an interference of plane-wave locsitons, build an analytic model for such unbounded locsitons, and derive and analyze dispersion relations for the locsitons in an equilateral triangular lattice. We draw useful analogies between 1D and 2D locsitons but also show that the 2D case enables locsitons with the most diverse and unusual properties. Using the nearest-neighbor approximation, we find the locsiton frequency band for different mutual orientations of the lattice and the incident field. We demonstrate a formation of distinct vector locsiton patterns consisting of multiple vortices in the LF distribution and suggest a way to design finite 2D lattices that exhibit such patterns at certain frequencies. We illustrate the role of lattice defects in supporting localized locsitons and also demonstrate the existence of ``magic shapes,'' for which the LF suppression at the exact atomic resonance is canceled.

DOI
10.1103/physreva.81.043801

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We study excitations of the local field (locsitons) in nanoscale two-dimensional (2D) lattices of strongly interacting resonant atoms and various unusual effects associated with them. Locsitons in low-dimensional systems and the resulting spatial strata and more complex patterns on a scale of just a few atoms were predicted by us earlier [A. E. Kaplan and S. N. Volkov, Phys. Rev. Lett. 101, 133902 (2008)]. These effects present a radical departure from the classical Lorentz-Lorenz theory of the local field (LF), which assumes that the LF is virtually uniform on this scale. We demonstrate that the strata and patterns in the 2D lattices may be described as an interference of plane-wave locsitons, build an analytic model for such unbounded locsitons, and derive and analyze dispersion relations for the locsitons in an equilateral triangular lattice. We draw useful analogies between 1D and 2D locsitons but also show that the 2D case enables locsitons with the most diverse and unusual properties. Using the nearest-neighbor approximation, we find the locsiton frequency band for different mutual orientations of the lattice and the incident field. We demonstrate a formation of distinct vector locsiton patterns consisting of multiple vortices in the LF distribution and suggest a way to design finite 2D lattices that exhibit such patterns at certain frequencies. We illustrate the role of lattice defects in supporting localized locsitons and also demonstrate the existence of ``magic shapes,'' for which the LF suppression at the exact atomic resonance is canceled.
The major assumption of the Lorentz-Lorenz theory about uniformity of local fields and atomic polarization in dense material does not hold in finite groups of atoms, as we reported earlier [A. E. Kaplan and S. N. Volkov, Phys. Rev. Lett. 101, 133902 (2008)]. The uniformity is broken at subwavelength scale, where the system may exhibit strong stratification of local field and dipole polarization, with the strata period being much shorter than the incident wavelength. In this paper, we further develop and advance that theory for the most fundamental case of one-dimensional arrays, and study nanoscale excitation of so-called ``locsitons'' (local field excitations) and their standing waves (strata) that result in size-related resonances and related large field enhancement in finite arrays of atoms. The locsitons may have a whole spectrum of spatial frequencies, ranging from long waves, to an extent reminiscent of ferromagnetic domains, to supershort waves, with neighboring atoms alternating their polarizations, which are reminiscent of antiferromagnetic spin patterns. Of great interest is the different kind of ``hybrid'' mode of excitation, greatly departing from any magnetic analogies. We also study differences between Ising-type near-neighbor approximation and the case where each atom interacts with all other atoms in the array. We find an infinite number of ``exponential eigenmodes'' in the lossless system in the latter case. At certain ``magic'' numbers of atoms in the array, the system may exhibit self-induced (but linear in the field) cancellation of resonant local-field suppression. We also studied nonlinear modes of locsitons and found optical bistability and hysteresis in an infinite array for the simplest modes.
We predict nanoscale field and dipole patterns due to the broken uniformity of a laser-driven local field in 1D and 2D lattices. They may result in size-related resonances and large field enhancement, which in turn can give rise to low-intensity nonlinear optical effects, e.g., optical bistability, even in the ultimate case of a pair of coupled atoms. At certain, "magic" numbers and configurations of atoms in a lattice, the system may exhibit the self-induced cancellation of the suppression of a local field.
We study the optical response of a two-dimensional (2D) square lattice of atoms using classical electrodynamics. Because of dipole-dipole interactions, the lattice atoms polarize as if the lattice were an atom with up to three resonance frequencies, with cooperatively shifted resonances and altered transition linewidths. We show that when the distance between two 2D lattices is large enough and Bragg reflections are absent, the lattices interact among themselves as if they radiated a plane wave whose amplitude is in accordance with the radiation from a dipole moment continuously distributed in the lattice plane. We employ these results to study light propagation in stacks of 2D lattices, drawing on simple qualitative pictures of the response of a 2D lattice and light propagation in one-dimensional (1D) waveguides. We show that a stack of 2D lattices may emulate regularly spaced atoms in a lossless 1D waveguide, and argue that in a suitable geometry the resonance shifts characteristic of 1D and 2D lattice structures may completely cancel to eliminate density-dependent resonance shifts of atoms bound to a three-dimensional (3D) lattice. A generalization to the case of anisotropic polarizability, such as in the presence of a magnetic field, reveals light frequencies induced by the magnetic field for which a 2D lattice is either completely transparent or completely opaque.
We study coherent and radiative interactions induced among two or more quantum units by coupling them to two-dimensional (2D) lattices acting as structured environments. This model can be representative of atoms trapped near photonic crystal slabs, trapped ions in Coulomb crystals, or to surface acoustic waves on piezoelectric materials, cold atoms on state-dependent optical lattices, or even circuit QED architectures, to name a few. We compare coherent and radiative contributions for the isotropic and directional regimes of emission into the lattice, for infinite and finite lattices, highlighting their differences and existing pitfalls, e.g., related to long-time or large-lattice limits. We relate the phenomenon of directionality of emission with linear-shaped isofrequency manifolds in the dispersion relation, showing a simple way to disrupt it. For finite lattices, we study further details such as the scaling of resonant number of lattice modes for the isotropic and directional regimes, and relate this behavior with known van Hove singularities in the infinite lattice limit. Furthermore, we export the understanding of emission dynamics with the decay of entanglement for two quantum, atomic or bosonic, units coupled to the 2D lattice. We analyze in some detail completely subradiant configurations of more than two atoms, which can occur in the finite lattice scenario, in contrast with the infinite lattice case. Finally, we demonstrate that induced coherent interactions for dark states are zero for the finite lattice.