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arXiv:0911.4805 · Journal of Computational and Theoretical Nanoscience

Optical Cooling of Atoms in Microtraps by Time-Delayed Reflection

Péter Horák, André Xuereb, Tim Freegarde

Published Jul 21, 2010• 3 citations
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Abstract

We present a theoretical analysis of a novel scheme for optical cooling of particles that does not in principle require a closed optical transition. A tightly confined laser beam interacting with a trapped particle experiences a phase shift, which upon reflection from a mirror or resonant microstructure produces a time-delayed optical potential for the particle. This leads to a nonconservative force and friction. A quantum model of the system is presented and analyzed in the semiclassical limit.

DOI
10.1166/jctn.2010.1539

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We present a theoretical analysis of a novel scheme for optical cooling of particles that does not in principle require a closed optical transition. A tightly confined laser beam interacting with a trapped particle experiences a phase shift, which upon reflection from a mirror or resonant microstructure produces a time-delayed optical potential for the particle. This leads to a nonconservative force and friction. A quantum model of the system is presented and analyzed in the semiclassical limit.
We investigate theoretically a novel optical technique to cool atomic or molecular species without a closed transition: a particle in front of a mirror illuminated by an off-resonant light beam. The interaction between the particle, the pump and the time-delayed reflected pump results in a net loss of energy from the particle to the field and therefore cooling. Cooling rates depending on particle position and coupling parameters are obtained by an analytical perturbative approach. Finally, we present a semiclassical computational model incorporating momentum diffusion, which will eventually allow us to predict steady-state temperatures.
Cooling and trapping of atoms with light provides us with samples far colder and denser than possible by any other means and enables us to study and control these systems in exquisite detail [1]. We can not only learn about these systems, but can devise experiments of such precision that we test the underlying physics. It is unfortunate therefore that the most effective techniques, Doppler cooling and the Magneto Optical Trap, rely on a simple energy level structure found only in a handful of elements. Finally, I will present an approach in which a particle can be cooled using the dipole, rather than the scattering, force. The dipole force is conservative, but by allowing the potential to vary in time, one can change the energy of a trapped particle. Specifically, if the potential depends on the position of the particle with some time delay, we can create a friction-like force [5, 6], and we are currently building an experiment to demonstrate this effect. This technique is not restricted to atoms with a simple structure, but requires only that the particle be polarisable; in principle, therefore, it can be extended without significant change to direct optical cooling of molecules.
The dipole force, which avoids the closed cycle of pumping and spontaneous emission that renders laser cooling unsuitable for molecules, is conservative: without dissipation, particles entering a trap retain the energy to escape. Fortunately, dissipation need not involve spontaneous emission if it instead results from the decoherence or decay of the optical trapping field that is coupled to the particle. To enhance the weak attraction of an atom to its reflection, cavity-mediated cooling recycles light through multiple reflections, amplifying the force and the retardation - a process related to the mechanical amplification in a near confocal cavity [5]. Resonant cavities and structures can increase the retardation, but not the intensity, even when the atoms or particles lie outside them - e.g. when the cavity is the narrow-band coating of a single mirror. Plasmon resonances of a structured metal can enhance both the delay and the optical intensity. Such processes, possible with arrays of micromirrors, resemble speckle field cooling [6], except that spontaneous emission is again replaced by decay of the optical field, and offer a new class of cooling mechanisms in which weak cooling is extended over a broad array, rather than concentrated at the centre of a single external cavity.
We calculate the loading efficiency and cooling rates in a bichromatic optical microtrap, where the optical potentials are generated by evanescent waves of cavity fields at a dielectric-vacuum interface. The cavity modified nonconservative dynamic light forces lead to efficient loading of the atoms as well as cooling without the need for spontaneous emission. Steady-state temperatures well below the trap depth, reaching the motional quantum regime, yield very long capturing times for a neutral atom.
We propose a cooling scheme for realizing single-photon sideband cooling on particles trapped in a statedependent optical potential.We develop a master rate equation from an ab initio model and find that in experimentally feasible conditions it is possible to reduce the average occupation number of the vibrational levels in one dimension by more than 90% by applying a frequency sweep on the cooling laser that sequentially cools all the motional states.Notably, this cooling scheme works also when a particle experiences a deeper trap in its internal ground state than in its excited state, a condition for which conventional single-photon sideband cooling does not work.In our analysis, we consider two cases: a two-level particle confined in an optical tweezer, and Li atoms confined in an optical lattice, and we find conditions for efficient cooling in both cases.The results from the model are confirmed by a full quantum Monte Carlo simulation of the system Hamiltonian.Our findings provide an alternative cooling scheme that can be applied in principle to any particle, e.g., atoms, molecules, or ions, confined in a state-dependent optical potential.