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arXiv:0907.4345 · Physical Review B

Superconducting state with a finite-momentum pairing mechanism in zero external magnetic field

Florian Loder, A. P. Kampf, Thilo Kopp

Published Jan 28, 2010• 57 citations
arXivHTMLPDF

Abstract

In the BCS theory of superconductivity, one assumes that all Cooper pairs have the same center-of-mass momentum. This is indeed enforced by self-consistency if the pairing interaction is momentum independent. Here, we show that for an attractive nearest-neighbor interaction, this is different. In this case, stable solutions with pairs with momenta $\mathbf{q}$ and $\ensuremath{-}\mathbf{q}$ coexist and, for a sufficiently strong interaction, one of these states becomes the ground state of the superconductor. The possibility for a finite-momentum pairing state emerges only for nodal superconductors and is accompanied by a charge order with wave vector $2\mathbf{q}$. For a weak pairing interaction, the ground state is a $d$-wave superconductor.

DOI
10.1103/physrevb.81.020511

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In the BCS theory of superconductivity, one assumes that all Cooper pairs have the same center-of-mass momentum. This is indeed enforced by self-consistency if the pairing interaction is momentum independent. Here, we show that for an attractive nearest-neighbor interaction, this is different. In this case, stable solutions with pairs with momenta q\mathbf{q}q and \ensuremath−q\ensuremath{-}\mathbf{q}\ensuremath−q coexist and, for a sufficiently strong interaction, one of these states becomes the ground state of the superconductor. The possibility for a finite-momentum pairing state emerges only for nodal superconductors and is accompanied by a charge order with wave vector 2q2\mathbf{q}2q. For a weak pairing interaction, the ground state is a ddd-wave superconductor.
We solve the two-electron problem on a square lattice with d-wave altermagnetism, considering both on-site and nearest-neighbor attractive interactions. The altermagnetic spin-splitting in the single-particle dispersion naturally gives rise to a ground state of two-electron bound pairs with nonzero center-of-mass momentum. The emergence of finite-momentum bound states suggests that altermagnetic spin splitting may favor pairing at nonzero center-of-mass momentum, which could be relevant for proposed Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconductivity in altermagnetic systems. Additionally, when the nearest-neighbor attraction is strong, the resulting finite-momentum bound pairs exhibit a mixture of both spin-singlet and spin-triplet characteristics, suggesting the possibility of unconventional superconductors, where spin-singlet and spin-triplet pairings coexist.
Pair density waves (PDWs) are superconducting states formed by Cooper pairs of electrons containing a nonzero center-of-mass momentum. They are characterized by a spatially modulated order parameter and may occur in a variety of emerging quantum materials such as cuprates, transition-metal dichalcogenides (TMDs), and Kagome metals. Despite extensive theoretical and numerical studies seeking PDWs in a variety of lattices and interacting settings, there is currently no exact mechanism that spontaneously favors a modulated solution of the superconducting order parameter. Here, we study the problem of two electrons subject to an anisotropic attractive potential. We solve the two-body Schr\"odinger wave equation exactly to determine the pair binding energy as a function of the center-of-mass momentum. We find that a modulated (finite momentum) pair is favored over a homogeneous (zero momentum) solution above a critical, intermediate interaction strength. Hence our exact result justifies previous mean-field approximations that obtain modulated ground states at finite but large interactions. Using this insight from the exact two-body solution, we construct a variational many-body wave function and show that the conclusions of the two-body problem are robust in the many-body limit. Our results thus lay the theoretical and microscopic foundation for the existence of PDWs.
Relation between the binding energy of a pair of electrons in Cooper's configuration and the magnitude of the attractive interaction between them is investigated theoretically for a two-dimensional electron gas when the electron pair has (a) zero and (b) finite center of mass momentum (CMM) first (i) in the background of a passive Fermi sea and (ii) with inclusion of the effect of Pauli exclusion principle in the presence of an active Fermi sea, at zero temperature. In the Cooper's approach (Cooper 1956 Phys. Rev. 104 1189) two pairing electrons are considered above the Fermi sea. Due to Pauli exclusion principle, these two electrons are forbidden to go into the states whose energies are less than the Fermi energy. Consequently, the role of the electrons which form the Fermi sea is passive in formation of electron pair (Fujita and Godoy 2001 Theory of High Temperature Superconductivity (Kluwer Academic Publishers)). However, in the case of an active Fermi sea, implying possible presence of multiple pairs of electrons coming out of the Fermi sea, the two electrons will have less available region in the momentum space for pair formation due to the Pauli blocking effect. In both the situations, threshold values of attractive interaction are found to exist to bind the electrons having finite CMM even with respect to the Fermi energy while with arbitrarily small value of attractive interaction they can be bound only in the case of zero CMM and that too in the presence of a passive Fermi sea. However, the presence of an active Fermi sea strongly opposes the pair formation having lower CMM. Furthermore, raising the range of the attractive interaction below and above the Fermi surface makes the pair formation more difficult due to enhanced Pauli blocking in this case. In the case of a passive Fermi sea however, with the increase in the range of the attractive interaction it becomes easier for the electron pairs to be in both Cooper pair state (CP) and true bound state (TB). These results are totally distinct from those obtained by Randeria et al (1989 Phys. Rev. Lett. 62 981, 1990 Phys. Rev. B 41 327) that a fermionic bound state in true vacuum is a necessary and sufficient condition for the Cooper pairing instability in the presence of a passive Fermi sea, independent of attractive interaction strength implying that for a potential which is attractive everywhere in two dimension, a two-body bound state exists for an arbitrarily weak attraction. Our calculations show, in the mean field approximation, that co-existence of TB state and CP state with various CMMs can occur only beyond a critical attractive interaction strength. This could lead to the formation of incoherent pairs even under strong coupling situation, which may hint onto the pseudo gap formation leading to some of the exotic features in the anomalous normal state seen in some of the exotic superconductors.
Abstract In weakly coupled BCS superconductors, only electrons within a tiny energy window around the Fermi energy, EF, form Cooper pairs. This may not be the case in strong coupling superconductors such as cuprates, FeSe, SrTiO3 or cold atom condensates where the pairing scale, EB, becomes comparable or even larger than EF. In cuprates, for example, a plausible candidate for the pseudogap state at low doping is a fluctuating pair density wave, but no microscopic model has yet been found which supports such a state. In this work, we write an analytically solvable model to examine pairing phases in the strongly coupled regime and in the presence of anisotropic interactions. Already for moderate coupling we find an unusual finite temperature phase, below an instability temperature Ti, where local pair correlations have non-zero center-of-mass momentum but lack long-range order. At low temperature, this fluctuating pair density wave can condense either to a uniform d-wave super- conductor or the widely postulated pair-density wave phase depending on the interaction strength. Our minimal model offers a unified microscopic framework to understand the emergence of both fluctuating and long range pair density waves in realistic systems.
An indispensable ingredient for pair density wave (PDW) superconductivity is the presence of an attractive pairing interaction at finite momentum. Here, we show how this condition can be met with straightforward electron-density interactions in multiband systems. The electron-density interaction, when projected to the band basis, acquires form factors with nontrivial momentum dependence and thereby exhibits a potential tendency to a finite-momentum pairing instability. By applying a mean field analysis to two simple multiband models, the checkerboard lattice and three-band Hubbard model, we find that PDW order can indeed become the leading instability if a strong nearest-neighbor attraction is present. Moreover, the condition for the transition from a uniform superconductor to a PDW superconductor is shown via a simple quantum geometric argument.
Superconductivity beyond the Gorkov decoupling is examined with an emphasis on the thermodynamic properties. In the Gorkov decoupling, the interaction term is factorized into the pairing correlation. Therefore, in contrast to the strong pair-pair correlation in coordinate space, the correlation between the Cooper pairs in momentum space is neglected. In this paper, in addition to the conventional pairing interaction, we consider a more general type of attractive interaction that cannot be factorized into the product of the pairing correlation. Accordingly, it becomes necessary to include the neglected correlation. We assume a variational functional where the general type of interaction is taken into account, and determine the state self-consistently at finite temperature. The following results are obtained: (1) The state obtained is more stable at low temperature, compared with the BCS state with the same parameters. (2) As the temperature is increased, our state approaches the BCS state. (3) At the same temperature as in the BCS theory, our system undergoes a phase transition from the superconducting phase to the normal phase.