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arXiv:0907.2350 · Physical Review A

Casimir-Polder interaction between an atom and a dielectric slab

Ana M. Contreras-Reyes, Claudia Eberlein

Published Sep 16, 2009• 23 citations
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Abstract

We present an explicit analytic calculation of the energy-level shift of an atom in front of a nondispersive and nondissipative dielectric slab. We work with the fully quantized electromagnetic field, taking retardation into account. We give the shift as a two-dimensional integral and use asymptotic analysis to find expressions for it in various retarded and nonretarded limiting cases. The results can be used to estimate the energy shift of an atom close to layered microstructures.

DOI
10.1103/physreva.80.032901

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We present an explicit analytic calculation of the energy-level shift of an atom in front of a nondispersive and nondissipative dielectric slab. We work with the fully quantized electromagnetic field, taking retardation into account. We give the shift as a two-dimensional integral and use asymptotic analysis to find expressions for it in various retarded and nonretarded limiting cases. The results can be used to estimate the energy shift of an atom close to layered microstructures.
We determine the energy-level shift experienced by a neutral atom due the quantum electromagnetic interaction with a layered dielectric body. We use the technique of normal-mode expansion to quantize the electromagnetic field in the presence of a layered, nondispersive, and nonabsorptive dielectric. We explicitly calculate the equal-time commutation relations between the electric field and vector potential operators. We show that the commutator can be expressed in terms of a generalized transverse $\ensuremath{\delta}$ function and that this is a consequence of using the generalized Coulomb gauge to quantize the electromagnetic field. These mathematical tools turn out to be very helpful in the calculation of the energy-level shift of the atom, which can be in its ground state or excited. The results for the shift are then analyzed asymptotically in various regions of the system's parameter space, with a view to providing quick estimates of the influence of a single dielectric layer on the Casimir-Polder interaction between an atom and a dielectric half space. We also investigate the impact of resonances between the wavelength of the atomic transition and the thickness of the top layer.
The energy–level shifts and the change in the rate of spontaneous emission are calculated for an atom located at a distanceZ from a dielectric half–space. The dielectric is a non–dispersive and non–absorbing medium characterized by a constant real refractive indexn. The explicit analytic formulae derived are applicable for arbitrary values ofn. All results are analysed in the non-retarded and retarded limits, which apply to the atom being close to or far from the interface, respectively, i.e. toZ being small or large on the scale of a wavelength of a typical atomic transition. For ground-state atoms, the energy–level shift varies as 1/Z3 in the non–retarded regime and as 1/Z4 in the retarded regime, which agrees with the Casimir–Polder result for the limitn→α. For excited–state atoms, the energy–level shifts receive additional contributions that oscillate with the distanceZ from the interface.
Quantum electrodynamic theory (QED) in the vicinity of macroscopic structures has achieved new importance due to its applicability, particularly in nanotechnology. There are many powerful methods for studying QED near media with diverse properties and geometries. However, applying them to a particular problem generally necessitates extensive numerical calculations. This is not the case for simple systems of high symmetry, in which the electromagnetic field can be quantised by explicit mode expansion, allowing exact analytic calculations. In the present thesis, we calculate the energy-level shift of a ground state atom near a non-dispersive and non-dissipative dielectric slab. The shift is due to the interaction of the atom with electromagnetic field fluctuations, which in turn are affected by the presence of the slab. Thus, a quantisation of the electromagnetic field in the presence of a layered system is required. We derive the field modes, which comprise of a continuous set of travelling modes (with incident, reflected and transmitted parts) and trapped modes, subject to repeated total internal reflection and emerge as an evanescent field outside the slab, they only exist at certain discrete frequencies. The shift is obtained by means of second-order perturbation theory. It splits up naturally into two contributions, due to the different nature of the modes, and a problem arises when we have to add them all. We have come up with a convenient method of summing over all modes, and its validity has been demonstrated by proving the completeness. The calculation of the shift follows as an application of our method. The result is analysed asymptotically for various regions, reducing to simple formulas that can be utilised in recent experiments, in which the thickness of the substrate matters.
We calculate the energy-level shifts of an atom near a dielectric microsphere. With the quantum electrodynamic linear-response formalism and the exact field susceptibility satisfying the boundary conditions, the energy shifts of a ground-state atom are calculated numerically. From the numerical results, in particular, we are able to identify the short-range instantaneous van der Waals interaction energy and the long-range Casimir-Polder retarded interaction energy between two polarizable objects (atom and cavity).
We calculate the atomic energy-level shift and the modified dipolar radiation rate inside a hollow dielectric cylinder and outside a solid cylinder using a quantum-mechanical linear-response formalism in the dipole approximation. We first derive the electromagnetic fields scattered by the cylindrical surface for an oscillating dipole inside and outside the cylinder. When an atom is located on the axis of the cylindrical hollow, we obtain analytic expressions of the atomic level shifts in two limiting cases: when bbb (radius of hollow) is very small, the level shift is proportional to ${b}^{\ensuremath{-}2}$ which is associated with the kinetic-energy change of the atomic electron, whereas when bbb is very large, the shift is proportional to ${b}^{\ensuremath{-}4}$ which is identified as the retarded (Casimir-Polder) interaction energy. Moreover, we calculate the atomic potentials as a function of the position of atoms in the hollow region, which is important for the atom-guiding experiment. We also calculate the decay rates and find enhanced rates inside and outside the cylinder. In particular, we compare the radiative properties of an atom inside the hollow cylinder with those between two plates, and those near a cylinder with near a single surface.
The Casimir-Polder potential for interaction between an excited atom and a ground-state one in the retarded case is obtained with the help of perturbation technique. The potential drops as ${R}^{\ensuremath{-}2}$ with the distance between the atoms [E. A. Power and T. Thirunamachandran, Phys. Rev. A 47, 2539 (1993)]. It results in divergent integrals for interaction between an excited atom and a dilute gas medium. We investigate interaction between two atoms embedded in a dielectric medium with the help of a method that enables us to make calculations beyond the perturbation technique. We take into account absorption of photons in the medium. This approach solves the problem of divergence. We consider interaction between an excited atom and a planar dielectric gas medium of ground-state atoms. We show that the retarded interaction between an excited atom and a gas of ground-state atoms is not oscillating but follows a simple power law. We show that to obtain a conventional nonretarded expression for the van der Waals force between an excited atom and a dilute gas, the distance between the atom and the interface should be much smaller than the free mean path of a photon in the medium. Interaction between an excited atom and a hemisphere of ground-state atoms is considered.