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arXiv:0905.4649 · Physical Review Letters

Frequency Matching in Light-Storage Spectroscopy of Atomic Raman Transitions

Leon Karpa, Gor Nikoghosyan, Frank Vewinger, Michael Fleischhauer, Martin Weitz

Published Aug 28, 2009• 21 citations
arXivHTMLPDF

Abstract

We investigate the storage of light in an atomic sample with a Lambda-type coupling scheme driven by optical fields at variable two-photon detuning. In the presence of electromagnetically induced transparency (EIT), light is stored and retrieved from the sample by dynamically varying the group velocity. It is found that for any two-photon detuning of the input light pulse within the EIT transparency window, the carrier frequency of the retrieved light pulse matches the two-photon resonance frequency with the atomic ground state transition and the control field. This effect which is not based on spectral filtering is investigated both theoretically and experimentally. It can be used for high-speed precision measurements of the two-photon resonance as employed, e.g., in optical magnetometry.

DOI
10.1103/physrevlett.103.093601

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We investigate the storage of light in an atomic sample with a Lambda-type coupling scheme driven by optical fields at variable two-photon detuning. In the presence of electromagnetically induced transparency (EIT), light is stored and retrieved from the sample by dynamically varying the group velocity. It is found that for any two-photon detuning of the input light pulse within the EIT transparency window, the carrier frequency of the retrieved light pulse matches the two-photon resonance frequency with the atomic ground state transition and the control field. This effect which is not based on spectral filtering is investigated both theoretically and experimentally. It can be used for high-speed precision measurements of the two-photon resonance as employed, e.g., in optical magnetometry.
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Electromagnetically induced transparency (EIT) effect is an effective means to store light field into the atom ensemble. The extra noise introduced in the stored procedure can be suppressed greatly under the condition of large one-photon detuning and proper two-photon detuning. In this paper, we experimentally investigate the slow light and light storage in 87Rb vapor by using EIT effect, and study the effects of the two-photon detuning on light pulse delay and light memory at 650 MHz one-photon red detuning. In order to avoid some unwanted effects under the high optical depth condition, such as four-wave mixing, etc., the temperature of the atomic cell is controlled at 65 degrees Celsius. The experimental results show that the delay and the retrieval signals are significant in a two-photon detuning range from 0 to 0.5 MHz. The pulse delay decreases with the increase of two-photon detuning. The delay is 0.36 ups at two-photon resonance, and it is 0.07 ups at 1 MHz two-photon detuning. We simulate the delayed light pulse by using a three-level -type EIT model. The shapes of the measured slow light are in agreement with the theoretical results. The retrieval signals are observed at different two-photon detunings. The shapes of the retrieval pulses change with the two-photon detuning. The shape variations of the retrieval pulses cannot be explained by the three-level EIT theoretical model. By considering the atomic Zeeman sublevels interacting with the left-circular and right-circular polarized components of probe and coupling fields, multiple -type EIT systems will be formed. The interference between the retrieval signals from multiple EIT subsystems causes the shape distortions of retrieval pulses. The retrieval efficiency is measured as a function of two-photon detuning. The retrieval efficiency oscillates, and multiple peaks appear with the increase of two-photon detuning. The first peak appears at two-photon resonance, and the second peak appears at 0.48 MHz two-photon detuning. Finally, we measure the retrieval efficiency as a function of the coupling power at 0.48 MHz two-photon detuning. The optimal retrieval efficiency reaches 25% when the coupling power is 100 mW. These results provide experimental reference for the quantum memory of continuous variables in the hot atom ensemble.
The optical properties of a five-level atomic system composed of a 'Lambda'-type four-level atomic and a tripod four-level atomic systems are investigated. It is found that the behaviors of electromagnetically induced transparency (EIT) and group velocity can be controlled by choosing appropriate parameters with the interacting dark resonances. In particular, when all the fields are on resonance, the slow light at the symmetric transparency windows with a much broader EIT width is obtained by tuning the intensity of the coupling field in comparison with its sub-system, which provides potential applications in quantum storage and retrieval of light.
Abstract We report on a method for measuring ac Stark shifts observed in stored light experiments while simultaneously determining the energetic splitting between the electronic ground states involved in the two-photon transition. To this end, we make use of the frequency matching effect in light storage spectroscopy. We find a linear dependence on the intensity of the control field applied during the retrieval phase of the experiment. At the same time, we observe that the light shift is insensitive to the intensity of the signal field which is in contrast to continuously operated electromagnetically induced transparency (EIT) or coherent population trapping (CPT) experiments, where the light shifts induced by all participating optical fields have to be taken into account. Our results may be of importance for future precision measurements in addition to or in combination with current EIT and CPT-type devices which are largely compatible with our approach and could benefit from the inherent robustness regarding operational conditions, shape of the resonances or intensity fluctuations in the signal field.
The broadband parametric fluorescence pulse (probe light) with center frequency resonant on the 87Rb^{87}\mathrm{Rb}87Rb D1{D}_{1}D1​ line was injected into a cold atomic ensemble with coherent light (control light). Due to the low gain in the parametric down conversion process, the probe light was in a highly bunched photon-pair state. By switching off the control light, the probe light within the electromagnetically induced transparency window was mapped on the atoms. When the control light was switched on, the probe light was retrieved and frequency-filtered storage was confirmed from the superbunching effect and an increase of the coherence time of the retrieved light.