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arXiv:0905.3722 · Physical Review Letters

Trapping and Manipulation of Isolated Atoms Using Nanoscale Plasmonic Structures

Darrick E. Chang, Jeff D. Thompson, Hongkun Park, Vladan Vuletić, Alexander S. Zibrov, P. Zoller, Mikhail D. Lukin

Published Sep 17, 2009• 124 citations
arXivHTMLPDF

Abstract

We propose and analyze a scheme to interface individual neutral atoms with nanoscale solid-state systems. The interface is enabled by optically trapping the atom via the strong near-field generated by a sharp metallic nanotip. We show that under realistic conditions, a neutral atom can be trapped with position uncertainties of just a few nanometers, and within tens of nanometers of other surfaces. Simultaneously, the guided surface plasmon modes of the nanotip allow the atom to be optically manipulated, or for fluorescence photons to be collected, with very high efficiency. Finally, we analyze the surface forces, heating and decoherence rates acting on the trapped atom.

DOI
10.1103/physrevlett.103.123004

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We propose and analyze a scheme to interface individual neutral atoms with nanoscale solid-state systems. The interface is enabled by optically trapping the atom via the strong near-field generated by a sharp metallic nanotip. We show that under realistic conditions, a neutral atom can be trapped with position uncertainties of just a few nanometers, and within tens of nanometers of other surfaces. Simultaneously, the guided surface plasmon modes of the nanotip allow the atom to be optically manipulated, or for fluorescence photons to be collected, with very high efficiency. Finally, we analyze the surface forces, heating and decoherence rates acting on the trapped atom.
We propose a novel scheme to generate nanoscale optical trap for cold atoms near the tapered Ag nanotip, in which we take a microdisk cavity near the nanoscale trap and form a nanoscale solid-state system to realize the loading of the isolated cold atoms. We calculate the field distribution by the FDTD method near the nanotip, and discuss the intensity, the optical potential and van der Waals potential as well as the dipole force for 87Rb atoms. We find that the total potential and dipole force can form an attracting nanoscale trap for cold atoms with red-detuned field and it can realize the effective trapping and manipulation of the isolated atoms, which can enable efficient fluorescence photon collection and strong coupling in the coupled optical fiber.
We theoretically propose blue-detuned optical trapping for neutral atoms via strong near-field interfacing in a plasmonic nanohole array. The optical field at resonance forms a nanoscale-trap potential with an FWHM of 200 nm and about ∼370  nm away from the nanohole; thus, a stable 3D atom trapping independent of the surface potential is demonstrated. The effective trap depth is more than 1 mK when the optical power of trapping light is only about 0.5 mW, while the atom scattering rate is merely about 3.31  s−1, and the trap lifetime is about 800 s. This compact plasmonic structure provides high uniformity of trap depths and a two-layer array of atom nanotraps, which should have important applications in the manipulation of cold atoms and collective resonance fluorescence.
We propose a novel scheme to guide neutral cold atoms in a nanoscale region based on surface plasmons (SPs) of one pair and two pairs of tips of metallic wedges with locally enhanced light intensity and sub-optical wavelength resolution. We analyze the near-field intensity distribution of the tip of the metallic wedge by the FDTD method, and study the total intensity as well as the total potential of optical potentials and van der Waals potentials for 87Rb atoms in the light field of one pair and two pairs of tips of metallic wedges. It shows that the total potentials of one pair and two pairs of tips of metallic wedges can generate a gravito-optical trap and a dark closed trap for nanoscale guiding of neutral cold atoms. Guided atoms can be cooled with efficient intensity-gradient Sisyphus cooling by blue-detuned light field. This provides an important step towards the generation of hybrid systems consisting of isolated atoms and solid devices.
We describe and demonstrate a method to deterministically trap single atoms near nanoscale solid-state objects. The trap is formed by the interference of an optical tweezer and its reflection from the nano object, creating a one-dimensional optical lattice where the first lattice site is at z0 ∼ λ/4 from the surface. Using a tapered optical fiber as the nanoscopic object, we characterize the loading into different lattice sites by means of the AC-Stark shift induced by a guided fiber mode. We demonstrate a loading efficiency of 94(6)% into the first lattice site, and measure the cooperativity for the emission of the atom into the guided mode of the nanofiber. We show that by tailoring the dimensions of the nanofiber the distance of the trap to the surface can be adjusted. This method is applicable to a large variety of nanostructures and represents a promising starting point for interfacing single atoms with arbitrary nanoscale solid-state systems.
Ultracold atom-traps on a chip enhances the practical application of atom traps in quantum information processing, sensing, and metrology. Plasmon mediated near-field optical potentials are promising for trapping atoms. The combination of plasmonic nanostructures and ultracold atoms has the potential to create a two dimensional array of neutral atoms with lattice spacing smaller than that of lattices created from interfering light fields -- the optical lattices. We report the design, fabrication and characterization of a nano-scale array of near-field optical traps for neutral atoms using plasmonic nanostructures. The building block of the array is a metallic nano-disc fabricated on the surface of an ITO-coated glass substrate. We numerically simulate the electromagnetic field-distribution using Finite Difference Time Domain method around the nanodisc, and calculate the intensity, optical potential and the dipole force for 87^{87}87Rb atoms. The optical near-field generated from the fabricated nanostructures is experimentally characterized by using Near-field Scanning Optical Microscopy. We find that the optical potential and dipole force has all the desired characteristics to trap cold atoms when a blue-detuned light-field is used to excite the nanostructures. This trap can be used for effective trapping and manipulation of isolated atoms and also for creating a lattice of neutral atoms having sub-optical wavelength lattice spacing. Near-field measurements are affected by the influence of tip on the sub-wavelength structure. We present a deconvolution method to extract the actual near-field profile from the measured data.
We propose a new class of nanoscale electro-optical traps for neutral atoms. A prototype is the toroidal trap created by a suspended, charged carbon nanotube decorated with a silver nanosphere dimer. An illuminating laser field, blue detuned from an atomic resonance frequency, is strongly focused by plasmons induced in the dimer and generates both a repulsive potential barrier near the nanostructure surface and a large viscous damping force that facilitates trap loading. Atoms with velocities of several meters per second may be loaded directly into the trap via spontaneous emission of just two photons.