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arXiv:0902.3586

Macroscopic QED - concepts and applications

Stefan Scheel, Stefan Yoshi Buhmann

Published Feb 20, 2009• 27 citations
arXivHTMLPDF

Abstract

In this article, we review the principles of macroscopic quantum electrodynamics and discuss a variety of applications of this theory to medium-assisted atom-field coupling and dispersion forces. The theory generalises the standard mode expansion of the electromagnetic fields in free space to allow for the presence of absorbing bodies. We show that macroscopic quantum electrodynamics provides the link between isolated atomic systems and magnetoelectric bodies, and serves as an important tool for the understanding of surface-assisted atomic relaxation effects and the intimately connected position-dependent energy shifts which give rise to Casimir-Polder and van der Waals forces.

DOI
10.48550/arxiv.0902.3586

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In this article, we review the principles of macroscopic quantum electrodynamics and discuss a variety of applications of this theory to medium-assisted atom-field coupling and dispersion forces. The theory generalises the standard mode expansion of the electromagnetic fields in free space to allow for the presence of absorbing bodies. We show that macroscopic quantum electrodynamics provides the link between isolated atomic systems and magnetoelectric bodies, and serves as an important tool for the understanding of surface-assisted atomic relaxation effects and the intimately connected position-dependent energy shifts which give rise to Casimir-Polder and van der Waals forces.
Macroscopic quantum electrodynamics - Concepts and applications In this article, we review the principles of macroscopic quantum electrodynamics and discuss a variety of applications of this theory to medium-assisted atom-field coupling and dispersion forces. The theory generalises the standard mode expansion of the electromagnetic fields in free space to allow for the presence of absorbing bodies. We show that macroscopic quantum electrodynamics provides the link between isolated atomic systems and magnetoelectric bodies, and serves as an important tool for the understanding of surface-assisted atomic relaxation effects and the intimately connected position-dependent energy shifts which give rise to Casimir—Polder and van der Waals forces.
Macroscopic quantum electrodynamics (MQED) provides a unified framework for describing quantum electromagnetic fields in arbitrary macroscopic environments. Central to this theory is the field correlation, which governs both radiative (e.g., Lamb shifts and the Purcell effect) and mechanical phenomena, such as van der Waals and Casimir forces. In this tutorial, we provide an overview of MQED and its extension to active media, highlighting fluctuation-induced forces as manifestations of gain-modified field correlations.
Within the frame of macroscopic quantum electrodynamics in causal media, a rigorous derivation of the van der Waals energy of an atomic system in the presence of an arbitrary arrangement of dispersing and absorbing dielectric bodies is given. As an application, the van der Waals potential of an atom in the presence of a dispersing and absorbing sphere is derived. Closed expressions for the long-distance (retardation) and short-distance (non-retardation) limits are given, and the effect of material absorption is discussed.
The Casimir-Polder force on a single atom in the presence of microscopic magneto-electric bodies is studied within the framework of macroscopic quantum electrodynamics. In the first part, time-independent perturbation theory is used show that the static Casimir-Polder force on a ground-state atom in the presence of an arbitrary arrangement of bodies can be expressed in terms of the atom's polarisability and the scattering part of the Green tensor characterising the bodies. This result is used to verify the origin of the force and to study various bodies of simple shapes. In the second part, a genuinely dynamical approach is developed by starting from the operator Lorentz force. It is found that the dynamics of the force on initially excited atoms is governed by irreversible spontaneous decay in the case of weak atom-field coupling, while Rabi oscillations may arise for strong atom-field coupling.
After giving an outline of the quantization scheme based on the microscopic Hopfield model of a dielectric bulk material, we show how the classical phenomenological Maxwell equations of the electromagnetic field in the presence of dielectric matter of given space- and frequency-dependent complex permittivity can be transferred to quantum theory. Including in the theory the interaction of the medium-assisted field with atomic systems, we present both the minimal-coupling Hamiltonian and the multipolar-coupling Hamiltonian in the Coulomb gauge. To illustrate the concept, we discuss the input--output relations of radiation and the transformation of radiation-field quantum states at absorbing four-port devices, and the spontaneous decay of an excited atom near the surface of an absorbing body and in a spherical micro-cavity with intrinsic material losses. Finally, we give an extension of the quantization scheme to other media such as amplifying media, magnetic media, and nonlinear media.
Within the frame of macroscopic QED in linear, causal media, we study the radiation force of Casimir-Polder type acting on an atom which is positioned near dispersing and absorbing magnetodielectric bodies and initially prepared in an arbitrary electronic state. It is shown that minimal and multipolar coupling lead to essentially the same lowest-order perturbative result for the force acting on an atom in an energy eigenstate. To go beyond perturbation theory, the calculations are based on the exact center-of-mass equation of motion. For a nondriven atom in the weak-coupling regime, the force as a function of time is a superposition of force components that are related to the electronic density matrix elements at a chosen time. Even the force component associated with the ground state is not derivable from a potential in the ususal way, because of the position dependence of the atomic polarizability. Further, when the atom is initially prepared in a coherent superposition of energy eigenstates, then temporally oscillating force components are observed, which are due to the interaction of the atom with both electric and magnetic fields.