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arXiv:0811.1884 · Physical Review E

Semiclassical theory for decay and fragmentation processes in chaotic quantum systems

Martha Gutiérrez, Daniel Waltner, Jack Kuipers, Klaus Richter

Published Apr 9, 2009• 18 citations
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Abstract

We consider quantum decay and photofragmentation processes in open chaotic systems in the semiclassical limit. We devise a semiclassical approach which allows us to consistently calculate quantum corrections to the classical decay to high order in an expansion in the inverse Heisenberg time. We present results for systems with and without time-reversal symmetry, as well as for the symplectic case, and extend recent results to nonlocalized initial states. We further analyze related photodissociation and photoionization phenomena and semiclassically compute cross-section correlations, including their Ehrenfest-time dependence.

DOI
10.1103/physreve.79.046212

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We consider quantum decay and photofragmentation processes in open chaotic systems in the semiclassical limit. We devise a semiclassical approach which allows us to consistently calculate quantum corrections to the classical decay to high order in an expansion in the inverse Heisenberg time. We present results for systems with and without time-reversal symmetry, as well as for the symplectic case, and extend recent results to nonlocalized initial states. We further analyze related photodissociation and photoionization phenomena and semiclassically compute cross-section correlations, including their Ehrenfest-time dependence.
We address the decay in open chaotic quantum systems and calculate semiclassical corrections to the classical exponential decay. We confirm random matrix predictions and, going beyond, calculate Ehrenfest time effects. To support our results we perform extensive numerical simulations. Within our approach we show that certain (previously unnoticed) pairs of interfering, correlated classical trajectories are of vital importance. They also provide the dynamical mechanism for related phenomena such as photoionization and photodissociation, for which we compute cross-section correlations. Moreover, these orbits allow us to establish a semiclassical version of the continuity equation.
We study the quantum probability to survive in an open chaotic system in the framework of the van Vleck-Gutzwiller propagator and present the first such calculation that accounts for quantum interference effects. Specifically we calculate quantum deviations from the classical decay after the break time for both broken and preserved time-reversal symmetry. The source of these corrections is identified in interfering pairs of correlated classical trajectories. In our approach the quantized chaotic system is modelled by a quatum graph.
States supported by chaotic open quantum systems fall into two categories: a majority showing instantaneous ballistic decay, and a set of quantum resonances of classically vanishing support in phase space. We present a theory describing these structures within a unified semiclassical framework. Emphasis is put on the quantum diffraction mechanism which introduces an element of probability and is crucial for the formation of resonances. Our main result is boundary conditions on the semiclassical propagation along system trajectories. Depending on whether the trajectory propagation time is shorter or longer than the Ehrenfest time, these conditions describe deterministic escape, or probabilistic quantum decay.
Using the supersymmetry technique, we analytically derive the recent result of Casati, Maspero, and Shepelyansky [Phys. Rev. E 56, R6233 (1997)] according to which the quantum dynamics of open chaotic systems follows the classical decay up to a new quantum relaxation time scale ${t}_{q}\ensuremath{\sim}\sqrt{{t}_{c}{t}_{H}}.$ This scale is larger than the classical escape time tc{t}_{c}tc​ but still much smaller than the Heisenberg time tH.{t}_{H}.tH​. For systems with orthogonal or unitary symmetry the quantum decay is slower than the classical one while for the symplectic case there is an intermediate regime in which the quantum decay is slightly faster.
We show that the mechanism of quantum freeze of fidelity decay for perturbations with a zero time average, recently discovered for a specific case of integrable dynamics [New J. Phys. 5, 109 (2003)], can be generalized to arbitrary quantum dynamics. We work out explicitly the case of a chaotic classical counterpart, for which we find semiclassical expressions for the value and the range of the plateau of fidelity. After the plateau ends, we find explicit expressions for the asymptotic decay, which can be exponential or Gaussian depending on the ratio of the Heisenberg time to the decay time. Arbitrary initial states can be considered; e.g., we discuss coherent states and random states.
We consider the continuity equation for open chaotic quantum systems in the semiclassical limit. First we explicitly calculate a semiclassical expansion for the probability current density using an expression based on classical trajectories. The current density is related to the survival probability via the continuity equation, and we show that this relation is satisfied within the semiclassical approximation to all orders. For this we develop recursion relation arguments which connect the trajectory structures involved for the survival probability, which travel from one point in the bulk to another, to those structures involved for the current density, which travel from the bulk to the lead. The current density can also be linked, via another continuity equation, to a correlation function of the scattering matrix whose semiclassical approximation is expressed in terms of trajectories that start and end in the lead. We also show that this continuity equation holds to all orders.