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arXiv:0805.3585 · Physical Review Letters

Semiclassical Mechanism for the Quantum Decay in Open Chaotic Systems

Daniel Waltner, Martha Gutiérrez, Arseni Goussev, Klaus Richter

Published Oct 23, 2008• 23 citations
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Abstract

We address the decay in open chaotic quantum systems and calculate semiclassical corrections to the classical exponential decay. We confirm random matrix predictions and, going beyond, calculate Ehrenfest time effects. To support our results we perform extensive numerical simulations. Within our approach we show that certain (previously unnoticed) pairs of interfering, correlated classical trajectories are of vital importance. They also provide the dynamical mechanism for related phenomena such as photoionization and photodissociation, for which we compute cross-section correlations. Moreover, these orbits allow us to establish a semiclassical version of the continuity equation.

DOI
10.1103/physrevlett.101.174101

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We address the decay in open chaotic quantum systems and calculate semiclassical corrections to the classical exponential decay. We confirm random matrix predictions and, going beyond, calculate Ehrenfest time effects. To support our results we perform extensive numerical simulations. Within our approach we show that certain (previously unnoticed) pairs of interfering, correlated classical trajectories are of vital importance. They also provide the dynamical mechanism for related phenomena such as photoionization and photodissociation, for which we compute cross-section correlations. Moreover, these orbits allow us to establish a semiclassical version of the continuity equation.
We consider quantum decay and photofragmentation processes in open chaotic systems in the semiclassical limit. We devise a semiclassical approach which allows us to consistently calculate quantum corrections to the classical decay to high order in an expansion in the inverse Heisenberg time. We present results for systems with and without time-reversal symmetry, as well as for the symplectic case, and extend recent results to nonlocalized initial states. We further analyze related photodissociation and photoionization phenomena and semiclassically compute cross-section correlations, including their Ehrenfest-time dependence.
We study the quantum probability to survive in an open chaotic system in the framework of the van Vleck-Gutzwiller propagator and present the first such calculation that accounts for quantum interference effects. Specifically we calculate quantum deviations from the classical decay after the break time for both broken and preserved time-reversal symmetry. The source of these corrections is identified in interfering pairs of correlated classical trajectories. In our approach the quantized chaotic system is modelled by a quatum graph.
States supported by chaotic open quantum systems fall into two categories: a majority showing instantaneous ballistic decay, and a set of quantum resonances of classically vanishing support in phase space. We present a theory describing these structures within a unified semiclassical framework. Emphasis is put on the quantum diffraction mechanism which introduces an element of probability and is crucial for the formation of resonances. Our main result is boundary conditions on the semiclassical propagation along system trajectories. Depending on whether the trajectory propagation time is shorter or longer than the Ehrenfest time, these conditions describe deterministic escape, or probabilistic quantum decay.
We consider the continuity equation for open chaotic quantum systems in the semiclassical limit. First we explicitly calculate a semiclassical expansion for the probability current density using an expression based on classical trajectories. The current density is related to the survival probability via the continuity equation, and we show that this relation is satisfied within the semiclassical approximation to all orders. For this we develop recursion relation arguments which connect the trajectory structures involved for the survival probability, which travel from one point in the bulk to another, to those structures involved for the current density, which travel from the bulk to the lead. The current density can also be linked, via another continuity equation, to a correlation function of the scattering matrix whose semiclassical approximation is expressed in terms of trajectories that start and end in the lead. We also show that this continuity equation holds to all orders.
We consider the continuity equation for open chaotic quantum systems in the semiclassical limit. First we explicitly calculate a semiclassical expansion for the probability current density using an expression based on classical trajectories. The current density is related to the survival probability via the continuity equation, and we show that this relation is satisfied within the semiclassical approximation to all orders. For this we develop recursion relation arguments which connect the trajectory structures involved for the survival probability, which travel from one point in the bulk to another, to those structures involved for the current density, which travel from the bulk to the lead. The current density can also be linked, via another continuity equation, to a correlation function of the scattering matrix whose semiclassical approximation is expressed in terms of trajectories that start and end in the lead. We also show that this continuity equation holds to all orders.
We study two classes of quantum phenomena associated with classical chaos in a variety of quantum models: (i) dynamical localization and its extension and generalization to interacting few- and many-body systems and (ii) quantum exponential divergences in high-order correlators and other diagnostics of quantum chaos. Dynamical localization (DL) is a subtle phenomenon related to Anderson localization. It hinges on quantum interference and is typically destroyed in presence of interactions. DL often manifests as a failure of a driven system to heat up, violating the foundations of statistical physics. Kicked rotor (KR) is a prototypical chaotic classical model that exhibits linear energy growth with time. The quantum kicked rotor (QKR) features DL instead: its energy saturates. Multiple attempts of many-body generalizations faced difficulties in preserving DL. Recently, DL was shown in a special integrable many-body model. We study non-integrable models of few- and many-body QKR-like systems and provide direct evidence that DL can persist there. In addition, we show how a novel related concept of localization landscape can be applied to study transport in rippled channels. Out-of-time-ordered correlator (OTOC) was proposed as an indicator of quantum chaos, since in the semiclassical limit, this correlator's possible exponential growth rate (CGR) resembles the classical Lyapunov exponent (LE). We show that the CGR in QKR is related, but distinct from the LE in KR. We also show a singularity in the OTOC at the Ehrenfest time tᴱ due to a delay in the onset of quantum interference. Next, we study scaling of OTOC beyond tᴱ. We then explore how the OTOC-based approach to quantum chaos relates to the random-matrix-theoretical description by introducing an operator we dub the Lyapunovian. Its level statistics is calculated for quantum stadium billiard, a seminal model of quantum chaos, and aligns perfectly with the Wigner-Dyson surmise. In the semiclassical limit, the Lyapunovian reduces to the matrix of uncorrelated finite-time Lyapunov exponents, connecting the CGR at early times, when the quantum effects are weak, to universal level repulsion that hinges on strong quantum interference. Finally, we consider quantum polygonal billiards: their classical counterparts are non-chaotic. We show exponential growth of the OTOCs in these systems, sharply contrasted with the classical behavior even before quantum interference develops.