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arXiv:0807.1691 · Physical Review A

Role of particle interactions in a many-body model of Feshbach-molecule formation in bosonic systems

Jing Li, Difa Ye, Chao Ma, Libin Fu, Jie Liu

Published Feb 24, 2009• 27 citations
arXivHTMLPDF

Abstract

We investigate a generalized many-body model of Feshbach molecule formation that includes the atom-atom, atom-molecule, and molecule-molecule interactions. We show that the picture of two-body molecule production depicted by the Landau-Zener model is significantly altered by the particle interactions. In the adiabatic limit, we work out a formula for the ceiling of conversion efficiency when the interaction strength is larger than a critical value. In the sudden limit, we derive a closed equation for the conversion efficiency using stationary phase approximation. Our theory predicts a significant role of the particle interactions in atom-molecule conversion when the atom density is high and the Feshbach resonance width is narrow.

DOI
10.1103/physreva.79.025602

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We investigate a generalized many-body model of Feshbach molecule formation that includes the atom-atom, atom-molecule, and molecule-molecule interactions. We show that the picture of two-body molecule production depicted by the Landau-Zener model is significantly altered by the particle interactions. In the adiabatic limit, we work out a formula for the ceiling of conversion efficiency when the interaction strength is larger than a critical value. In the sudden limit, we derive a closed equation for the conversion efficiency using stationary phase approximation. Our theory predicts a significant role of the particle interactions in atom-molecule conversion when the atom density is high and the Feshbach resonance width is narrow.
We investigate the Feshbach conversion of fermionic atom pairs to condensed bosonic molecules with a microscopic model that accounts for the repulsive interactions among all the particles involved. We find that the conversion efficiency is enhanced by the interaction between bosonic molecules, while it is suppressed by the interactions between fermionic atoms and between atoms and molecules. In the adiabatic limit, the combined effect of these interactions can lead to a ceiling of less than 100% on the conversion efficiency for a narrow Feshbach resonance. Our theory agrees with the recent Rice experiment on 6 Li.
We investigate the dynamics of converting cold bosonic atoms to molecules when an external magnetic field is swept across a Feshbach resonance. Our analysis relies on a quantum microscopic model that accounts for many-body effects in the association process. We show that the picture of two-body molecular production depicted by the Landau-Zener model is significantly altered due to many-body effects. In the nonadiabatic regime, we derive an analytic expression for molecular conversion efficiency that explains the discrepancy between the prediction of the Landau-Zener formula and the experimental data [E. Hodby et al., Phys. Rev. Lett. 94, 120402 (2005)]. Our theory is further extended to the formation of heteronuclear diatomic molecules and gives some interesting predictions.
We investigate the production efficiency of ultracold molecules in bosonic 85 Rb and fermionic 40 K when the magnetic field is swept across a Feshbach resonance.For adiabatic sweeps of the magnetic field, the conversion efficiency of each species is solely determined by the phase space density of the atomic cloud, in contrast to a number of theoretical predictions.Our novel model for the adiabatic pairing process, developed from general physical principles, accurately predicts the conversion efficiency for both ultracold gases of bosons and of fermions.In the non-adiabatic regime our measurements of the 85 Rb molecule conversion efficiency follow a Landau Zener model, with a conversion efficiency that is characterized by the density divided by the time derivative of the magnetic field.
We consider in detail the situation of applying a time-dependent external magnetic field to a 87 Rb atomic Bose–Einstein condensate held in a harmonic trap, in order to adiabatically sweep the interatomic interactions across a Feshbach resonance to produce diatomic molecules. To this end, we introduce a minimal two-body Hamiltonian depending on just five measurable parameters of a Feshbach resonance, which accurately determines all low-energy binary scattering observables, in particular, the molecular conversion efficiency of just two atoms. Based on this description of the microscopic collision phenomena, we use the many-body theory of Köhler and Burnett (2002 Phys. Rev. A 65 033601) to study the efficiency of the association of molecules in a 87 Rb Bose–Einstein condensate during a linear passage of the magnetic-field strength across the 100 mT Feshbach resonance. We explore different, experimentally accessible, parameter regimes, and compare the predictions of Landau–Zener, configuration interaction, and two-level mean-field calculations with those of the microscopic many-body approach. Our comparative studies reveal a remarkable insensitivity of the molecular conversion efficiency with respect to both the details of the microscopic binary collision physics and the coherent nature of the Bose–Einstein condensed gas, provided that the magnetic-field strength is varied linearly. We provide the reasons for this universality of the molecular production achieved by linear ramps of the magnetic-field strength, and identify the Landau–Zener coefficient determined by Mies et al (2000 Phys. Rev. A 61 022721) as the main parameter that controls the efficiency.
We investigate the production efficiency of ultracold molecules in bosonic 85Rb and fermionic 40K when the magnetic field is swept across a Feshbach resonance. For adiabatic sweeps of the magnetic field, our novel model shows that the conversion efficiency of both species is solely determined by the phase space density of the atomic cloud, in contrast with a number of theoretical predictions. In the nonadiabatic regime our measurements of the 85Rb molecule conversion efficiency follow a Landau-Zener model.
We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of 40{}^{40}40K and 87{}^{87}87Rb atoms, where we can create 40{}^{40}40K87{}^{87}87Rb molecules with a conversion efficiency as high as 45%. In the limit of fast magnetic sweeps and small molecule fraction, we find that the time scale of molecule production is accurately predicted by a parameter-free model that uses only the atomic densities, masses, and the known Feshbach resonance parameters. We find that molecule production efficiency saturates for slower magnetic sweeps, at which point the maximum number of Feshbach molecules depends primarily on the atoms' phase-space density. At higher temperatures, our measurements agree with a phenomenological model that successfully describes the formation of bosonic molecules from either Bose or Fermi gases. However, for quantum degenerate atom gas mixtures, we measure significantly fewer molecules than this model predicts.