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arXiv:0804.4416 · Physical Review A

Jahn-Teller systems from a cavity QED perspective

Jonas Larson

Published Sep 22, 2008• 51 citations
arXivHTMLPDF

Abstract

Jahn-Teller systems and the Jahn-Teller effect are discussed in terms of cavity QED models. By expressing the field modes in a quadrature representation, it is shown that certain setups of a two-level system interacting with a bimodal cavity are described by the Jahn-Teller $E\ifmmode\times\else\texttimes\fi{}\ensuremath{\epsilon}$ Hamiltonian. We identify the corresponding adiabatic potential surfaces and the conical intersection. The effects of a nonzero geometrical Berry phase, governed by encircling the conical intersection, are studied in detail both theoretically and numerically. The numerical analysis is carried out by applying a wave packet propagation method, more commonly used in molecular or chemical physics, and analytic expressions for the characteristic time scales are presented. It is found that the collapse-revival structure is greatly influenced by the geometrical phase and as a consequence, the field intensities contain direct information about this phase. We also mention the link between the Jahn-Teller effect and the Dicke phase transition in cavity QED.

DOI
10.1103/physreva.78.033833

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Jahn-Teller systems and the Jahn-Teller effect are discussed in terms of cavity QED models. By expressing the field modes in a quadrature representation, it is shown that certain setups of a two-level system interacting with a bimodal cavity are described by the Jahn-Teller E\ifmmode×\else\texttimes\fi\ensuremathϵE\ifmmode\times\else\texttimes\fi{}\ensuremath{\epsilon}E\ifmmode×\else\texttimes\fi\ensuremathϵ Hamiltonian. We identify the corresponding adiabatic potential surfaces and the conical intersection. The effects of a nonzero geometrical Berry phase, governed by encircling the conical intersection, are studied in detail both theoretically and numerically. The numerical analysis is carried out by applying a wave packet propagation method, more commonly used in molecular or chemical physics, and analytic expressions for the characteristic time scales are presented. It is found that the collapse-revival structure is greatly influenced by the geometrical phase and as a consequence, the field intensities contain direct information about this phase. We also mention the link between the Jahn-Teller effect and the Dicke phase transition in cavity QED.
We demonstrate that Berry phases may greatly affect the dynamics of spin-orbit-coupled Bose-Einstein condensates. The effective model Hamiltonian under consideration is shown to be equivalent to the $E\ifmmode\times\else\texttimes\fi{}\ensuremath{\epsilon}$ Jahn-Teller model first introduced in molecular physics. The corresponding conical intersection is identified and the Berry phase acquired for a wave packet encircling the intersection is studied. It is found that this phase manifests itself in the density profile of the condensate, making it a directly measurable quantity via time-of-flight detection. Moreover, the non-Abelian gauge structure of the system is addressed and we verify how it affects the dynamics.
In 1937 the Jahn-Teller (JT) effect addressed the instability (potential or actual) of non-linear symmetric molecules with degenerate orbital electronic states. In view of the large variety of JT activity that has taken place since then, we might broaden our perspective to look at works whose subjects fall under the more general heading of "Strong interactions between two dissimilar systems" (where one system is usually bosonic and the other fermionic). In these intervening years we find several highly important works in Physics and Chemistry that come under this heading and were either connected with, or arose from, JT systems, problems and approaches. Apart from high temperature superconductors, we mention Yang-Mills gauge-forces, symmetry breaking (in elementary particles), conical intersections in molecular potential surfaces, surface crossings between them in chemical reactions, entanglements in the quantum theory of measurements and Berry phases. We elaborate on the last two topics. We show first that the slow evolution of a Txe coupling from the weak to strong regime can model the quantum mechanical three-state measurement situation, when the positions of the nuclei acts as the measuring device. We then employ recently derived integral relations between component moduli and phases in a time dependent wave-function to demonstrate the equivalence between the state-reduction and the phase decoherence interpretations of the measurement process.
Recent theoretical schemes for utilizing cavity QED models as quantum simulators are reviewed. By considering a quadrature representation for the fields, it is shown how Jahn-Teller models, effective Abelian or non-Abelian gauge potentials, transverse Hall currents, and relativistic effects naturally arise in these systems. Some of the analytical predictions are verified numerically using realistic experimental parameters taking into account for system losses. Thereby demonstrating their feasibility with current experimental setups.
We revisit earlier studies on Berry phases suggested to appear in certain cavity QED settings. It has been especially argued that a nontrivial geometric phase is achievable even in the situation of no cavity photons. We, however, show that such results hinge on imposing the rotating wave approximation (RWA), while without the RWA no Berry phases occur in these schemes. A geometrical interpretation of our results is obtained by introducing semiclassical energy surfaces which in a simple way brings out the phase-space dynamics. With the RWA, a conical intersection between the surfaces emerges and encircling it gives rise to the Berry phase. Without the RWA, the conical intersection is absent and therefore the Berry phase vanishes. It is believed that this is a first example showing how the application of the RWA in the Jaynes-Cummings model may lead to false conclusions, regardless of the mutual strengths between the system parameters.
This paper deals with the concept of adiabaticity for fully quantum mechanical cavity QED models. The physically interesting cases of Gaussian and standing wave shapes of the cavity mode are considered. An analytical approximate measure for adiabaticity is given and compared with numerical wave packet simulations. Good agreement is obtained where the approximations are expected to be valid. Usually for cavity QED systems, the large atom-field detuning case is considered as the adiabatic limit. We, however, show that adiabaticity is also valid, for the Gaussian mode shape, in the opposite limit. Effective semiclassical time-dependent models, which do not take into account the shape of the wave packet, are derived. Corrections to such an effective theory, which are purely quantum mechanical, are discussed. It is shown that many of the results presented can be applied to time-dependent two-level systems.
The Jaynes-Cummings model, with and without the rotating wave approximation, is expressed in the conjugate variable representation and solved numerically by wave packet propagation. Both cases are then cast into systems of two coupled harmonic oscillators, reminiscent of coupled bound electronic potential curves of diatomic molecules. Using the knowledge of such models, this approach of the problem gives new insight of the dynamics. The effect of the rotating wave approximation is discussed. The collapse-revival phenomenon is especially analyzed in a non-standard manner. Extensions of the method is briefly mentioned in terms of a three-level atom and the Dicke model.