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arXiv:0712.1773 · Physical Review E

Collective atomic recoil laser as a synchronization transition

J. Javaloyes, M. Perrin, Antonio Politi

Published Jul 8, 2008• 75 citations
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Abstract

We consider here a model previously introduced to describe the collective behavior of an ensemble of cold atoms interacting with a coherent electromagnetic field. The atomic motion along the self-generated spatially periodic force field can be interpreted as the rotation of a phase oscillator. This suggests a relationship with synchronization transitions occurring in globally coupled rotators. In fact, we show that whenever the field dynamics can be adiabatically eliminated, the model reduces to a self-consistent equation for the probability distribution of the atomic "phases." In this limit, there exists a formal equivalence with the Kuramoto model, though with important differences in the self-consistency conditions. Depending on the field-cavity detuning, we show that the onset of synchronized behavior may occur through either a first- or second-order phase transition. Furthermore, we find a secondary threshold, above which a periodic self-pulsing regime sets in, that is immediately followed by the unlocking of the forward-field frequency. At yet higher, but still experimentally meaningful, input intensities, irregular, chaotic oscillations may eventually appear. Finally, we derive a simpler model, involving only five scalar variables, which is able to reproduce the entire phenomenology exhibited by the original model.

DOI
10.1103/physreve.78.011108

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We consider here a model previously introduced to describe the collective behavior of an ensemble of cold atoms interacting with a coherent electromagnetic field. The atomic motion along the self-generated spatially periodic force field can be interpreted as the rotation of a phase oscillator. This suggests a relationship with synchronization transitions occurring in globally coupled rotators. In fact, we show that whenever the field dynamics can be adiabatically eliminated, the model reduces to a self-consistent equation for the probability distribution of the atomic "phases." In this limit, there exists a formal equivalence with the Kuramoto model, though with important differences in the self-consistency conditions. Depending on the field-cavity detuning, we show that the onset of synchronized behavior may occur through either a first- or second-order phase transition. Furthermore, we find a secondary threshold, above which a periodic self-pulsing regime sets in, that is immediately followed by the unlocking of the forward-field frequency. At yet higher, but still experimentally meaningful, input intensities, irregular, chaotic oscillations may eventually appear. Finally, we derive a simpler model, involving only five scalar variables, which is able to reproduce the entire phenomenology exhibited by the original model.
Networks of globally coupled oscillators exhibit phase transitions from incoherent to coherent states. Atoms interacting with the counterpropagating modes of a unidirectionally pumped high-finesse ring cavity form such a globally coupled network. The coupling mechanism is provided by collective atomic recoil lasing, i.e., cooperative Bragg scattering of laser light at an atomic density grating, which is self-induced by the laser light. Under the rule of an additional friction force, the atomic ensemble is expected to undergo a phase transition to a state of synchronized atomic motion. We present the experimental investigation of this phase transition by studying the threshold behavior of this lasing process.
We show that a model for the collective atomic recoil laser, previously introduced to include collisions with an external buffer gas, can be reduced to a single dynamical equation for the probe amplitude. This is the result of a clever adiabatic elimination of the atomic variables and of the assumption of a negligible effect of the probe field onto the atomic motion. This reduced model provides a fairly accurate description of the phase diagram of the original set of equations and allows for the investigation of more realistic regimes, where the direct simulation of the full model would be otherwise unfeasible. As a result, we find that the onset of a coherent field can be either described by a second- or first-order transition, the former scenario being observable only below a given temperature. Moreover, the first-order transition is accompanied by an intrinsic optical bistability region.
The standard model introduced to describe the collective atomic recoil of an ensemble of atoms interacting with a strong electromagnetic field has been here extended by the inclusion of collisions with a buffer gas. As a result, we find that in the thermodynamic limit the coherent emission of radiation exhibits a continuous phase transition upon increasing the pump intensity. The output laser field is strictly larger than 0 only above a critical value. We find that the transition is not associated with the onset of spatial ordering but rather with the onset of a synchronization between the polarization phase and spatial position. A coherence parameter is introduced to characterize the phase transition.
An ensemble of periodically ordered atoms coherently scatters the light of an incident laser beam. The scattered and the incident light may interfere and give rise to a light intensity modulation and thus to optical dipole forces which, in turn, emphasize the atomic ordering. This positive feedback is at the origin of the collective atomic recoil laser (CARL). We demonstrate this dynamics using ultracold atoms confined by dipole forces in a unidirectionally pumped far red‐detuned high‐finesse optical ring cavity. Under the influence of an additional dissipative force exerted by an optical molasses the atoms, starting from an unordered distribution, spontaneously form a density grating moving at constant velocity. Additionally, steady state lasing is observed in the reverse direction if the pump laser power exceeds a certain threshold. We compare the dynamics of the atomic trajectories to the behavior of globally coupled oscillators, which exhibit phase transitions from incoherent to coherent states if the coupling strength exceeds a critical value.
A cloud of ultra-cold atoms is loaded into the attractive potential of a light wave that is generated by two counter-propagating modes of a high-finesse ring resonator. The two modes are coupled by the atoms due to coherent Rayleigh scattering and generate a potential which acts back on the motion of the atoms. This feedback leads to a new frequency component and can be described in terms of the long time proposed collective atomic recoil laser (CARL). This model is investigated experimentally and extended by introducing an optical friction force acting on the atoms. This allows for steady state operation of the CARL. Furthermore, it leads to a threshold behaviour of the CARL that translates into a novel type of phase transition: while passing the threshold the initially homogeneous atomic distribution is bunched in space and velocity. With this behaviour the system turns out to acquire some of the main features of the so-called Kuramoto model which provides a very general description of a network of limit cycle oscillators.
Pattern formation of atoms in high-finesse optical resonators results from the mechanical forces of light associated with superradiant scattering into the cavity mode. It occurs when the laser intensity exceeds a threshold value such that the pumping processes counteract the losses. We consider atoms driven by a laser and coupling with a mode of a standing-wave cavity and describe their dynamics with a Fokker-Planck equation, in which the atomic motion is semiclassical but the cavity field is a full quantum variable. The asymptotic state of the atoms is a thermal state, whose temperature is solely controlled by the detuning between the laser and the cavity frequency and by the cavity loss rate. From this result we derive the free energy and show that in the thermodynamic limit self-organization is a second-order phase transition. The order parameter is the field inside the resonator to which one can associate a magnetization in analogy to ferromagnetism, the control field is the laser intensity, but the steady state is intrinsically out of equilibrium. In the symmetry-broken phase, quantum noise induces jumps of the spatial density between two ordered patterns: We characterize the statistical properties of this temporal behavior at steady state and show that the thermodynamic properties of the system can be extracted by detecting the light at the cavity output. The results of our analysis are in full agreement with previous studies; we extend them by deriving a self-consistent theory which is valid also when the cavity field is in the shot-noise limit and elucidate the nature of the self-organization transition.