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arXiv:0709.4644 · Physical Review A

Conditional preparation of states containing a definite number of photons

Malcolm N. O’Sullivan, Kam Wai Clifford Chan, Vasudevan Lakshminarayanan, Robert W. Boyd

Published Feb 5, 2008• 20 citations
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Abstract

A technique for conditionally creating single-mode or multimode photon-number states is analyzed using Bayesian theory. We consider the heralded $N$-photon states created from the photons produced by an unseeded optical parametric amplifier when the heralding detector is the time-multiplexed photon-number-resolving detector recently demonstrated by Fitch et al. [Phys. Rev. A 68, 043814 (2003)] and simultaneously by Achilles et al. [Opt. Lett. 28, 2387 (2003)]. We find that even with significant loss in the heralding detector, fields with sub-Poissonian photon-number distributions can be created. We also show that heralded multimode fields created using this technique are more robust against detector loss than are single-mode fields.

DOI
10.1103/physreva.77.023804

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We present an experimental method for creating and verifying photon-number states created by non-degenerate, third-order nonlinear-optical photon-pair sources. By using spatially multiplexed, thresholding single-photon detectors and inverting a conditional probability matrix, we determine the photon-number probabilities created through heralded spontaneous four-wave-mixing. The deleterious effects of noise photons on reliable heralding are investigated and shown to degrade the conditional preparation of two-photon number states more than they degrade conditional single-photon states. We derive the equivalence between the presence of unwanted noise in the herald channel and loss in the signal channel of heralded experiments. A procedure for characterizing the noise-photon contributions, and a means of estimating the herald noise-free photon-number distribution is demonstrated.
Conditional preparation is a well-established technique for quantum state engineering of light. A general trend is to increase the number of heralding detection events in such a realization to reach larger photon-number states or their arbitrary superpositions. In contrast to pulsed implementations, where detections only occur within the pulse window, for continuous-wave light the temporal separation of the conditioning detections is an additional degree of freedom and a critical parameter. Based on a theoretical study by Nielsen and M\o{}lmer [A. E. B. Nielsen and K. M\o{}lmer, Phys. Rev. A 75, 043801 (2007)] and on a continuous-wave two-mode squeezed vacuum from a nondegenerate optical parametric oscillator, we experimentally investigate the generation of two-photon state with tunable delay between the heralding events. The present work illustrates the temporal multimode features in play for conditional state generation based on continuous-wave light sources and quantifies the compromise between preparation rate and fidelity in this scenario.
Generation of highly non-classical quantum states of light is essential for optical quantum information processing and quantum metrology. Given the lack of sufficiently strong nonlinear interactions between optical fields, the commonly employed optical quantum-state preparation schemes are conditional, based on nonlinearity induced by heralding photon number measurement on a part of a multimode squeezed Gaussian state. Development and optimization of such probabilistic quantum-state engineering schemes represents one of the central challenges in current quantum optics. As technology advances and experiments progress to detection of higher numbers of photons, the maximization of the heralding probability becomes essential to ensure sufficiently high state-preparation rates. Here, we show that for the conditional quantum state preparation schemes based on Gaussian states and photon number measurements the maximization of the heralding probability can be formulated as finding solution to a system of polynomial equations, which offers an efficient way to find the optimal configuration and allows us to apply techniques dedicated specifically to solving such systems of equations. Our approach can seamlessly incorporate bounds on the available single-mode quadrature squeezing, which is highly experimentally relevant. We mainly consider generation of finite superpositions of Fock states but show that the approach can be straightforwardly extended to generation of squeezed superpositions of Fock states. We focus on Gaussian states with vanishing coherent displacements, hence the conditionally generated states have well defined photon number parity. We illustrate our general methodology through examples of generation of single-mode states with two and three heralding modes, and generation of two-mode states with two heralding modes.
Current sources of heralded single photons based on nonlinear optics operate in a probabilistic manner. In order to build quantum-enhanced devices based around the use of single photons, compact, turn-key and deterministic sources are required. A possible solution is to multiplex a number of sources to increase the single-photon generation probability and in so doing reducing the waiting time to deliver large numbers of photons simultaneously, from independent sources. Previously it has been shown that, in the ideal case, 17 multiplexed sources allow deterministic generation of heralded single photons [Christ and Silberhorn, Phys. Rev. A 85, 023829 (2012)]. Here we extend this analysis to include undesirable effects of detector inefficiency and photon loss on a number of multiplexed sources using a variety of different detectors for heralding. We compare these systems for fixed signal-to-noise ratio to allow a direct comparison of performance for real- world heralded single photon sources.