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arXiv:0707.1221 · Physical Review A

Motional frequency shifts of trapped ions in the Lamb-Dicke regime

Ion Lizuain, Juan Gonzalo Muga, Jürgen Eschner

Published Sep 7, 2007• 16 citations
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Abstract

First order Doppler effects are usually ignored in laser driven trapped ions when the recoil frequency is much smaller than the trapping frequency (Lamb-Dicke regime). This means that the central, carrier excitation band is supposed to be unaffected by vibronic transitions in which the vibrational number changes. While this is strictly true in the Lamb-Dicke limit (infinitely tight confinement), the vibronic transitions do play a role in the Lamb-Dicke regime. In this paper we quantify the asymptotic behavior of their effect with respect to the Lamb-Dicke parameter. In particular, we give analytical expressions for the frequency shift, ``pulling'' or ``pushing,'' produced in the carrier absorption band by the vibronic transitions both for Rabi and Ramsey schemes. This shift is shown to be independent of the initial vibrational state.

DOI
10.1103/physreva.76.033808

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First order Doppler effects are usually ignored in laser driven trapped ions when the recoil frequency is much smaller than the trapping frequency (Lamb-Dicke regime). This means that the central, carrier excitation band is supposed to be unaffected by vibronic transitions in which the vibrational number changes. While this is strictly true in the Lamb-Dicke limit (infinitely tight confinement), the vibronic transitions do play a role in the Lamb-Dicke regime. In this paper we quantify the asymptotic behavior of their effect with respect to the Lamb-Dicke parameter. In particular, we give analytical expressions for the frequency shift, pulling'' or pushing,'' produced in the carrier absorption band by the vibronic transitions both for Rabi and Ramsey schemes. This shift is shown to be independent of the initial vibrational state.
We investigate laser-driven vibronic transitions of a single two-level atomic ion in harmonic and hard-wall traps. In the Lamb-Dicke regime, for tuned or detuned lasers with respect to the internal frequency of the ion, and weak or strong laser intensities, the vibronic transitions occur at well-isolated Rabi resonances, where the detuning-adapted Rabi frequency coincides with the transition frequency between vibrational modes. These vibronic resonances are characterized as avoided crossings of the dressed levels (eigenvalues of the full Hamiltonian). Their peculiarities due to symmetry constraints and trapping potential are also examined.
The interaction of a cold trapped ion with a strong laser field is studied in a configuration in which quasienergetic levels become important but heating of the system is unessential. Absorption spectroscopy of the quasienergetic states of a strongly confined and laser-driven trapped ion is analyzed by probing vibrational transitions. Calculations are carried out analytically by using the master equation in quasienergetic state representation. We consider a V\mathsf{V}V-level scheme for the ion with a resonant strong pump field and a weak probe field. The steady-state and time-evolution behavior of the system is discussed and the probe-field absorption spectrum for various initial population distributions of the motional state is calculated. It is found that the absorption spectrum displays vibrational sidebands with multipeak splitting due to the nonlinear dependence of the Rabi frequencies on both the Lamb-Dicke parameter and the trap occupation number. This multipeak splitting has interesting consequences and can be useful for the measurement of the initial trap number population distribution.
The first sideband Raman excitations driven by counter-propagating Raman beams are analysed for the trapped ion under the localization condition in or beyond the Lamb-Dicke regime. It is demonstrated that multiquantum processes in the vibrational couplings produce significant effects on the the first sideband Raman transitions and the relevant Raman displacements for the trapped ion beyond the Lamb-Dicke regime. The quantum features of the vibrational states attained by displacing the motional ground state are demonstrated to be closely associated with the nonlinear vibronic couplings. Quantum entanglement, and quantum interference as well, are discussed for ion traps with various Raman excitation and localization conditions. The results are compared with the recent experiment reported by Monroe C et al in 1996 Science 272 1131-5.
For a single trapped ion, the excitation spectrum of a narrow optical transition consists of a Doppler- and recoil-free carrier accompanied by motional sidebands, which are equally spaced by the trap secular frequency and lie under a Doppler-broadened envelope that is shifted by the photon recoil. Outside the Lamb-Dicke regime, the large photon recoil distributes the line strength across many sidebands and suppresses excitation of the carrier. With multiple ions, the motional spectrum becomes dense, and the carrier is further weakened. Here, we predict a counterintuitive revival effect: increasing the number of ions in a linear chain can restore strong carrier excitation even under trapping conditions far from the single-ion Lamb-Dicke regime. Using a quantum-mechanical model of the excitation dynamics in linear ion chains, we find that sufficiently long chains concentrate the spectrum into the carrier. This effect enables efficient excitation of light ions at short wavelengths. It may also benefit multi-ion optical clocks and mixed-species quantum-logic spectroscopy.
It is well known that electronic transitions driven by nearly resonant travelling- or standing- wave lasers are often accompanied with vibrational sideband transitions of a single trapped ion undergoing quantized center-of-mass motion [1], Our previous studies showed that quantum statistics of radiation fields can be used to manipulate the vibronic motion of a trapped ion localised within the Lamb-Dicke limit (LDL) [2]. The present paper addresses quantum manipulating vibronic motion of an ion trapped far beyond the LDL.
The effects of higher-order Lamb–Dicke approximations (LDAs), on engineering motional quantum states of a single trapped cold ion, are discussed. By measuring the internally electronic states of a single trapped cold ion, which is driven by two classical laser beams tuning respectively to the first upper and lower sidebands, we show that the externally macroscopic vibrational states superposed by either even or odd number states are generated. Under the LDA (i.e., only the first order effect of LD parameter η is considered), these states just are the usual even and odd coherent states. For relative large values of η, we showed that the effects of higher-order LDAs, i.e., terms relating to ηk, k ≥ 2, are not negligible. They might significantly enhance certain nonclassical properties, e.g., squeezing and antibunching effects of the generated macroscopic quantum states.