We systematically investigate the universal spin decoherence dynamics of a localized electron in an arbitrary nuclear spin bath, which can even be far away from equilibrium due to the weak nuclear-lattice interaction. We show that the electron spin relaxation dynamics (as well as spin pure dephasing and Hahn echo decay) can always have a universal behavior as long as the initial state is composed of a sufficiently large amount of spin eigenstates. For a given system, the pattern of the universal dynamics depends on the complicated initial condition only via a single parameter, which measures the amount of phase coherence between different spin eigenstates in the initial state. Our results apply even when the number of the involved nuclei is not large and, therefore, provide a solid foundation in the comparison of the theoretical/numerical results to the experimental measurement. As an example, we also show the numerical results for systems of noninteracting spin bath in a zero magnetic field regime and discuss the features of universal decoherent dynamics.
We systematically investigate the universal spin decoherence dynamics of a localized electron in an arbitrary nuclear spin bath, which can even be far away from equilibrium due to the weak nuclear-lattice interaction. We show that the electron spin relaxation dynamics (as well as spin pure dephasing and Hahn echo decay) can always have a universal behavior as long as the initial state is composed of a sufficiently large amount of spin eigenstates. For a given system, the pattern of the universal dynamics depends on the complicated initial condition only via a single parameter, which measures the amount of phase coherence between different spin eigenstates in the initial state. Our results apply even when the number of the involved nuclei is not large and, therefore, provide a solid foundation in the comparison of the theoretical/numerical results to the experimental measurement. As an example, we also show the numerical results for systems of noninteracting spin bath in a zero magnetic field regime and discuss the features of universal decoherent dynamics.
We study decoherence induced on a two-level system coupled to a one-dimensional quantum spin chain. We consider the cases where the dynamics of the chain is determined by the Ising, XY, or Heisenberg exchange Hamiltonian. This model of quantum baths can be of fundamental importance for the understanding of decoherence in open quantum systems, since it can be experimentally engineered by using atoms in optical lattices. As an example, here we show how to implement a pure dephasing model for a qubit system coupled to an interacting spin bath. We provide results that go beyond the case of a central spin coupled uniformly to all the spins of the bath, in particular showing what happens when the bath enters different phases, or becomes critical; we also study the dependence of the coherence loss on the number of bath spins to which the system is coupled and we describe a coupling-independent regime in which decoherence exhibits universal features, irrespective of the system-environment coupling strength. Finally, we establish a relation between decoherence and entanglement inside the bath. For the Ising and the XY models we are able to give an exact expression for the decay of coherences, while for the Heisenberg bath we resort to the numerical time-dependent density matrix renormalization group.
The quantum dynamics of mesoscopic or macroscopic systems is always complicated by their coupling to many `environmental' modes. At low T these environmental effects are dominated by localized modes, such as nuclear and paramagnetic spins, and defects (which also dominate the entropy and specific heat). This environment, at low energies, maps onto a `spin bath' model. This contrasts with `oscillator bath' models (originated by Feynman and Vernon) which describe delocalized environmental modes such as electrons, phonons, photons, magnons, etc. The couplings to N spin bath modes are independent of N (rather than the ~O(1/( N ) 1/2 ) dependence typical of oscillator baths), and often strong. One cannot in general map a spin bath to an oscillator bath (or vice versa); they constitute distinct `universality classes' of quantum environment. We show how the mapping to spin bath models is made, and then discuss several examples in detail, including moving particles, magnetic solitons, nanomagnets, and SQUIDs, coupled to nuclear and paramagnetic spin environments. We then focus on the `central spin' model, which couples a central two-level system to a background spin bath. It is the spin bath analogue of the famous `spin-boson' oscillator model, and describes, e.g., the tunnelling dynamics of nanoscopic and mesoscopic magnets and superconductors. We show how to average over (or `integrate out') spin bath modes, using an operator instanton technique, to find the central spin dynamics. The formal manouevres involve four separate averages - each average corresponds physically to a different `decoherence' mechanism acting on the central spin dynamics. Each environmental spin has its own topological `spin phase', which by interacting with the phase of the central system, decoheres it - this can happen even without dissipation. We give analytic results for the central spin correlation functions, under various conditions. We then describe the application of this theory to magnetic and superconducting systems. Particular attention is given to recent work on tunnelling magnetic macromolecules, where the role of the nuclear spin bath in controlling the tunnelling is very clear; we also discuss other magnetic systems in the quantum regime, and the influence of nuclear and paramagnetic spins on flux dynamics in SQUIDs. Finally, we discuss decoherence mechanisms and coherence experiments in superconductors and magnets. We show that a spin bath environment causes decoherence even in the T 0 limit. Control of this decoherence will be essential in the effort to construct `qubits' for quantum computers.
We investigate in detail, using both analytical and numerical tools, the decoherence of electron spins in quantum dots (QDs) coupled to a bath of nuclear spins in magnetic fields or with various initial bath polarizations, focusing on the longitudinal relaxation in low and moderate field and polarization regimes. An increase of the initial polarization of nuclear-spin bath has the same effect on the decoherence process as an increase of the external magnetic field, namely, the decoherence dynamics changes from smooth decay to damped oscillations. This change can be observed experimentally for a single QD and for a double-QD setup. Our results indicate that substantial increase of the decoherence time requires very large bath polarizations, and the use of other methods (dynamical decoupling or control of the nuclear spins distribution) may be more practical for suppressing decoherence of QD-based qubits.
We study the decoherence of a spin in a quantum dot due to its hyperfine coupling to a randomly fluctuating bath of nuclear spins. The system is modeled by the central spin model with the spin bath initially being at infinite temperature. We calculate the spectrum and time evolution of the coherence factor using a Monte Carlo sampling of the exact eigenstates obtained via the algebraic Bethe ansatz. The exactness of the obtained eigenstates allows us to study the nonperturbative regime of weak magnetic fields in a full quantum mechanical treatment. In particular, we find a large nondecaying fraction in the zero-field limit. The crossover from strong to weak fields is similar to the decoherence starting from a pure initial bath state treated previously. We compare our results to a simple semiclassical picture [Merkulov et al., Phys. Rev. B 65, 205309 (2002)] and find surprisingly good agreement. Finally, we discuss the effect of weakly coupled spins and show that they will eventually lead to complete decoherence.
We solve the long-standing central spin problem for a general set of inhomogeneous bath couplings and a large class of initial bath states. We compute the time evolution of the coherence of a central spin coupled to a spin bath by resumming all orders of the time-convolutionless master equation, thus avoiding the need to assume weak coupling to the bath. The fully quantum, non-markovian solution is obtained in the large-bath limit and is valid up to a time scale set by the largest coupling constant. Our result captures the full decoherence of an electron spin qubit coupled to a nuclear spin bath in a GaAs quantum dot for experimentally relevant parameters. In addition, our solution is quite compact and can readily be used to make quantitative predictions for the decoherence process and to guide the design of nuclear state preparation protocols.
Control of electron spin decoherence in contact with a mesoscopic bath of many interacting nuclear spins in an InAs quantum dot is studied by solving the coupled quantum dynamics. The nuclear spin bath, because of its bifurcated evolution predicated on the electron spin up or down state, measures the which-state information of the electron spin and hence diminishes its coherence. The many-body dynamics of the nuclear spin bath is solved with a pair-correlation approximation. In the relevant timescale, nuclear pair-wise flip–flops, as elementary excitations in the mesoscopic bath, can be mapped into the precession of non-interacting pseudo-spins. Such mapping provides a geometrical picture for understanding the decoherence and for devising control schemes. A close examination of nuclear bath dynamics reveals a wealth of phenomena and new possibilities of controlling the electron spin decoherence. For example, when the electron spin is flipped by a π-pulse at τ, its coherence will partially recover at as a consequence of quantum disentanglement from the mesoscopic bath. In contrast to the re-focusing of inhomogeneously broadened phases by conventional spin-echoes, the disentanglement is realized through shepherding quantum evolution of the bath state via control of the quantum object. A concatenated construction of pulse sequences can eliminate the decoherence with arbitrary accuracy, with the nuclear–nuclear spin interaction strength acting as the controlling small parameter.