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arXiv:0706.4029 · New Journal of Physics

Dynamics of a qubit coupled to a broadened harmonic mode at finite detuning

Francesco Nesi, Milena Grifoni, Elisabetta Paladino

Published Sep 10, 2007• 29 citations
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Abstract

We study the dynamics of a symmetric two-level system strongly coupled to a broadened harmonic mode. Upon mapping the problem on to a spin–boson model with peaked spectral density, we show how analytic solutions can be obtained, at arbitrary detuning and finite temperatures, in the case of large Q -factors of the oscillator. One, two or more dominating oscillation frequencies of the two-level particle can be observed as a consequence of the entanglement with the oscillator. Our approximated analytical solution agrees well with numerical predictions obtained within the non-interacting blip approximation.

DOI
10.1088/1367-2630/9/9/316

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In this PhD thesis we have been concerned with dissipative and decoherence processes which take place specifically for quantum systems in a dissipative bistable potential. This potential describes a Hamiltonian system whose spectrum is composed by a ladder of levels, grouped as doublets under the potential barrier and being almost equally spaced above it. The system interacts with a thermal environment, fully characterized by the so-called bath spectral density. The dynamical quantity we looked at is the so-called reduced density matrix (RDM), obtained by tracing out the full density matrix the environmental degrees of freedom. The matrix elements for the RDM are exactly evaluated by means of the Feynman-Vernon real-time path-integral technique. Depending on which regime of parameters we are interested in, i.e. temperature and coupling strength with the reservoir, a few or several energy levels contribute to the dynamics. In particular, a two-level system (TLS) is first analyzed, corresponding to the regime where only the lowest doublet is energetically accessible. We discussed in the beginning the case of a TLS interacting with Ohmic and super-Ohmic baths and then the situation in which a symmetric TLS is assumed to be coupled with an external detector, like a dc-SQUID, the latter being coupled to an Ohmic environment. This model provides a better description of a real qubit, as frequently discussed in various experiments. In the former case, we developed a theory called Weakly-Interacting Blip Approximation (WIBA), which is nonperturbative in the coupling strength as well as in the tunneling frequency and gives reliable results over a wide range of temperatures and coupling strength to the thermal environment. In the latter case, the dynamics was evaluated upon starting from the Non-Interacting Blip Approximation (NIBA) and approximating the NIBA kernels up to first order in the detector-bath coupling strength. Analytical results, valid also at finite detuning, were obtained and we showed that our theory correctly reproduces the onset of multiple oscillation frequencies in the dynamics due to the entanglement between TLS and detector. Finally, we discussed the more general case of an M-level system coupled with an Ohmic environment. This situation describes the case of a bistable potential where the temperature is high enough that higher-lying energy levels are being populated and the system cannot be reduced to a simple TLS. Many are the experimental situations which can be described by our theory. We developed a novel approximation called Weakly-Interacting VR-Blip Approximation (VR-WIBA) for the dynamics in a driven dissipative bistable potential. In the regimes of low to moderate temperatures and coupling strengths, we exploited a separation of time scales between tunneling and vibrational relaxation events and we could derive analytical kernels for the intra- and inter-well dynamics.

•Jan 1, 2007•1 citation
We study the dynamics of a symmetric two-level system strongly coupled to a broadened harmonic mode. Upon mapping the problem on to a spin–boson model with peaked spectral density, we show how analytic solutions can be obtained, at arbitrary detuning and finite temperatures, in the case of large Q -factors of the oscillator. One, two or more dominating oscillation frequencies of the two-level particle can be observed as a consequence of the entanglement with the oscillator. Our approximated analytical solution agrees well with numerical predictions obtained within the non-interacting blip approximation.
We propose an approximation scheme to describe the dynamics of the spin-boson model when the spectral density of the environment shows a peak at a characteristic frequency ΩΩΩ which can be very close (or even equal) to the spin Zeeman frequency ΔΔΔ. Mapping the problem onto a two-state system (TSS) coupled to a harmonic oscillator (HO) with frequency ω0ω_0ω0​ we show that the representation of displaced HO states provides an appropriate basis to truncate the Hilbert space of the TSS-HO system and therefore a better picture of the system dynamics. We derive an effective Hamiltonian for the TSS-HO system, and show it furnishes a very good approximation for the system dynamics even when its two subsystems are moderately coupled. Finally, assuming the regime of weak HO-bath coupling and low temperatures, we are able to analytically evaluate the dissipative TSS dynamics.
Abstract. We propose an approximation scheme to describe the dynamics of the spin-boson model when the spectral density of the environment shows a peak at a characteristic frequency Ω which can be very close (or even equal) to the spin Zeeman frequency ∆. Mapping the problem onto a two-state system (TSS) coupled to a harmonic oscillator (HO) with frequency ω0 we show that the representation of displaced HO states provides an appropriate basis to truncate the Hilbert space of the TSS-HO system and therefore a better picture of the system dynamics. We derive an effective Hamiltonian for the TSS-HO system, and show it furnishes a very good approximation for the system dynamics even when its two subsystems are moderately coupled. Finally, assuming the regime of weak HO-bath coupling and low temperatures, we are able to analytically evaluate the dissipative TSS dynamics.
We present a novel approximation scheme to describe the influence of a harmonic bath on the dynamics of a two-level particle over almost the whole regime of temperatures and coupling to the environment, for a wide class of bath spectral densities. Starting from the exact path integral solution for the two-level system density matrix, effective intra-blip correlations are fully included, while inter-blip and blip-sojourn interactions are considered up to first order. In the proper regimes, an excellent agreement with conventional perturbative approaches and ab initio path-integral results is found.
We consider the Landau-Zener problem for a two-level system (or qubit) when this system interacts with one harmonic oscillator mode that is initially set to a finite-temperature thermal equilibrium state. The oscillator could represent an external mode that is strongly coupled to the qubit, e.g., an ionic oscillation mode in a molecule, or it could represent a prototypical uncontrolled environment. We analyze the qubit's occupation probabilities at the final time in a number of regimes, varying the qubit and oscillator frequencies, their coupling strength, and the temperature. In particular, we find a surprising nonmonotonic dependence on the coupling strength and temperature.
The dissipative quantum dynamics of a two-level system interacting with a structured reservoir consisting of a damped harmonic mode is investigated by means of the numerically exact path integral Monte Carlo method. This approach provides benchmark results in a broad range of parameter space, in particular, in those domains which are not accessible by approximate methods and alternative numerical schemes, that is, strong coupling between system and harmonic mode and from low to high temperatures. For low temperatures the numerical data are quantitatively in agreement with the noninteracting blip approximation only in the regimes of very weak and very strong coupling. It turns out that the entangled dynamics of the two-level system and the harmonic mode is relatively robust so that its signatures are observable up to relatively strong friction and high temperatures. Nonequilibrium initial preparations of the reservoir with respect to the initial state of the system give rise, for strong interactions, to a stepwise decay of the population, thus displaying coherent dynamics of the bath. The impact of an additional Ohmic bath coupled directly to the two-level system is studied as well, including the case where both reservoirs carry different temperatures.
In this PhD thesis we have been concerned with dissipative and decoherence processes which take place specifically for quantum systems in a dissipative bistable potential. This potential describes a Hamiltonian system whose spectrum is composed by a ladder of levels, grouped as doublets under the potential barrier and being almost equally spaced above it. The system interacts with a thermal environment, fully characterized by the so-called bath spectral density. The dynamical quantity we looked at is the so-called reduced density matrix (RDM), obtained by tracing out the full density matrix the environmental degrees of freedom. The matrix elements for the RDM are exactly evaluated by means of the Feynman-Vernon real-time path-integral technique. Depending on which regime of parameters we are interested in, i.e. temperature and coupling strength with the reservoir, a few or several energy levels contribute to the dynamics. In particular, a two-level system (TLS) is first analyzed, corresponding to the regime where only the lowest doublet is energetically accessible. We discussed in the beginning the case of a TLS interacting with Ohmic and super-Ohmic baths and then the situation in which a symmetric TLS is assumed to be coupled with an external detector, like a dc-SQUID, the latter being coupled to an Ohmic environment. This model provides a better description of a real qubit, as frequently discussed in various experiments. In the former case, we developed a theory called Weakly-Interacting Blip Approximation (WIBA), which is nonperturbative in the coupling strength as well as in the tunneling frequency and gives reliable results over a wide range of temperatures and coupling strength to the thermal environment. In the latter case, the dynamics was evaluated upon starting from the Non-Interacting Blip Approximation (NIBA) and approximating the NIBA kernels up to first order in the detector-bath coupling strength. Analytical results, valid also at finite detuning, were obtained and we showed that our theory correctly reproduces the onset of multiple oscillation frequencies in the dynamics due to the entanglement between TLS and detector. Finally, we discussed the more general case of an M-level system coupled with an Ohmic environment. This situation describes the case of a bistable potential where the temperature is high enough that higher-lying energy levels are being populated and the system cannot be reduced to a simple TLS. Many are the experimental situations which can be described by our theory. We developed a novel approximation called Weakly-Interacting VR-Blip Approximation (VR-WIBA) for the dynamics in a driven dissipative bistable potential. In the regimes of low to moderate temperatures and coupling strengths, we exploited a separation of time scales between tunneling and vibrational relaxation events and we could derive analytical kernels for the intra- and inter-well dynamics.