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arXiv:quant-ph/9810004 · Physical Review A

Classical and quantum signatures of competing χ(2) nonlinearities

Andrew G. White, Ping Koy Lam, Matthew S. Taubman, Monika A. M. Marte, Stephan Schiller, David E. McClelland, Hans‐A. Bachor

Published Jun 1, 1997• 33 citations
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Abstract

We report the observation of the quantum effects of competing ${\mathrm{\ensuremath{\chi}}}^{(2)}$ nonlinearities. We also report classical signatures of competition, namely, clamping of the second-harmonic power and production of nondegenerate frequencies in the visible. Theory is presented that describes the observations as resulting from competition between various ${\mathrm{\ensuremath{\chi}}}^{(2)}$ up-conversion and down-conversion processes. We show that competition imposes hitherto unsuspected limits to both power generation and squeezing. The observed signatures are expected to be significant effects in practical systems.

DOI
10.1103/physreva.55.4511

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Physical Review A•Mar 1, 1994•60 citations
We report the observation of the quantum effects of competing \ensuremathχ(2){\mathrm{\ensuremath{\chi}}}^{(2)}\ensuremathχ(2) nonlinearities. We also report classical signatures of competition, namely, clamping of the second-harmonic power and production of nondegenerate frequencies in the visible. Theory is presented that describes the observations as resulting from competition between various \ensuremathχ(2){\mathrm{\ensuremath{\chi}}}^{(2)}\ensuremathχ(2) up-conversion and down-conversion processes. We show that competition imposes hitherto unsuspected limits to both power generation and squeezing. The observed signatures are expected to be significant effects in practical systems.
The mutual influence of second-harmonic generation and nondegenerate downconversion inside the same cavity is studied. The threshold behavior and the stability of a semiclassical solution with all four modes oscillating resonantly is investigated. It is shown that under certain conditions the self-pulsing instability that occurs in second-harmonic generation is absent in the combined system. The squeezing spectra for the quadrature-phase amplitudes in the second harmonic and the fundamental, as well as the photon statistics in the downconverted modes, are derived analytically. As one of the various nonclassical features of this system, the second harmonic is found to exhibit excellent noise suppression at very large frequencies, with the frequency component of best squeezing being tunable by the pump parameter. The intricate interaction of the two nonlinear processes can give rise to twin beams of correlated photons, with sub-Poissonian statistics in each beam. These results are contrasted with the results for each nonlinear process by itself.
The competition between the ${\ensuremath{\chi}}^{(2)}$ nonlinearity of a resonant second-harmonic-generation (SHG) system and an added ${\ensuremath{\chi}}^{(3)}$ nonlinearity shifts the Hopf bifurcation of the standard SHG towards higher photon numbers eventually completely stabilizing the system. Remarkably, perfect squeezing survives the stabilization. Two important consequences are discussed, namely, efficient bright squeezing generation and strong suppression of the excess noise which, for parameters corresponding to an experiment reported in the literature, can be reduced by two orders of magnitude without diminishing the squeezing. Possible experimental implementations are finally discussed.
Abstract In this work, we examine the quantum features of a multi-waveguide nonlinear coupler exploiting the second-and third-order nonlinearities. The considered system contains four identical channels, each with a single fundamental transverse mode. The essence of this type of nonlinear coupler is to examine the effect of two or more competing nonlinearities on the generated nonclassical features in this class of devices. Here, we consider the case of second harmonic generation, wherein the fundamental harmonic (FH) fields are up-converted in pairs to double-frequency second harmonic (SH) fields, which are then evanescently coupled with the fields from other Kerr nonlinear waveguides. Using the positive P representation of the phase space, the time-evolution of the density matrix could be mapped to the corresponding Fokker–Planck equation of a classical quasiprobability distribution. Using Langevin stochastic equation, an exact representation of the system in phase space led to the demonstration of sub-Poissonian property, squeezing, and entanglement. With more effective squeezing achieved in all channel waveguides, the present system with χ(2)–χ(3) interaction can be a more efficient alternative to other versions of nonlinear couplers such as the quantum optical dimer (QOD) and Kerr nonlinear coupler (KNC). Furthermore, such a structure offers more flexibility in coupled-mode interactions in the form of correlation between the modes in different waveguides. This provides a better mechanism for the generation of enhanced nonclassical effects.
The interaction between two cavity resonant nonlinear processes in an intracavity ${\mathrm{\ensuremath{\chi}}}^{(2)}$ medium is studied, namely frequency doubling of a pump field of frequency ${\mathrm{\ensuremath{\omega}}}_{1}$ and subsequent down-conversion of the second harmonic to a pair of photons of frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$\ifmmode\pm\else\textpm\fi{}\ensuremath{\Delta}. A closed set of semiclassical equations of motion for appropriately chosen quantities of the full system is derived and an explicit stationary solution is given. Its features and stability are discussed, the most striking being a stable plateau in the second harmonic, i.e., the field of frequency ${\mathrm{\ensuremath{\omega}}}_{2}$=2${\mathrm{\ensuremath{\omega}}}_{1}$ becomes independent of the pump field scrE1{\mathit{scrE}}_{1}scrE1​, provided scrE1{\mathit{scrE}}_{1}scrE1​ is larger than a certain threshold value. It is demonstrated that undamped self-pulsing can only prevail, if the ratio of the rates of second harmonic generation over and parametric down-conversion exceeds a value which depends solely on the relative damping rates of the second harmonic and fundamental, which yields a tentative theoretical explanation of the experimentally observed quenching of the self-pulsing.
We analyze the evolution of quantum noise in both the fundamental and the harmonic fields that are undergoing traveling-wave interaction in a second-order [χ(2)] nonlinear medium. Assuming perfect phase matching between the fundamental and the harmonic fields and arbitrary input boundary conditions, the behavior of quantum noise in the propagating fields is studied by linearization of the nonlinear-operator equations around the mean-field values. We first consider the degenerate case that is applicable to type-I phase-matching geometries, obtaining expressions for squeezing in both the fundamental and the harmonic fields. We then analyze the polarization-nondegenerate case that applies to type-II phase-matching geometries. In the special case, when the two orthogonally polarized fundamental inputs are of equal amplitude, we obtain analytical results and show that the type-II phase-matched second-harmonic-generation process can be configured to generate sub-Poissonian light in both polarization components of the fundamental field. Finally, we numerically solve the linearized quadrature-operator equations along with the nonlinear mean-field equations for the general case of type-II phase matching. For both type-I and type-II processes, we find that whenever the fundamental field experiences deamplification it is associated with amplitude squeezing and phase desqueezing. If, in contrast, the fundamental field experiences amplification, then it is accompanied by amplitude desqueezing, but with squeezing in the phase quadrature. The harmonic field is amplitude squeezed if the input boundary condition leads to harmonic conversion and is phase squeezed if the input boundary condition leads to parametric amplification.
We analyze squeezing of both the fundamental and harmonic fields undergoing traveling-wave, second-harmonic generation (SHG) in second-order (${\mathrm{\ensuremath{\chi}}}^{(2)}$) nonlinear media. We take into account depletion of the fundamental field as well as the phase mismatch between the fundamental and harmonic fields. The behavior of the quantum noises on the propagating fields is studied by linearizing the nonlinear operator equations around the mean-field values. We first consider the degenerate case that is applicable to type-I phase-matching geometries, obtaining expressions for squeezing in both the fundamental and harmonic fields under the conditions of perfect phase matching and large phase mismatch. We show that in the case of a large phase mismatch, the intensity-dependent self-phase shift of the fundamental field, arising due to cascading of the ${\mathrm{\ensuremath{\chi}}}^{(2)}$ nonlinearity, is responsible for the squeezing generation. We also numerically solve the linearized quadrature-operator equations together with the nonlinear mean-field equations. We find that in the case of a finite phase mismatch the harmonic field can be highly squeezed. This is in contrast to the perfectly phase-matched case where the maximum squeezing is limited to 50%. Finally, we analyze the nondegenerate case that applies to type-II phase-matching geometries. Here we show that the commonly used type-II phase-matched SHG process with the input harmonic field in the vacuum state is equivalent to a type-I SHG process in parallel with a degenerate optical-parametric process. The latter causes squeezing in the mode that is polarized orthogonal to the fundamental beam. In the perfect phase-matching case, the squeezing in the orthogonally polarized mode follows the simple expression S=1-\ensuremath{\gamma}, where \ensuremath{\gamma} is the harmonic conversion frequency.