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arXiv:quant-ph/9804071 · Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

Coherent and incoherent chaotic tunneling near singlet-doublet crossings

Sigmund Kohler, Ralf Utermann, Peter Hänggi A, Thomas Dittrich

Published Dec 1, 1998• 60 citations
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Abstract

In the spectrum of systems showing chaos-assisted tunneling, three-state crossings are formed when a chaotic singlet intersects a tunnel doublet. We study the dissipative quantum dynamics in the vicinity of such crossings. A harmonically driven double well coupled to a bath serves as a model. Markov and rotating-wave approximations are introduced with respect to the Floquet spectrum of the time-dependent central system. The resulting master equation is integrated numerically. We find various types of transient tunneling, determined by the relation of the level width to the inherent energy scales of the crossing. The decay of coherent tunneling can be significantly retarded or accelerated. Modifications of the quantum asymptotic state by the crossing are also studied. The comparison with a simple three-state model shows that in contrast to the undamped case, the participation of states outside the crossing cannot be neglected in the presence of dissipation.

DOI
10.1103/physreve.58.7219

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In the spectrum of systems showing chaos-assisted tunneling, three-state crossings are formed when a chaotic singlet intersects a tunnel doublet. We study the dissipative quantum dynamics in the vicinity of such crossings. A harmonically driven double well coupled to a bath serves as a model. Markov and rotating-wave approximations are introduced with respect to the Floquet spectrum of the time-dependent central system. The resulting master equation is integrated numerically. We find various types of transient tunneling, determined by the relation of the level width to the inherent energy scales of the crossing. The decay of coherent tunneling can be significantly retarded or accelerated. Modifications of the quantum asymptotic state by the crossing are also studied. The comparison with a simple three-state model shows that in contrast to the undamped case, the participation of states outside the crossing cannot be neglected in the presence of dissipation.
The dynamical behavior of a two-level system coupled linearly to a dissipative bath of two-level systems whose tunneling splittings and coupling parameters are distributed according to an Ohmic spectrum is studied using numerical path integral methods as well as the noninteracting blip approximation for an equivalent harmonic environment characterized by a scaled spectral density. Comparisons with the behaviors of the conventional spin-boson model of similar coupling strength reveal a weaker quenching of coherence in the present case. Finally, the boundary in parameter space between coherent and incoherent dynamics is mapped.
We study the quantal dynamics of a harmonically driven quartic double well in the presence of dissipation. A master equation for the reduced density operator is derived in the Floquet representation. In the classical limit, this system corresponds to a Duffing oscillator with Ohmic damping. We present numerical results for the transient time evolution and for the stationary sate. The influence of the weak dissipation on interference effects in the context of driven tunnelling is discussed on the basis of these results. We find that the coherent suppression of tunnelling can be stabilized by reservoir-induced noise for a suitably chosen temperature.
The interplay between classical chaos and quantum tunneling is examined in driven nonlinear systems, with emphasis on how semi classical phase space structures influence purely quantum transport phenomena. We show that, in the presence of external driving and stochastic perturbations, tunneling rates acquire an activated form determined by effective classical barriers, providing a transparent link between chaotic dynamics and quantum tunneling. Within this framework, chaos assisted tunneling and coherent destruction of tunneling emerge as closely related manifestations of the same underlying phase space restructuring and interference effects induced by driving. The results offer a unified perspective on tunneling control in non integrable systems and remain relevant for modern studies of driven quantum dynamics and decoherence resistant transport.
Double-well potentials are widely used to model phenomena in physics and chemistry. The system is assumed to be formed in a metastable state, its dynamical evolution providing the clues for the interpretation of the experimental data. Quantum mechanics predicts coherent oscillations of probability between wells if the double-well potential is nearly symmetric and irreversible exponential decay if the final well has an infinite width. For very asymmetric double-well potentials, these two extreme behaviors are expected to coexist. The purpose of the present paper is to investigate this coexistence and its evolution as a function of the width of (or density of states in) the second well. In this sense, increasing the density of states can be regarded as a mechanism for coherence breakdown. The dynamical evolution of the metastable state can be simulated by solving numerically the time-dependent Schroedinger equation (TDSE). This approach is general, intuitive, and gives access to time scales and dynamical effects. It also allows the inclusion of phenomenological dissipation.
A compound tunneling mechanism from one integrable region to another mediated by a delocalized state in an intermediate chaotic region of phase space was recently introduced to explain peculiar features of tunneling in certain two-dimensional systems. This mechanism is known as chaos-assisted tunneling. We study its consequences for the distribution of the level splittings and obtain a general analytical form for this distribution under the assumption that chaos assisted tunneling is the only operative mechanism. %The validity of this form can then in %principle be checked either numerically or even experimentally. We have checked that the analytical form we obtain agrees with splitting distributions calculated numerically for a model system in which chaos-assisted tunneling is known to be the dominant mechanism. The distribution depends on two parameters: The first gives the scale of the splittings and is related to the magnitude of the classically forbidden processes, the second gives a measure of the efficiency of possible barriers to classical transport which may exist in the chaotic region. If these are weak, this latter parameter is irrelevant; otherwise it sets an energy scale at which the splitting distribution crosses over from one type of behavior to another. The detailed form of the crossover is also obtained and found to be in good agreement with numerical results for models for chaos-assisted tunneling.
We present a detailed study of the non-Markovian two-state system dynamics for the regime of incoherent quantum tunneling. Using perturbation theory in the system tunneling amplitude $\ensuremath{\Delta}$, and in the limit of strong system-bath coupling, we determine the short-time evolution of the reduced density matrix and thereby find a general equation of motion for the non-Markovian evolution at longer times. We relate the nonlocality in time due to the non-Markovian effects with the environment characteristic response time. In addition, we study the incoherent evolution of a system with a double-well potential, where each well consists of several quantized energy levels. We determine the crossover temperature to a regime where many energy levels in the wells participate in the tunneling process, and observe that the required temperature can be much smaller than the one associated with the system plasma frequency. We also discuss experimental implications of our theoretical analysis.