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arXiv:quant-ph/9708023 · Physical Review Letters

Quantum-Controlled Few-Photon State Generated by Squeezed Atoms

Hiroki Saito, Masahito Ueda

Published Nov 17, 1997• 31 citations
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Abstract

General principles and experimental schemes for generating a desired few-photon state from an aggregate of squeezed atoms are presented. Quantum-statistical information of the collective atomic dipole is found to be faithfully transferred to the photon state even in a few-photon regime. The controllability of few-photon states is shown to increase with increasing the number of squeezed atoms.

DOI
10.1103/physrevlett.79.3869

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This results in still further improvement of the rate of atomic spin squeezing. A complete model includes the effects of photon-atom scattering and other noise and loss effects on the overall rate of squeezing. Previous derivations of noise due to photon-atom scattering have started with the unjustified assumptions that the atomic and photonic decoherence channels were both Gaussian and independent of correlations between the two subsystems. They then proceed with very general statistical arguments that rely upon these simplifications. My work begins with the more fundamental master equation picture in which I find the Linblad jump operators. I find that in general the photonic and atomic loss channels are not independent, with the intensity of the light dictating the details of this dependence, and find the conditions under which the Gaussian approximation holds. Squeezing and loss is initially treated assuming ensembles of spin-1/2 atoms, but this work is further extended to higher dimensional subsystems. For a higher spin case, preparing the atoms in spin coherent states is not optimal. One can engineer a stronger interaction by preparing the atoms in an atomic "cat state", i.e., a superposition of the two stretch states along the direction of propagation of the light beam. The fluctuations of such a state are more strongly coupled to the light, resulting in a stronger nonlinearity. This leads to strong correlations between the atoms, but they are not immediately useful for squeezing; the cat state must be coherently mapped to a coherent state to achieve atomic spin squeezing. The state created in this manner is ultimately more squeezed than that achieved with the same interaction but prepared initially in a coherent state.

•Jul 2, 2011•1 citation
General principles and experimental schemes for generating a desired few-photon state from an aggregate of squeezed atoms are presented. Quantum-statistical information of the collective atomic dipole is found to be faithfully transferred to the photon state even in a few-photon regime. The controllability of few-photon states is shown to increase with increasing the number of squeezed atoms.
This paper develops an idea of manipulating the squeezed atom state to generate a few-photon state whose phase or photon-number fluctuations are prescribed at our disposal. The squeezed atom state is a collective atomic state whose quantum fluctuations in population difference or collective dipole are smaller than those of the coherent atom state. It is shown that the squeezed atom state can be generated by the interaction of atoms with a coherent state of the electromagnetic field, and that it can be used as a tunable source of squeezed radiation. A variety of squeezed states including the photonnumber squeezed state and the phase squeezed state can be produced by manipulating the atomic state. This is owing to the fact that quantumstatistical information of the atomic state is faithfully transferred to that of the photon state. Possible experimental situations to implement our theory are discussed.
This paper develops a method of manipulating the squeezed atom state to generate a few-photon state whose phase or photon-number fluctuations are prescribed at our disposal. The squeezed-atom state is a collective atomic state whose quantum fluctuations in population difference or collective dipole are smaller than those of the coherent atom state. It is shown that the squeezed-atom state can be generated by the interaction of atoms with a coherent state of the electromagnetic field, and that it can be used as a tunable source of squeezed radiation. A variety of squeezed states, including the photon-number squeezed state and the phase squeezed state, can be produced by manipulating the atomic state. This is owing to the fact that quantum-statistical information of the atomic state is faithfully transferred to that of the photon state. Possible experimental situations to implement our theory are discussed.
Quantum control of many body atomic spins is often pursued in the context of an atom-light quantum interface, where a quantized light field acts as a "quantum bus" that can be used to entangle distant atoms. One key challenge is to improve the coherence of the atom-light interface and the amount of atom-light entanglement it can generate, given the constraints of working with multilevel atoms and optical fields in a 3D geometry. We have explored new ways to achieve this, through rigorous optimization of the spatial geometry, and through control of the internal atomic state. Our basic setup consists of a quantized probe beam passing through an atom cloud held in a dipole trap, first generating spin-probe entanglement through the Faraday interaction, and then using backaction from a measurement of the probe polarization to squeeze the collective atomic spin. The relevant figure of merit is the metrologically useful spin squeezing determined by the enhancement in the resolution of rotations of the collective spin, relative to the commonly used spin coherent state. With an optimized free-space geometry, and by using a 2-color probe scheme to suppress tensor light shifts, we achieve 3(2) dB of metrologically useful spin squeezing. We can further increase atom-light coupling by implementing internal state control to prepare spin states with larger initial projection noise relative to the spin coherent state. Under the right conditions this increase in projection noise can lead to stronger measurement backaction and increased atom-atom entanglement. With further internal state control the increased atom-atom entanglement can then be mapped to a basis where it corresponds to improved squeezing of, e.g., the physical spin-angular momentum or the collective atomic clock pseudospin. In practice, controlling the collective spin of N ~ 10⁶ atoms in this fashion is an extraordinarily difficult challenge because errors in the control of individual atoms tend to be highly correlated. By employing precise internal state control, we have prepared and detected projection noise limited "cat" states (which have initial projection noise that is larger by a factor of 2f = 8 for Cs relative to the spin coherent state) and estimate that we can generate up to 6.0(5) dB of metrologically useful spin squeezing, demonstrating the advantage of using the internal atomic structure as a resource for ensemble control.
We summarize our recent work on quantum information with atomic ensembles. In particular, we describe techniques for storing and manipulating quantum information in collective states of mesoscopic ensembles. Quantum information processing is is accomplished by optical excitation into states with strong dipole-dipole interactions. The resulting “dipole blockade” can be used to inhibit transitions into all but singly excited collective states. This can be employed for a controlled generation of collective atomic spin states as well as non-classical photonic states and for scalable quantum logic gates. Furthermore, we present schemes for entangling a very large number of atoms of a spinor 1 Bose Einstein condensate based on collisional interaction between atoms. As a final example, we discuss the possiblilty of creating entangled atomic states of a few bosonic atoms in a setup which mimics a “fractional quantum Hall effect” and allows the manipulation of anyonic excitations.
We present a theoretical framework to describe the collective emission of light by entangled atomic states. Our theory applies to the low-excitation regime, where most of the atoms are initially in the ground state, and relies on a bosonic description of the atomic excitations. In this way, the problem of light emission by an ensemble of atoms can be solved exactly, including dipole-dipole interactions and multiple light scattering. Explicit expressions for the emitted photonic states are obtained in several situations, such as those of atoms in regular lattices and atomic vapors. We determine the directionality of the photonic beam, the purity of the photonic state, and the renormalization of the emission rates. We also show how to observe collective phenomena with ultracold atoms in optical lattices and how to use these ideas to generate photonic states that are useful in the context of quantum information.
In this thesis I explore the use of collective spin angular momentum as a platform for quantum information processing. Such systems have several nice features that make them excellent choices for such protocols, especially ones where information is also stored in photonic variables. The longer coherence times of atoms makes it possible to store information from light in atoms for future use, and it is generally easier to couple atomic variables than to create nonlinear interactions of light. Above and beyond the advantages of atomic systems, collective atomic systems have additional strengths. In the limit of a large number of atoms, the collective variables of atomic systems have a natural connection to the bosonic algebra of light (known as the Holstein-Primakoff or HP approximation) where components of the collective spin angular momentum effectively act as quadratures, making them natural systems for coupling to light. Also, collectively addressing the atoms allows one to access a large state space without individual addressing of the atoms. A natural first step towards control of these collective variables is generating large amounts of atomic spin squeezing. In the HP approximation going from rotations to squeezing corresponds to going from linear to quadratic interactions in the atomic quadratures; for extremely large squeezing one should see the breakdown of the HP approximation and the ability to generate arbitrary collective atomic states. I have sought to improve previous schemes for the spin squeezing of atomic ensembles, such as the proposal of Takeuchi et. al. based on coherent quantum feedback. In this scheme a beam of linearly polarized light passes through the atomic ensemble (prepared in a coherent state), coupling to the atoms through a state-dependent index of refraction (the Faraday effect). The light is then passed through a wave-plate and reflected back through the atoms for a second pass. This double-pass scheme leads to an effective nonlinearity as the atomic fluctuations are mapped onto the light on the first pass and then back on to the atoms in the second pass. The light acts as a bus coupling each atom to each of the others. This nonlinear interaction forms a shearing of the atomic coherent state that results in squeezing. The light is entangled to the atoms through these interactions, and remains entangled as it escapes the system. This leads to decoherence of the atoms as the light is lost to the environment, reducing the amount of spin squeezing achieved. The first step towards improving the double-pass scheme was to add a quantum eraser step in which the light is disentangled from the squeezed atoms. By first measuring one quadrature of the light, and then performing a measurement-dependent rotation on the atomic ensemble, it is possible to decouple the atoms and light so that the loss of the light does not reduce the atomic squeezing. This results in an improvement of the rate of atomic spin squeezing. The nonlinear shearing interaction that remains still falls short of the exponential squeezing seen in optical parametric amplification. The reason for this can be seen by decomposing the shearing interaction into squeezing along a given quadrature followed by a rotation. The rotation leads to a constantly changing axis along which the squeezing occurs, and thus the squeezing builds up more slowly. This can be corrected for by breaking up the light pulse into a sequence of small pulses, and performing a small phase matching rotation after each pulse. The squeezing then adds up along a constant direction, rather than along a constantly varying direction. This results in still further improvement of the rate of atomic spin squeezing. A complete model includes the effects of photon-atom scattering and other noise and loss effects on the overall rate of squeezing. Previous derivations of noise due to photon-atom scattering have started with the unjustified assumptions that the atomic and photonic decoherence channels were both Gaussian and independent of correlations between the two subsystems. They then proceed with very general statistical arguments that rely upon these simplifications. My work begins with the more fundamental master equation picture in which I find the Linblad jump operators. I find that in general the photonic and atomic loss channels are not independent, with the intensity of the light dictating the details of this dependence, and find the conditions under which the Gaussian approximation holds. Squeezing and loss is initially treated assuming ensembles of spin-1/2 atoms, but this work is further extended to higher dimensional subsystems. For a higher spin case, preparing the atoms in spin coherent states is not optimal. One can engineer a stronger interaction by preparing the atoms in an atomic "cat state", i.e., a superposition of the two stretch states along the direction of propagation of the light beam. The fluctuations of such a state are more strongly coupled to the light, resulting in a stronger nonlinearity. This leads to strong correlations between the atoms, but they are not immediately useful for squeezing; the cat state must be coherently mapped to a coherent state to achieve atomic spin squeezing. The state created in this manner is ultimately more squeezed than that achieved with the same interaction but prepared initially in a coherent state.