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arXiv:quant-ph/9707014 · Physical Review Letters

Improvement of Frequency Standards with Quantum Entanglement

Susana F. Huelga, Chiara Macchiavello, Thomas Pellizzari, ARTUR K. EKERT, Martin Bodo Plenio, J. I. Cirac

Published Nov 17, 1997• 999 citations
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Abstract

The optimal precision of frequency measurements in the presence of decoherence is discussed. We analyze different preparations of $n$ two-level systems as well as different measurement procedures. We show that standard Ramsey spectroscopy on uncorrelated atoms and optimal measurements on maximally entangled states provide the same resolution. The best resolution is achieved using partially entangled preparations with a high degree of symmetry.

DOI
10.1103/physrevlett.79.3865

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The optimal precision of frequency measurements in the presence of decoherence is discussed. We analyze different preparations of nnn two-level systems as well as different measurement procedures. We show that standard Ramsey spectroscopy on uncorrelated atoms and optimal measurements on maximally entangled states provide the same resolution. The best resolution is achieved using partially entangled preparations with a high degree of symmetry.
The precision of frequency measurements performed on trapped ions in the presence of decoherence is analysed. In particular, standard Ramsey spectroscopy on uucorrelated ions and optimal measurements on maximally entangled states are proved to lead to the same resolution, while the best precision is achieved using partially entangled preparations. The use of symrnetrisation procedures is proposed and it is shown how this allows to overcome even the optimal precision achievable when both the initial preparation and the final measurement are optimized. These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.
It is known that partially entangled state gives improved sensitivity of Ramsey spectroscopy in the presence of decoherence, whereas maximally entangled state gives no improvement. However it has been an open question whether the absolute limit in the improvement is attainable by optimal entanglement alone or via measurement optimization. In this Paper, we answer this question by showing that even sub-optimal entanglement generated by the simplest spin squeezing can asymptotically attain the absolute improvement with increasing number of atoms.
A quantum system can be prepared in an entangled state that is very sensitive to changes introduced to its dynamics and thus potentially can be utilized as a precise sensor of dynamics parameters. NNN entangled two-level atoms evolving unitarily can be used for frequency estimation with Heisenberg-limited precision which scales as ${N}^{\ensuremath{-}2}$, whereas uncorrelated states give only a standard-limited precision which scales as ${N}^{\ensuremath{-}1}$. As entangled states are also sensitive to disturbances introduced by interactions with external environments, quantum enhancement of the precision may be significantly limited for open quantum systems. This is the case when an interaction with an environment leads to local Markovian dephasing and the precision scales as ${N}^{\ensuremath{-}1}$ for all atom preparations. For local non-Markovian dephasing, however, Matsuzaki et al. [Phys. Rev. A 84, 012103 (2011)] and Chin et al. [Phys. Rev. Lett. 109, 233601 (2012)] showed that the atoms prepared in the maximally entangled state achieve Zeno scaling $\ensuremath{\propto}\phantom{\rule{0.16em}{0ex}}{N}^{\ensuremath{-}3/2}$ in precision and argued that this limit should hold for any entangled state. Here we prove that Zeno scaling is indeed the best possible scaling for all local non-Markovian dephasing models which feature initial Zeno dynamics. Moreover, Zeno scaling can hold only for experiments in the Zeno-dynamics regime, otherwise scaling of the precision is standard.
I analyze a metrological strategy for improving the precision of frequency estimation via Ramsey interferometry with strings of atoms in the presence of correlated dephasing. This strategy does not employ entangled states but rather a product state which evolves into a stationary state under the influence of correlated dephasing. It is shown that by using this state an improvement in precision compared to standard Ramsey interferometry can be gained. This improvement is not an improvement in scaling; i.e., the estimation precision has the same scaling with the number of atoms as the standard quantum limit but gains an improvement proportional to the free evolution time in the Ramsey interferometer. Since a stationary state is used, this evolution time can be substantially larger than in standard Ramsey interferometry which is limited by the coherence time of the atoms.
Squeezing of quantum fluctuations by means of entanglement is a well-recognized goal in the field of quantum information science and precision measurements. In particular, squeezing the fluctuations via entanglement between 2-level atoms can improve the precision of sensing, clocks, metrology, and spectroscopy. Here, we demonstrate 3.4 dB of metrologically relevant squeezing and entanglement for greater, similar 10(5) cold caesium atoms via a quantum nondemolition (QND) measurement on the atom clock levels. We show that there is an optimal degree of decoherence induced by the quantum measurement which maximizes the generated entanglement. A 2-color QND scheme used in this paper is shown to have a number of advantages for entanglement generation as compared with a single-color QND measurement.
Ramsey interferometry is a widely used tool for precisely measuring transition frequencies between two energy levels of a quantum system, with applications in time keeping, precision spectroscopy, quantum optics, and quantum information. Often, the coherence time of the quantum system surpasses the one of the oscillator probing the system, thereby limiting the interrogation time and associated spectral resolution. Correlation spectroscopy overcomes this limitation by probing two quantum systems with the same noisy oscillator for a measurement of their transition frequency difference; this technique has enabled very precise comparisons of atomic clocks. Here, we extend correlation spectroscopy to the case of multiple quantum systems undergoing strong correlated dephasing. We model Ramsey correlation spectroscopy with N particles as a multiparameter phase estimation problem and demonstrate that multiparticle correlations can assist in reducing the measurement uncertainties even in the absence of entanglement. We derive precision limits and optimal sensing techniques for this problem and compare the performance of probe states and measurement with and without entanglement. Using one- and two-dimensional ion Coulomb crystals with up to 91 qubits, we experimentally demonstrate the advantage of measuring multiparticle correlations for reducing phase uncertainties and apply correlation spectroscopy to measure ion-ion distances, transition frequency shifts, laser-ion detunings, and path-length fluctuations. Our method can be straightforwardly implemented in experimental setups with globally coherent qubit control and qubit-resolved single-shot readout and is, thus, applicable to other physical systems such as neutral atoms in tweezer arrays. Published by the American Physical Society 2024