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arXiv:quant-ph/9610013 · Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics

Chaos in time-dependent variational approximations to quantum dynamics

Fred Cooper, John F. Dawson, Salman Habib, Robert D. Ryne

Published Feb 1, 1998• 46 citations

Abstract

Dynamical chaos has recently been shown to exist in the Gaussian approximation in quantum mechanics and in the self-consistent mean field approach to studying the dynamics of quantum fields. In this study, we first note that any variational approximation to the dynamics of a quantum system based on the Dirac action principle leads to a classical Hamiltonian dynamics for the variational parameters. Since this Hamiltonian is generically nonlinear and nonintegrable, the dynamics thus generated can be chaotic, in distinction to the exact quantum evolution. We then restrict our attention to a system of two biquadratically coupled quantum oscillators and study two variational schemes, the leading order large-$N$ (four canonical variables) and Hartree (six canonical variables) approximations. The chaos seen in the approximate dynamics is an artifact of the approximations: this is demonstrated by the fact that its onset occurs on the same characteristic time scale as the breakdown of the approximations when compared to numerical solutions of the time-dependent Schr\"odinger equation.

DOI: 10.1103/physreve.57.1489

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Dynamical chaos has recently been shown to exist in the Gaussian approximation in quantum mechanics and in the self-consistent mean field approach to studying the dynamics of quantum fields. In this study, we first note that any variational approximation to the dynamics of a quantum system based on the Dirac action principle leads to a classical Hamiltonian dynamics for the variational parameters. Since this Hamiltonian is generically nonlinear and nonintegrable, the dynamics thus generated can be chaotic, in distinction to the exact quantum evolution. We then restrict our attention to a system of two biquadratically coupled quantum oscillators and study two variational schemes, the leading order large-

N

(four canonical variables) and Hartree (six canonical variables) approximations. The chaos seen in the approximate dynamics is an artifact of the approximations: this is demonstrated by the fact that its onset occurs on the same characteristic time scale as the breakdown of the approximations when compared to numerical solutions of the time-dependent Schr"odinger equation.

Nonlinearity in Quantum Mechanics may have extrinsic or intrinsic origins and is a liable route to a chaotic behaviour that can be of difficult observations. In this paper, we propose two forms of nonlinear Hamiltonian, which explicitly depend upon the phase of the wave function and produce chaotic behaviour. To speed up the slow manifestation of chaotic effects, a resonant laser field assisting the time evolution of the systems causes cumulative effects that might be revealed, at least in principle. The nonlinear Schrödinger equation is solved within the two-state approximation; the solution displays features with characteristics similar to those found in chaotic Classical Mechanics: sensitivity on the initial state, dense power spectrum, irregular filling of the Poincaré map and exponential separation of the trajectories of the Bloch vector σ in the Bloch sphere.

Based on simple first-order quantum corrections to classical equations of motion, which we show to be closely related to Gaussian wave-packet dynamics (GWD) and a time-dependent variational principle (TDVP), we deduce that quantum corrections to classical dynamics should typically become most pronounced when the classical system becomes chaotic. The time duration over which classical dynamics, GWD, or TDVP may provide good approximations is much shorter when the classical dynamics are chaotic. However, for certain situations involving very short laser pulses, these approximations can be very accurate. The same concepts are applicable to paraxial wave optics, which may offer simpler experimental studies of ``quantum chaos'': the distinction between classical and ``quantum'' chaos is in large part the distinction between ray versus wave behavior.

We investigate variational principles for the approximation of quantum dynamics that apply for approximation manifolds that do not have complex linear tangent spaces. The first one, dating back to McLachlan [Mol. Phys. 8, 39–44 (1964)], minimizes the residuum of the time-dependent Schrödinger equation, while the second one, originating from the lecture notes of Kramer and Saraceno [Geometry of the Time-Dependent Variational Principle in Quantum Mechanics, Lecture Notes in Physics Vol. 140 (Springer, Berlin, 1981)], imposes the stationarity of an action functional. We characterize both principles in terms of metric and symplectic orthogonality conditions, consider their conservation properties, and derive an elementary a posteriori error estimate. As an application, we revisit the time-dependent Hartree approximation and frozen Gaussian wave packets.

We describe a quantum many-body system undergoing multiple resonant tunneling which exhibits chaotic behavior in numerical simulations of a mean field approximation. This phenomenon, which has no counterpart in the classical limit, is due to effective nonlinearities in the tunneling process and can be observed in principle within a heterostructure. 03.65.-w, 05.45.+b, 73.40.Gk Typeset using REVT E X In current studies the problem of quantum chaos is usually posed in the following terms. We are given a system which exhibits chaotic behavior classically: does this property survive quantization? Typically one studies the spectrum of the quantum mechanical Hamiltonian operator. However spectral differences at the quantum level between classically integrable and chaotic systems do not seem to imply dramatic differences in the time evolution of the quantum mechanical observables. Relics of classical chaos exist in low dimensional systems in short wavelength or large quantum numbers limits ...

The time-dependent variational principle using generalized Gaussian trial functions yields a finite dimensional approximation to the full quantum dynamics and is used in many disciplines. It is shown how these ``semiquantum'' dynamics may be derived via the Ehrenfest theorem and recast as an extended classical gradient system with the fluctuation variables coupled to the average variables. An extended potential is constructed for a one-dimensional system. The semiquantal behavior is shown to be chaotic even though the system has regular classical behavior and the quantum behavior had been assumed regular.

I shall discuss the quantum and classical dynamics of a class of nonlinear Hamiltonian systems. The discussion will be restricted to systems with one degree of freedom. Such systems cannot exhibit chaos, unless the Hamiltonians are time dependent. Thus we shall consider systems with a potential function that has a higher than quadratic dependence on the position and, furthermore, we shall allow the potential function to be a periodic function of time. This is the simplest class of Hamiltonian system that can exhibit chaotic dynamics. I shall show how such systems can be realized in atom optics, where very cold atoms interact with optical dipole potentials of a far-off resonance laser. Such systems are ideal for quantum chaos studies as (i) the energy of the atom is small and action scales are of the order of Planck's constant, (ii) the systems are almost perfectly isolated from the decohering effects of the environment and (iii) optical methods enable exquisite time dependent control of the mechanical potentials seen by the atoms.