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arXiv:quant-ph/0703031 · Physical Review A

Cold polar molecules in two-dimensional traps: Tailoring interactions with external fields for novel quantum phases

Andrea Micheli, Guido Pupillo, Hans Peter Büchler, P. Zoller

Published Oct 3, 2007• 221 citations
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Abstract

We discuss techniques to engineer effective long-range interactions between polar molecules using external static electric and microwave fields. We consider a setup where molecules are trapped in a two-dimensional pancake geometry by a far-off-resonance optical trap, which ensures the stability of the dipolar collisions. We detail how to modify the shape and the strength of the long-range part of interaction potentials, which can be utilized to realize interesting quantum phases in the context of cold molecular gases.

DOI
10.1103/physreva.76.043604

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We discuss techniques to engineer effective long-range interactions between polar molecules using external static electric and microwave fields. We consider a setup where molecules are trapped in a two-dimensional pancake geometry by a far-off-resonance optical trap, which ensures the stability of the dipolar collisions. We detail how to modify the shape and the strength of the long-range part of interaction potentials, which can be utilized to realize interesting quantum phases in the context of cold molecular gases.
We discuss techniques to tune and shape the long-range part of the interaction potentials in quantum gases of bosonic polar molecules by dressing rotational excitations with static and microwave fields. This provides a novel tool towards engineering strongly correlated quantum phases in combination with low-dimensional trapping geometries. As an illustration, we discuss the 2D superfluid-crystal quantum phase transition for polar molecules interacting via an electric-field-induced dipole-dipole potential.
We investigate collisions of polar molecules in quasi-2D traps in the presence of an external electric field perpendicular to the collision plane. We use the quantum-defect model characterized by two dimensionless parameters: yyy and sss. The first of them is related to the probability of the reaction at short distances, whereas the latter one defines the wave function phase at short distances. For yyy close to unity we obtain universal collision rates determined by the quantum reflection process from the long-range part of the interaction potential that depends only on the van der Waals coefficient, dipole-dipole interaction and the trap frequency. For small short-range reaction probabilities collision rates are highly nonuniversal and trap induced shape resonances are visible. For high dipole moments we observe the damping of reactive collisions, which can stabilize the ultracold gas of polar molecules. The calculations were performed with help of multichannel wave funcion propagation by imposing short-range boundary condition derived from the quantum-defect model.
We design dipolar quantum many-body Hamiltonians that will facilitate the realization of exotic quantum phases under current experimental conditions achieved for polar molecules. The main idea is to modulate both single-body potential barriers and two-body dipolar interactions on a spatial scale of tens of nanometers to strongly enhance energy scales and, therefore, relax temperature requirements for observing new quantum phases of engineered many-body systems. We consider and compare two approaches. In the first, nanoscale barriers are generated with standing-wave optical light fields exploiting optical nonlinearities. In the second, static electric-field gradients in combination with microwave dressing are used to write nanostructured spatial patterns on the induced electric dipole moments, and thus dipolar interactions. We study the formation of interlayer and interface bound states of molecules in these configurations, and provide detailed estimates for binding energies and expected losses for present experimental setups.
We study quantum degenerate polar molecules with large dipole moments. We show that the internal structure of the polar molecules allows us to tune and shape the long‐range part of the interaction, while the strength of the long‐range interaction easily exceeds the kinetic energy of the gas. The stability of the system is guaranteed by a strong transverse trapping potential confining the particles into two‐dimensional planes. For typical experimental parameters, we find the the ground state is characterized by a crystalline phase, separated from the superfluid phase via a quantum phase transition for a critical interaction strength.