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arXiv:quant-ph/0701224 · Physical Review A

Scattering of polarized laser light by an atomic gas in free space: A quantum stochastic differential equation approach

Luc Bouten, John K. Stockton, Gopal Sarma, Hideo Mabuchi

Published May 23, 2007• 16 citations
arXivHTMLPDF

Abstract

We propose a model, based on a quantum stochastic differential equation (QSDE), to describe the scattering of polarized laser light by an atomic gas. The gauge terms in the QSDE account for the direct scattering of the laser light into different field channels. Once the model has been set, we can rigorously derive quantum filtering equations for balanced polarimetry and homodyne detection experiments, study the statistics of output processes, and investigate a strong driving, weak coupling limit.

DOI
10.1103/physreva.75.052111

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We propose a model, based on a quantum stochastic differential equation (QSDE), to describe the scattering of polarized laser light by an atomic gas. The gauge terms in the QSDE account for the direct scattering of the laser light into different field channels. Once the model has been set, we can rigorously derive quantum filtering equations for balanced polarimetry and homodyne detection experiments, study the statistics of output processes, and investigate a strong driving, weak coupling limit.
Quantum stochastic differential equations have been used to describe the dynamics of an atom interacting with the electromagnetic field via absorption/emission processes. Here, by using the full quantum stochastic Schrödinger equation proposed by Hudson and Parthasarathy, we show that such models can be generalized to include other processes into the interaction. In the case of a two-level atom we construct a model on the basis of some physical requirements, the main being a balance equation on the fluxes of the ingoing and outgoing photons; in this model the atom-field interaction turns out to be due either to absorption/emission processes either to direct scattering processes, which simulate the interaction due to virtual transitions to the levels which have been eliminated from the description. To see the effects of the new terms, we consider both direct and heterodyne detection of the fluorescence light emitted by an atom stimulated by a monochromatic coherent laser and we deduce from these two detection schemes the expressions of the total, elastic and inelastic electromagnetic cross sections and the spectral distribution of the fluorescence light. The total cross section, as a function of the frequency of the stimulating laser, can present not only a Lorentzian shape, but the full variety of Fano profiles; intensity dependent widths and shifts are obtained. The fluorescence spectrum can present complicated shapes, according to the values of the various parameters; when the direct scattering is not important the usual symmetric triplet structure of the Mollow spectrum appears (for high intensity of the stimulating laser), while a strong contribution of the direct scattering process can distort such a triplet structure or can even make it to disappear.
Just at the beginning of quantum stochastic calculus Hudson and Parthasarathy proposed a quantum stochastic Schrodinger equation linked to dilations of quantum dynamical semigroups. Such an equation has found applications in physics, mainly in quantum optics, but not in its full generality. It has been used to give, at least approximately, the dynamics of photoemissive sources such as an atom absorbing and emitting light or matter in an optical cavity, which exchanges light with the surrounding free space. But in these cases the possibility of introducing the gauge (or number) process in the dynamical equation has not been considered. In this paper we show, in the case of the simplest photoemissive source, namely a two-level atom stimulated by a laser, how the full Hudson-Parthasarathy equation allows to describe in a consistent way not only absorption and emission, but also the elastic scattering of the light by the atom. Morever, we study the differential and total cross sections for the scattering of laser light by the atom, as a function of the frequency of the stimulating laser. The resulting line-shape is very interesting. Not only a Lorentzian shape is permitted, but the full variety of Fano profiles can be obtained. The dependence of the line shape on the intensity of the stimulating laser is computed; in particular, the resonance position turns out to be intensity dependent, a phenomenon known as lamp shift.
We show that well above threshold the use of linearized Ito quantum stochastic differential equations allows a systematic description of all quantum stochastic properties of laser light including the phase properties. This is accomplished by the use of mixed field-atom operators which are phase independent and around whose finite mean values we may linearize. As a consequence we are able to derive an equation for an operator describing the phase properties of the laser light. We illustrate our method by applying it to three different models for sub-shot-noise lasers.
The derivation of a quantum Markovian model for an optomechanical system consisting of a quantum mechanical mirror interacting with quantum optical input fields via radiation pressure is a difficult problem which ultimately involves the scattering process of quantum stochastic calculus. We show that, while the scattering process may be approximated in a singular limit by regular processes using different schemes, the limit model is highly sensitive to the mathematical interpretation of the approximation scheme. We find two main types of stochastic limits of regular models, and illustrate the origin of this difference at the level of one-particle scattering. As an alternative modeling scheme, we consider models of mirrors as nontrivial dielectric media with boundaries that are themselves quantized. Rather than treating the plane waves for the electromagnetic field, we take the actual physical modes and quantize these. The input-output formalism is then obtained in the far zone where the plane-wave approximation is valid. Several examples are considered, and the quantum stochastic model is derived. We also consider the quantum trajectories problem for continual measurement of the reflected output fields, and derive the stochastic master equations for homodyning and photon-counting detection to estimate the mirror observables.
By means of quantum stochastic calculus we construct a model for an atom with two degenerate levels which is stimulated by a circularly polarized laser and we compute its fluorescence spectrum. Let us stress that, once the model for the unitary atom–field dynamics has been given, then the spectrum is computed without further approximations. If only the absorption/emission term is included in the interaction, we reobtain the Mollow spectrum in the case of a monochromatic laser and the Kimble–Mandel spectrum in the case of a ‘phase diffusion model’ for a non-monochromatic laser. However, our model can also describe another type of light scattering, a ‘direct scattering’ due to the response of the atom as a whole, which we expect to be small but which interferes with the scattering due to the absorption/emission channel. When both the scattering channels are introduced we obtain a modification of the Mollow–Kimble–Mandel spectrum, which shares its main features with the usual case, but which presents some asymmetries even in the case of no detuning.
We study interactions of light with a sample of two-level atoms. Quantum statistical effects of degenerate boson and fermion gases are described by using the quantum field theory of atom-photon interactions, fully including the angular momentum degeneracies. Coupled propagation equations are given for light and matter fields, and plausible general simplifications are enumerated.^ In the limit of large atom-field detuning, multiple scattering of light and QED linewidths and line shifts may be ignored, and the propagation equations of light and matter fields may be decoupled. A general expression for the spectrum of the scattered light is derived, complete with the dependence on atomic level scheme, on various light polarizations, and on the geometry of the experiment. With these simplifications we are able to find distinct qualitative features in the spectrum of the scattered light in the case of both fermions and bosons that depend on the statistics of atoms. This is because for bosons (fermions), those scattering events in which an atom recoils to an already occupied state are enhanced (inhibited).^ As the driving light gets closer to the atomic resonance, multiple scattering and vacuum fluctuations of the electromagnetic fields should also be taken into account. We write the equations of motion for the excited state field operators by eliminating the vacuum electromagnetic field. It is always assumed that the driving external laser field is in the coherent state. We find in the limit of low light intensity, a hierarchy of equations of motion for correlation functions that contain one excited-atom field and one, two, three, etc., ground state atom fields. It is conjectured that the entire linear hierarchy may be solved by solving numerically the classical equations for the coupled system of electromagnetic fields and charged harmonic oscillators. We discuss the emergence of resonant dipole-dipole interactions and collective linewidths, and delineate the limits of validity of the column density approach in terms of non-cooperative atoms by presenting a mathematical example in which this approach is exact. ^