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arXiv:quant-ph/0701167 · Physical Review Letters

Cold-Atom Physics Using Ultrathin Optical Fibers: Light-Induced Dipole Forces and Surface Interactions

G. Sagué, E. Vetsch, Wolfgang Alt, Dieter Meschede, Arno Rauschenbeutel

Published Oct 16, 2007• 174 citations
arXivHTMLPDF

Abstract

The strong evanescent field around ultrathin unclad optical fibers bears a high potential for detecting, trapping, and manipulating cold atoms. Introducing such a fiber into a cold-atom cloud, we investigate the interaction of a small number of cold cesium atoms with the guided fiber mode and with the fiber surface. Using high resolution spectroscopy, we observe and analyze light-induced dipole forces, van der Waals interaction, and a significant enhancement of the spontaneous emission rate of the atoms. The latter can be assigned to the modification of the vacuum modes by the fiber.

DOI
10.1103/physrevlett.99.163602

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The strong evanescent field around ultrathin unclad optical fibers bears a high potential for detecting, trapping, and manipulating cold atoms. Introducing such a fiber into a cold-atom cloud, we investigate the interaction of a small number of cold cesium atoms with the guided fiber mode and with the fiber surface. Using high resolution spectroscopy, we observe and analyze light-induced dipole forces, van der Waals interaction, and a significant enhancement of the spontaneous emission rate of the atoms. The latter can be assigned to the modification of the vacuum modes by the fiber.
We study the force of light on a two-level atom near an ultrathin optical fiber using the mode function method and the Green tensor technique. We show that the total force consists of the driving-field force, the spontaneous-emission recoil force, and the fiber-induced van der Waals potential force. Due to the existence of a nonzero axial component of the field in a guided mode, the Rabi frequency and, hence, the magnitude of the force of the guided driving field may depend on the propagation direction. When the atomic dipole rotates in the meridional plane, the spontaneous-emission recoil force may arise as a result of the asymmetric spontaneous emission with respect to opposite propagation directions. The van der Waals potential for the atom in the ground state is off-resonant and opposite to the off-resonant part of the van der Waals potential for the atom in the excited state. Unlike the potential for the ground state, the potential for the excited state may oscillate depending on the distance from the atom to the fiber surface.
In this thesis, I present the realization of a fiber-optical interface using optically trapped cesium atoms, which is an efficient tool for coupling light and atoms. The basic principle of the presented scheme relies on the trapping of neutral cesium atoms in a two-color evanescent field surrounding a nanofiber. The strong confinement of the fiber guided light, which also protrudes outside the nanofiber, provides strong confinement of the atoms as well as efficient coupling to near-resonant light propagating through the fiber. In chapter 1, the necessary physical and mathematical background describing the propagation of light in an optical fiber is presented. The exact solution of Maxwell’s equations allows us to model fiber-guided light fields which give rise to the trapping potentials and the atom-light coupling in the close vicinity of a nanofiber. Chapter 2 gives the theoretical background of light-atom interaction. A quantum mechanical model of the light-induced shifts of the relevant atomic levels is reviewed, which allows us to quantify the perturbation of the atomic states due to the presence of the trapping light-fields. The experimental realization of the fiber-based atom trap is the focus of chapter 3. Here, I analyze the properties of the fiber-based trap in terms of the confinement of the atoms and the impact of several heating mechanisms. Furthermore, I demonstrate the transportation of the trapped atoms, as a first step towards a deterministic delivery of individual atoms. In chapter 4, I present the successful interfacing of the trapped atomic ensemble and fiber-guided light. Three different approaches are discussed, i.e., those involving the measurement of either near-resonant scattering in absorption or the emission into the guided mode of the nanofiber. In the analysis of the spectroscopic properties of the trapped ensemble we find good agreement with the prediction of theoretical model discussed in chapter 2. In addition, I introduce a non-destructive scheme for the interrogation of the atoms states, which is sensitive to phase shifts of far-detuned fiber-guided light interacting with the trapped atoms. The inherent birefringence in our system, induced by the atoms, changes the state of polarization of the probe light and can be thus detected via a Stokes vector measurement.
We study the force of light on a two-level atom near an ultrathin optical fiber using the mode function method and the Green tensor technique. We show that the total force consists of the driving-field force, the spontaneous-emission recoil force, and the fiber-induced van der Waals potential force. Due to the existence of a nonzero axial component of the field in a guided mode, the Rabi frequency and, hence, the magnitude of the force of the guided driving field may depend on the propagation direction. When the atomic dipole rotates in the meridional plane, the spontaneous-emission recoil force may arise as a result of the asymmetric spontaneous emission with respect to opposite propagation directions. The van der Waals potential for the atom in the ground state is off-resonant and opposite to the off-resonant part of the van der Waals potential for the atom in the excited state. Unlike the potential for the ground state, the potential for the excited state may oscillate depending on the distance from the atom to the fiber surface.
We use evanescent laser light to guide atoms through hollow-core optical fibers. The light, detuned to the blue side of rubidium's D2{D}_{2}D2​ resonance lines, is launched into the glass region of a hollow capillary fiber and guided through the fiber by total internal reflection from the glass walls. Atoms interacting with the evanescent component of the field are repelled from the wall and guided through the fiber hollow. A second laser tuned to the red side of resonance is used to initially inject the atoms into the evanescent guide. An optical intensity threshold for guiding is observed as the evanescent-field-induced dipole forces exceed the van der Waals forces.
Tapered optical fiber with subwavelength diameter waist, an optical nanofiber, provides a unique and versatile platform for manipulating atoms and photons. In the guided modes of the nanofibers, the optical field can be tightly confined in the transverse direction while enabling strong interaction with the surrounding medium in the evanescent region. Combining laser-cooled atoms with nanofibers has enabled surprising quantum optics experiments, e.g. the efficient channeling of emission from single atoms into the fiber-guided modes, spectroscopy of near-surface atoms, high optical depth with an array of atoms optically trapped around the nanofiber, atomic memories and Bragg reflectors for fiber-guided photons, chiral light-matter interaction etc. In addition, using moderate longitudinal confinement in nanofiber cavities has enabled strong coupling between a single atom and fiber-guided photons. In this article, I review some of the key experimental demonstrations on the “atom＋nanofiber” platform.
Cold atomic ensembles offer precise tools for probing near-field interactions, yet experimental data linking atom dynamics to surface-induced forces remains limited. This study investigated the interaction between atoms and a dielectric surface using an atomic fountain measurement technique, in which cold rubidium atoms were released from a moving optical dipole trap. The launched cold atoms were irradiated with an evanescent light detuned from the D2_22​ transition by $-$20.2 to $+$20.2 MHz, after which they were recaptured by reactivating the optical dipole trap. Our measurements revealed that the number of recaptured atoms decreased with increasing flight time, and the decay was suppressed under blue-detuned conditions. We modeled the motion dynamics of the cold atomic ensemble, incorporating Casimir-Polder interactions between the dielectric surface and cold atoms, and observed that the rate of decrease in the number of residual atoms depended on the value of the van der Waals potential coefficient C3C_3C3​. The calculation results demonstrated good agreement with the experimental results, allowing us to estimate C3=5.6−1.9+2.4×10−49C_3 = 5.6^{+2.4}_{-1.9} \times 10^{-49}C3​=5.6−1.9+2.4​×10−49 Jm3^33 by comparing simulations with the experimental results across various C3C_3C3​ values, accounting for experimental errors.