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arXiv:quant-ph/0611084 · Physical Review A

Coherent control in a decoherence-free subspace of a collective multilevel system

Martin Kiffner, Jörg Evers, Christoph H. Keitel

Published Mar 12, 2007• 27 citations
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Abstract

Decoherence-free subspaces (DFS's) in systems of dipole-dipole interacting multilevel atoms are investigated theoretically. It is shown that the collective state space of two dipole-dipole interacting four-level atoms contains a four-dimensional DFS. We describe a method that allows us to populate the antisymmetric states of the DFS by means of a laser field, without the need for a field gradient between the two atoms. We identify these antisymmetric states as long-lived entangled states. Further, we show that any single-qubit operation between two states of the DFS can be induced by means of a microwave field. Typical operation times of these qubit rotations can be significantly shorter than for a nuclear spin system.

DOI
10.1103/physreva.75.032313

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Decoherence-free subspaces (DFS's) in systems of dipole-dipole interacting multilevel atoms are investigated theoretically. It is shown that the collective state space of two dipole-dipole interacting four-level atoms contains a four-dimensional DFS. We describe a method that allows us to populate the antisymmetric states of the DFS by means of a laser field, without the need for a field gradient between the two atoms. We identify these antisymmetric states as long-lived entangled states. Further, we show that any single-qubit operation between two states of the DFS can be induced by means of a microwave field. Typical operation times of these qubit rotations can be significantly shorter than for a nuclear spin system.
We propose schemes to design and control a time-dependent decoherence-free subspace (DFS) in a dissipative atom-cavity system. These schemes use atoms with three internal energy levels, which allows for the DFS to be multidimensional---a condition important for quantum sensing, simulation, and computation. We consider the use of tunable external driving lasers to transfer the system from a coherent spin state to a highly degenerate DFS. We find that the typical state in the DFS is highly entangled. Throughout evolution the state is kept in an instantaneous DFS, thereby allowing for pure states to be prepared. We develop adiabatic shortcuts to carry out this evolution with higher purity and fidelity than standard adiabatic and dissipative methods.
A scheme to drive and manipulate a finite-dimensional quantum system in decoherence-free subspaces (DFSs) by Lyapunov control is proposed. Control fields are established by the Lyapunov function. This proposal can drive the open quantum system into DFSs and manipulate it to any desired eigenstate of the free Hamiltonian. An example which consists of a four-level system with three long-lived states driven by two lasers is presented to demonstrate the scheme. We have performed numerical simulations of the dynamics of the four-level system, which show that the scheme works well.
Microscopic models based on multilevel atoms are central to optimizing nonlinear optical responses and the coherent control of light. These models are traditionally based on single-atom effects that are parametrically extrapolated to include collective effects, such as an enhanced response or propagation within atomic media. In this work, we present a systematic analysis of the cooperative effects arising in driven systems composed of multilevel atoms coupled via a common electromagnetic environment. The analysis is based on an interplay between dressed states induced by the driving field and photon exchanges, and collective decay channels. This theory is applied to the case of four-wave mixing induced by a pair of lasers acting on an atomic pair with internal levels in the diamond configuration. The effect of interatomic correlations and collective decay over the photons created in this nonlinear process is then explored. We identify three regions of operation: (i) laser-dominated, (ii) intermediate, and (iii) dipole-dominated. The dependence of single- and two-photon correlations is studied in detail for each region by varying atomic orientations and laser parameters consistent with current experiments involving atomic gases. Photonic correlation functions are shown to exhibit a transition from a Lorentz-like dependence on the two-photon detuning—with general features that can be obtained in an isolated atom scheme—to a two-peaked distribution when the dipole-dipole interactions become relevant. For weak Rabi frequencies whose value is smaller than the highest collective decay rate, the atoms are trapped inside their ground state as they approach each other. It is found that the anisotropy of the dipole-dipole interaction and its wave nature are essential to understand the behavior of the photon correlations. Signatures of these processes are identified for existing experimental realizations. The intuition obtained from this connection helps to uncover relevant parameters that could be exploited for quantum control protocols based on dispersive and dissipative cooperative effects in multilevel systems.
The cause of decoherence in a quantum system can be traced back to the interaction with the environment. As it has been pointed out by Dicke, in a system of N two-level atoms, where each of the atoms is individually dipole coupled to the environment, there are collective, subradiant states, that have no dipole coupling to photon modes, and therefore, they are expected to decay slower. This property also implies that these type of states decohere slower. We propose a scheme which will create such states. First, the two-level atoms are placed in a strongly detuned cavity and one of the atoms, called the control atom is excited. The time evolution of the coupled atom-cavity system leads to an appropriately entangled state of the atoms. By the aid of a suitable single-atom phase transformation, it is possible to drive the atomic state into the subradiant, i.e., decoherence-free subspace. Up to a certain average number of photons, the result is independent of the state of the cavity. The analysis of the conditions shows that this scheme is feasible with present day techniques achieved in atom-cavity interaction experiments.
Quantum interference and coherence effects in the interaction of atoms with the quantized electromagnetic field are investigated theoretically. A general master equation for the description of atom-field interactions is introduced. The interplay of the concepts of complementarity and interference in the time-energy domain are studied on the basis of the fluorescence light emitted by a single laser-driven atom, where the coherence of spontaneous processes gives rise to quantum interference in the spectrum of resonance fluorescence. The vacuum-induced dipole-dipole interaction in pairs of multi-level atoms is analyzed. It is shown that the interaction between orthogonal transition dipole moments of different atoms does not only influence the system dynamics crucially, but implies that the few-level approximation in general cannot be applied to near-degenerate Zeeman sublevels of the atomic level scheme. Potential applications of dipole-dipole interacting multi-level atoms for the implementation of decoherence-free subspaces and the generation of entanglement between atomic states are examined. The generation of an entangled state of the radiation field with a macroscopic number of photons is discussed on the basis of a single-atom laser.
We present a scheme to drive a finite-dimensional quantum system into the decoherence-free subspaces (DFS) by Lyapunov control. Control fields are established by Lyapunov function. This proposal works well for both closed and open quantum systems, with replacing the DFS by desired subspaces for closed systems. An example which consists of a four-level system with three degenerate states driven by three lasers is presented to gain further insight on the scheme. Numerical simulations for the dynamics of the system are performed and the results are good.