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arXiv:quant-ph/0604037 · Physical Review Letters

Universal Approach to Optimal Photon Storage in Atomic Media

Alexey Vyacheslavovich Gorshkov, Axel André, Michael Fleischhauer, Anders Søndberg Sørensen, Mikhail D. Lukin

Published Mar 19, 2007• 369 citations
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Abstract

We present a universal physical picture for describing storage and retrieval of photon wave packets in a Lambda-type atomic medium. This physical picture encompasses a variety of different approaches to pulse storage ranging from adiabatic reduction of the photon group velocity and pulse-propagation control via off-resonant Raman fields to photon-echo-based techniques. Furthermore, we derive an optimal control strategy for storage and retrieval of a photon wave packet of any given shape. All these approaches, when optimized, yield identical maximum efficiencies, which only depend on the optical depth of the medium.

DOI
10.1103/physrevlett.98.123601

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We present a universal physical picture for describing storage and retrieval of photon wave packets in a Lambda-type atomic medium. This physical picture encompasses a variety of different approaches to pulse storage ranging from adiabatic reduction of the photon group velocity and pulse-propagation control via off-resonant Raman fields to photon-echo-based techniques. Furthermore, we derive an optimal control strategy for storage and retrieval of a photon wave packet of any given shape. All these approaches, when optimized, yield identical maximum efficiencies, which only depend on the optical depth of the medium.
We derive an optimal control strategy for storage and retrieval of a photon wavepacket of any given shape in a Lambda-type atomic medium with a limited optical depth. The control is provided by an appropriately shaped classical laser field. We present a universal physical picture encompassing different pulse-storage techniques ranging from adiabatic reduction of the photon group velocity and pulse-propagation control via off-resonant Raman fields to photon-echo based approaches. When properly optimized, all three approaches yield identical maximum efficiencies, which only depend on the optical depth of the medium. Extending the model to include Doppler broadening, we find the surprising result that at high enough optical depth all atoms contribute coherently as if the medium were homogeneously broadened.
In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)], we presented a universal physical picture for describing a wide range of techniques for storage and retrieval of photon wave packets in $\ensuremath{\Lambda}$-type atomic media in free space, including the adiabatic reduction of the photon group velocity, pulse-propagation control via off-resonant Raman techniques, and photon-echo based techniques. This universal picture produced an optimal control strategy for photon storage and retrieval applicable to all approaches and yielded identical maximum efficiencies for all of them. In the present paper, we present the full details of this analysis as well some of its extensions, including the discussion of the effects of non-degeneracy of the two lower levels of the $\ensuremath{\Lambda}$ system. The analysis in the present paper is based on the intuition obtained from the study of photon storage in the cavity model in the preceding paper [Gorshkov et al., previous paper, Phys. Rev. A. 76, 033804 (2007)].
In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)], we used a universal physical picture to optimize and demonstrate equivalence between a wide range of techniques for storage and retrieval of photon wave packets in $\ensuremath{\Lambda}$-type atomic media in free space, including the adiabatic reduction of the photon group velocity, pulse-propagation control via off-resonant Raman techniques, and photon-echo-based techniques. In the present paper, we perform the same analysis for the cavity model. In particular, we show that the retrieval efficiency is equal to C∕(1+C)C∕(1+C)C∕(1+C) independent of the retrieval technique, where CCC is the cooperativity parameter. We also derive the optimal strategy for storage and, in particular, demonstrate that at any detuning one can store, with the optimal efficiency of C∕(1+C)C∕(1+C)C∕(1+C), any smooth input mode satisfying $TC\ensuremath{\gamma}⪢1$ and a certain class of resonant input modes satisfying $TC\ensuremath{\gamma}\ensuremath{\sim}1$, where TTT is the duration of the input mode and $2\ensuremath{\gamma}$ is the transition linewidth. In the two subsequent papers of the series, we present the full analysis of the free-space model and discuss the effects of inhomogeneous broadening on photon storage.
In a recent paper [Gorshkov et al., Phys. Rev. Lett. 98, 123601 (2007)] and in the two preceding papers [Gorshkov et al., this issue, Phys. Rev. A 76, 033804 (2006); 76, 033805 (2006)], we used a universal physical picture to optimize and demonstrate equivalence between a wide range of techniques for storage and retrieval of photon wave packets in homogeneously broadened $\ensuremath{\Lambda}$-type atomic media, including the adiabatic reduction of the photon group velocity, pulse-propagation control via off-resonant Raman techniques, and photon-echo-based techniques. In the present paper, we generalize this treatment to include inhomogeneous broadening. In particular, we consider the case of Doppler-broadened atoms and assume that there is a negligible difference between the Doppler shifts of the two optical transitions. In this situation, we show that, at high enough optical depth, all atoms contribute coherently to the storage process as if the medium were homogeneously broadened. We also discuss the effects of inhomogeneous broadening in solid state samples. In this context, we discuss the advantages and limitations of reversing the inhomogeneous broadening during the storage time, as well as suggest a way for achieving high efficiencies with a nonreversible inhomogeneous profile.
We show that there is no need for adiabatic passage in the storage and retrieval of information in the optically thick vapor of Lambda-type atoms. This information can be mapped into and retrieved out of long-lived atomic coherence with nearly perfect efficiency by strong writing and reading pulses with steep rising and falling edges. We elucidate similarities and differences between the ``adiabatic'' and ``instant'' light storage techniques, and conclude that for any switching time, an almost perfect information storage is possible if the group velocity of the signal pulse is much less than the speed of light in the vacuum c and the bandwidth of the signal pulse is much less then the width of the two-photon resonance. The maximum loss of the information appears in the case of instantaneous switching of the writing and reading fields compared with adiabatic switching, and is determined by the ratio of the initial group velocity of the signal pulse in the medium and speed of light in the vacuum c, which can be very small. Quantum restrictions to the storage efficiency are also discussed.