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arXiv:quant-ph/0602185 · Annals of Physics

On the assumption of initial factorization in the master equation for weakly coupled systems II: Solvable models

K. Yuasa, S. Tasaki, P. Facchi, G. Kimura, H. Nakazato, I. Ohba, S. Pascazio

Published Aug 10, 2006• 18 citations
arXivHTMLPDF
DOI
10.1016/j.aop.2006.06.003

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We analyze some solvable models of a quantum mechanical system in interaction with a reservoir when the initial state is not factorized. We apply Nakajima-Zwanzig's projection method by choosing a reference state of the reservoir endowed with the mixing property. In van Hove's limit, the dynamics is described in terms of a master equation. We observe that Markovianity becomes a valid approximation for timescales that depend both on the form factors of the interaction and on the observables of the reservoir that can be measured.
We consider the reduced dynamics of a small quantum system in interaction with a reservoir when the initial state is factorized. We present a rigorous derivation of a GKLS master equation in the weak-coupling limit for a generic bath, which is not assumed to have a bosonic or fermionic nature, and whose reference state is not necessarily thermal. The crucial assumption is a reservoir state endowed with a mixing property: the n-point connected correlation function of the interaction must be asymptotically bounded by the product of two-point functions (clustering property).
We investigate the effects of initial states on the dynamics of a quantum spin-boson model using an efficient variational polaron master equation approach. The transformation of a factorized system-environment initial state into the variational polaron frame introduces inhomogeneous terms in the master equation, essential for accurately describing non-Markovian dynamics beyond the weak coupling regime. To efficiently account for these effects, we formulate the dynamics in an extended auxiliary Liouville space, converting the resulting integro-differential equations into coupled ordinary differential equations. We further introduce a simplified variational polaron technique for computing the time evolution of expectation values of general observables, including those that do not commute with the polaron transformation, overcoming a major limitation of previous approaches and enabling the unified treatment of coherence and population dynamics. The effects of transformed initial states generated from arbitrary factorized initial states are systematically characterized through expectation values and trace-distance analysis, providing insight into the associated bath-relaxation dynamics over a broad range of tunneling amplitudes, temperatures, and coupling strengths. Comparison with the weak-coupling master equation reveals a delay phenomenon associated with multi-bath-quanta processes, pronounced at intermediate coupling strengths and tunneling amplitudes. We further show that coherent superposition initial states induce stronger nonequilibrium effects than localized states, with inhomogeneous terms playing a crucial role in the short-time dynamics. The proposed formalism applies to both undriven and resonantly driven spin-boson models, providing a computationally efficient framework for open quantum-system dynamics with arbitrary factorized initial states and general physical observables.