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arXiv:quant-ph/0510192 · Journal of the Optical Society of America B

Influence of a repump laser on a nearly degenerate four-wave-mixing spectrum in atomic vapors

Wei Jiang, Qun-feng Chen, Yongsheng Zhang, G.-C. Guo

Published Aug 1, 2006• 0 citations
arXivHTMLPDF

Abstract

The influence of a repump laser on a nearly degenerate four-wave-mixing (ND-FWM) spectrum was investigated. We found the amplitude and the line shape of the NDFWM depended strongly on the detuning of the repump field. A five-peak structure was observed, and at some certain repump detuning a dip appeared at the central peak. A rough analysis was proposed to explain this effect.

DOI
10.1364/josab.23.001615

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The influence of a repump laser on a nearly degenerate four-wave-mixing (ND-FWM) spectrum was investigated. We found the amplitude and the line shape of the NDFWM depended strongly on the detuning of the repump field. A five-peak structure was observed, and at some certain repump detuning a dip appeared at the central peak. A rough analysis was proposed to explain this effect.
Nearly degenerate four-wave mixing (NDFWM) in a traveling-wave semiconductor laser amplifier is demonstrated by simultaneously injecting two lights of slightly different frequencies in the same direction. A new frequency light at an expected frequency for NDFWM is observed with the same order of output as that of the injected light. The output power ratio of the three beams is strongly dependent on the sign of the frequency detuning. Theoretical analysis, in which the carrier rate equation is coupled with nonlinear Maxwell’s equations, explains the experimental results well. The observed behaviors are attributed to a unique third-order nonlinearity stemming from saturation-induced refractive index change in the semiconductor gain medium.
We have investigated degenerate four-wave mixing (DFWM) in a strongly absorbing molecular gas. A theory taking into account saturable absorption of the interacting beams is used to explain the dependence of the DFWM reflectivity on laser intensity and on the molecular number density. These parameters have a great influence on the observed spectra, owing to linear absorption that suppresses the DFWM signal in the line center of the molecular transitions. The great sensitivity of the spectra to the experimental conditions limits the applicability of DFWM for spectroscopic studies in absorbing media.
Degenerate four-wave mixing (DFWM) line shapes are investigated in sodium vapor near the D(2) resonance line using nearly Fourier-transform-limited pulses. At low pump intensities sub-Doppler resolution is obtained. When the Rabi frequency associated with the pump intensity becomes comparable with the ground-state hyperfine frequency separation of sodium, each component of the double-peaked DFWM spectrum splits further into two components. An adiabatic-following model explains the near-resonant intensity dependence of the DFWM signal. A qualitative explanation of the observed splitting is also given.
We present an experimental study of cw nearly degenerate four-wave-mixing emission in a Doppler broadened Rb atomic system. With the fixed detuning of an intense pump laser for the Rb D2{\mathit{D}}_{2}D2​ line, the nearly degenerate four-wave-mixing emission exhibits three peaks as a probe laser is scanned across the same Rb D2{\mathit{D}}_{2}D2​ line. The observed three-peaked spectrum can be interpreted as the resonances in the energy structure of the dressed atomic states.
Nearly degenerate four-wave mixing (NDFWM) within a closed degenerate two-level atomic transition is theoretically and experimentally examined. Using the model presented by Lezama et al. [Phys. Rev. A 61, 013801 (2000)] the NDFWM spectra corresponding to different pump and probe polarization cases are calculated and discussed. The calculated spectra are compared to the observation of NDFWM within the ${6S}_{1/2}(F=4)\ensuremath{\rightarrow}{6P}_{3/2}(F=5)$ transition of cesium in a phase conjugation experiment using magneto-optically cooled atoms.
We explore the use of degenerate four-wave-mixing (DFWM) intensity noise fluctuations as a spectroscopic tool for the study of atomic dynamics. Experimental results obtained from the spectral analysis of the intensity noise of the DFWM signal produced by a free running diode laser in a rubidium vapor cell are presented. For low exciting field intensities, the spectra are single peaked with a linewidth comparable to the atomic natural linewidth while at higher intensities a structure devleops revealing the existence of a dynamic Stark effect. The results are compared with numerical simulations of the power spectrum of the DFWM signal produced by a phase-diffusing field incident on two-level atoms.