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arXiv:quant-ph/0507046 · Physical Review A

Optimal focusing for maximal collection of entangled narrow-band photon pairs into single-mode fibers

Daniel Ljunggren, Maria Tengner

Published Dec 2, 2005• 108 citations
arXivHTMLPDF

Abstract

We present a theoretical and experimental investigation of the emission characteristics and the flux of photon pairs generated by spontaneous parametric downconversion in quasi-phase matched bulk crystals for the use in quantum communication sources. We show that, by careful design, one can attain well defined modes close to the fundamental mode of optical fibers and obtain high coupling efficiencies also for bulk crystals, these being more easily aligned than crystal waveguides. We distinguish between singles coupling, ${\ensuremath{\gamma}}_{\mathrm{s}}$ and ${\ensuremath{\gamma}}_{\mathrm{i}}$, conditional coincidence, ${\ensuremath{\mu}}_{\mathrm{i}\ensuremath{\mid}\mathrm{s}}$, and pair coupling, ${\ensuremath{\gamma}}_{\mathrm{c}}$, and show how each of these parameters can be maximized by varying the focusing of the pump mode and the fiber-matched modes using standard optical elements. Specifically we analyze a periodically poled KTP-crystal pumped by a $532\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ laser creating photon pairs at $810\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ and $1550\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$. Numerical calculations lead to coupling efficiencies above 93% at optimal focusing, which is found by the geometrical relation $L∕{z}_{R}$ to be $\ensuremath{\approx}1$ to 2 for the pump mode and $\ensuremath{\approx}2$ to 3 for the fiber-modes, where $L$ is the crystal length and ${z}_{R}$ is the Rayleigh-range of the mode-profile. These results are independent on $L$. By showing that the single-mode bandwidth decreases $\ensuremath{\propto}1∕L$, we can therefore design the source to produce and couple narrow bandwidth photon pairs well into the fibers. Smaller bandwidth means both less chromatic dispersion for long propagation distances in fibers, and that telecom Bragg gratings can be utilized to compensate for broadened photon packets---a vital problem for time-multiplexed qubits. Longer crystals also yield an increase in fiber photon flux $\ensuremath{\propto}\sqrt{L}$, and so, assuming correct focusing, we can only see advantages using long crystals.

DOI
10.1103/physreva.72.062301

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We report results regarding a source of polarization entangled photon pairs created by the process of spontaneous parametric downconversion in two orthogonally oriented, periodically poled, bulk KTiOPO4{\mathrm{KTiOPO}}_{4}KTiOPO4​ crystals. The source emits light colinearly at the nondegenerate wavelengths of 810 and 1550nm1550\phantom{\rule{0.3em}{0ex}}\mathrm{nm}1550nm, and is optimized for a single-mode optical fiber collection and long-distance quantum communication. The configuration favors long crystals, which promote a high photon-pair production rate at a narrow bandwidth, together with a high pair probability in fibers. The quality of entanglement is limited by chromatic dispersion, which we analyze by determining the output state. We find that such a decoherence effect is strongly material dependent, providing for long crystals an upper bound on the visibility of the coincidence fringes of 41% for KTiOPO4{\mathrm{KTiOPO}}_{4}KTiOPO4​, and zero for LiNbO3{\mathrm{LiNbO}}_{3}LiNbO3​. The best obtained raw visibility, when canceling decoherence with an extra piece of crystal, was $91\ifmmode\pm\else\textpm\fi{}0.2%$, including background counts. We confirm by a violation of the CHSH-inequality ($S=2.679\ifmmode\pm\else\textpm\fi{}0.004$ at $55\phantom{\rule{0.3em}{0ex}}{\mathrm{s}}^{\ensuremath{-}1∕2}$ standard deviations) and by complete quantum state tomography that the fibers carry high-quality entangled pairs at a maximum rate of $55\ifmmode\times\else\texttimes\fi{}{10}^{3}\phantom{\rule{0.3em}{0ex}}{\mathrm{s}}^{\ensuremath{-}1}\phantom{\rule{0.2em}{0ex}}{\mathrm{THz}}^{\ensuremath{-}1}\phantom{\rule{0.2em}{0ex}}{\mathrm{mW}}^{\ensuremath{-}1}$.
Entangled photon pairs play a crucial role in emerging quantum technologies, acting as tamper-proof padlocks in secure quantum communication, ultra-precise probes in quantum metrology and high-fidelity information carriers in photonic quantum computing. Amongst the many technological possibilities for generating photon pairs, sources based on spontaneous parametric down-conversion (SPDC) in second-order nonlinear crystals are still the workhorse tool in quantum optics laboratories, and more recently even in long-distance quantum communication with satellites. SPDC is a widely used method to create entangled photon pairs. The number of photon pairs that can be detected in a particular choice of collection modes, typically being optical single-mode fibers, depends critically on the spatial characteristics of the multi-mode SPDC emission as well as the particular beam waist of the collection modes. While several studies have already addressed the issue of optimal fiber coupling of SPDC photons in theory and experiment, the results of these studies arrive at different conclusions. Here, we present the results of a comprehensive experimental study on the optimal collection of photon pairs into single-mode optical fibers. Our approach is based on quasi-phase-matched type II SPDC from a periodically poled KTiOPO4 (ppKTP) crystal. We discuss the influence of pump and collection focal parameters on the spectral brightness and heralding efficiency, as well as practical issues of alignment tolerances into an optical single mode fiber. Further, Using two-photon interference (Hong-Ou-Mandel interference), we assess the spectral bandwidth of the photon pairs for variable crystal lengths. The results are in good agreement with our theoretical model, thus providing the recipe of building ultra bright and stable entangled photon sources.
We extend our earlier results of a bright source of non‐degenerate polarization entangled photon‐pairs by making a thorough theoretical and experimental investigation of its single‐mode emission and state‐decoherence. Using two perpendicular bulk crystals of periodically poled KTP, the source directly creates the polarization‐entangled state (|HH〉 + |VV〉)/√ with signal and idler wavelengths of 810 nm and 1550 nm, respectively. In order to optimize the coupling into single‐mode fiber we have developed a numerical algorithm which determines the emission mode and the fiber coupling efficiency for a given crystal length and focussing of the pump. For a 4.5 mm long crystal the optimal focussing of the pump is to a beam waist radius of 14 μm. With these focussing conditions the computer calculations give the lowest M2 value for the emission mode, M2 ≈ 3, and the best possible fiber coupling efficiency, γ ≈ 75%. Using the theoretical results to optimize our experimental setup we obtained photon count rates of 1.4 MHz singles and 12 kHz coincidences, and visibilities H, V: 99.6% and 45°: 94.2%.
A theoretical investigation of the performance of single-mode coupled spontaneous parametric downconversion sources is proposed, which only requires very few assumptions of practical interest: quasi-degenerate collinear generation and narrow bandwidth obtained through spectral filtering. Other assumptions, such as pump-beam spatial and temporal envelopes, target single-mode profile and size, and nonlinear susceptibility distribution, are only taken into account in the final step of the computation, thus making the theory general and flexible. Figures of merit for performance include absolute coupled brightness and conditional coupling efficiency. Their optimization is investigated using functions that only depend on dimensionless parameters, so that the results provide the best experimental configuration for a whole range of design choices (e.g., crystal length, pump power, etc.). A particular application of the theory is validated by an experimental optimization obtained under compatible assumptions. A comparison with other works and proposals for numerically implementing the theory under less stringent assumptions is also provided.
We present an ultrabright polarization-entangled photon source that is optimally coupled into single-mode fibers (SMFs). This study theoretically and experimentally examines the characteristics of spontaneous parametric down-conversion (SPDC) photons, including their spectrum, bandwidth, emission angle, and intensity, as functions of crystal length, temperature and beam waist condition. Notably, we measure the collinear spatial modes of photon-pairs and collection optics under various beam waist conditions and analyze them using a collinear Gaussian approximation model. By employing a simple mode-matching optical setup, we optimize the SMF coupling and heralding efficiencies of the photon-pairs. Consequently, we achieve a spectral brightness exceeding 2.0 MHz/mW/nm from a fiber-coupled entangled photon source, utilizing a 30-mm ppKTP crystal inside a polarization Sagnac interferometer. This represents the highest spectral brightness of SPDC photons generated using a CW laser pumped bulk crystal to date. Polarization entanglement was verified by a quantum state tomography and a polarization-correlation measurement. The fidelity of the entangled state is measured to be 97.8 % and the Bell-CHSH value S = 2.782 +- 0.04. The results obtained here provide practical insights for designing high-performance SPDC sources for satellite-based communication and long-distance optical links with extremely high-photon loss.