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arXiv:quant-ph/0506264 · Optics Letters

Quantum noise frequency correlations of multiply scattered light

Peter Lodahl

Published Jan 1, 2006• 12 citations
arXivHTMLPDF

Abstract

Frequency correlations in multiply scattered light that are present in quantum fluctuations are investigated. The speckle correlations for quantum and classical noise are compared and are found to depend markedly differently on optical frequency, which was confirmed in a recent experiment. Furthermore, novel mesoscopic correlations are predicted that depend on the photon statistics of the incoming light.

DOI
10.1364/ol.31.000110

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Frequency correlations in multiply scattered light that are present in quantum fluctuations are investigated. The speckle correlations for quantum and classical noise are compared and are found to depend markedly differently on optical frequency, which was confirmed in a recent experiment. Furthermore, novel mesoscopic correlations are predicted that depend on the photon statistics of the incoming light.
The paper presents the first experimental study of the propagation of quantum noise through an elastic, multiple scattering medium. Two different types of quantum noise measurements have been carried out: total transmission and short-range frequency correlations. When comparing shot noise (quantum) to technical noise (classical) a markedly different behavior is observed. The experimental results are found to be in agreement with a quantum model for multiple scattering of light, which allows extracting both static and dynamic scattering properties of the medium. A new quantum correlation in multiple scattering is proposed.
Multiple scattering is a very common phenomenon since it occurs any time a wave meets a disordered medium. As almost any natural object has random structure in one form or another, the variety of the processes involving multiple scattering spans from electronic transport in solids to propagation of sound in a forest. In principle, multiple scattering is completely deterministic, and in the absence of absorption also reversible, which means that the information encoded into the incident wave can be perfectly recovered. However, in practice, due to its extreme complexity we often consider this process to be random, which leads to information loss. Within this approach correlations can be an important instrument of information recovery, because they directly quantify the amount of knowledge we get about the wave in a particular point from the measurement performed in a different point. In the first part of this thesis we study a novel type of mesoscopic correlations between the light intensities at the opposite sides of an opaque scattering slab. We study its dependence on the scattering medium properties and the incoming light beam parameters. In the last chapter of the first part we show how this correlation can be used to retrieve non-invasively the information about the shape of an object placed behind the scattering medium. In the second part we switch to the quantum aspects of the light propagation inside the scattering materials. We show that certain class of quantum correlations, quantum discord, can be present in the multimode output state of the scattered light even when the input light is in a thermal state, which is commonly considered classical. We propose a non-classicality measure based on the strength of this correlation, applying it to characterize the advantage due to the quantum measurement in discrimination of two coherent states in their mixture.
We report the observation of speckle patterns in quantum correlations within light that is scattered by a disordered medium. The random medium is illuminated with spatially entangled photon pairs, and fourth-order speckle patterns are spatially resolved by two independently scanning detectors. Spatial entanglement gives two-photon speckle a much richer structure than ordinary one-photon speckle. Our experiments demonstrate that two-photon speckle from a surface scatterer and a volume scatterer look entirely different.
The irradiation of a dilute cloud of cold atoms with a coherent light field produces a random intensity distribution known as laser speckle. Its statistical fluctuations contain information about the mesoscopic scattering processes at work inside the disordered medium. Following up on earlier work by Assaf and Akkermans [Phys. Rev. Lett. 98, 083601 (2007)], we analyze how static speckle-intensity correlations are affected by an internal Zeeman degeneracy of the scattering atoms. It is proven on general grounds that the speckle correlations cannot exceed the standard Rayleigh law. On the contrary, because which-path information is stored in the internal atomic states, the intensity correlations suffer from strong decoherence and become exponentially small in the diffusive regime applicable to an optically thick cloud.
Understanding the complex interactions of the quantum light with different media provides valuable insights into potential applications in quantum tomography, microscopy, circuit and network design, and imaging. This thesis investigates quantum light interaction with two types of media: I. Random media entailing multiple scattering (Chapters 2-5), and II. Structured media, specifically designed to control quantum interferences (Chapters 6 and 7). In the first part of the thesis, and through solving the Lippmann-Schwinger equation for collections of small scatterers, a first principle scalar model for multiple scattering in finite-sized random media is developed. This efficient numerical model serves as the basis for investigating the coherent backscattering, a manifestation of weak localization in random media, for several bounded random media and various illuminations. Through employing mode expansion, next, the developed model is adapted to a general class of quantum-optical studies and quantum correlations are successfully derived and analyzed in scattering from finite disordered structures as well as systems of few scatterers. In multiple scattering of two-photon states in weak localization regime, the emergence of coherent two-photon backscattering is presented for the first time in coincidence detection, and it is demonstrated that quantum correlations can be used as a probe of entanglement dimensionality. Multiple scattering of two-photon states results in granular patterns known as speckle patterns. The statistical properties of single- and two-photon speckle patterns in scattering of different states are numerically calculated and the speckle visibilities and relevant parameters are derived. Specifically, the deviation of the probability density functions from negative exponential distributions, traditionally recognized as Rayleigh statistics in classical scattering, is identified, and shown to significantly depend on the presence of entanglement. Lastly, a different numerical implementation (based on COMSOL Multiphysics package) is used to consolidate our findings by incorporating the polarization effects. Coherent backscattering and coherent two-photon backscattering are observed for co-polarized fields in scattering from synthesized disordered media. It is demonstrated that depending on the particle exchange symmetry in polarization entangled excitation, the photons can exhibit statistical tendency to bunch together in the same mode, appear in separate modes (antibunching), or show a mixed response after multiple scattering. These bosonic-, fermionic-, and anyonic-like behaviors are studied in connection with coherent backscattering phenomenon, and it is demonstrated that the degree of enhancement in backscattering depends on the exchange symmetries. The simplicity and effectiveness of the implemented scattering analysis and the significance of the consequent conclusions suggest our approach as a promising platform for ‘numerical experiments’ without the limitations of analytical or semi-analytical models, and a practical tool prior to experiments. In the second part of the thesis, the random media operating as multimode platforms are replaced with engineered surfaces, i.e., metasurfaces, to realize targeted quantum interferences. First, a design roadmap for general lossy, asymmetric, and unbalanced coupling networks is presented, allowing to achieve maximum programmability in two-photon interferences. Next, two switchable metasurface-based coupling networks are designed to control nonclassical two-photon interferences via thermally driven crystallographic phase transitions. Numerical simulations confirm smooth transition between coalescence and anti-coalescence, aiming to address the current need in quantum optics for free-space compact devices creating tunable quantum interferences and acting as fast modulators for the second order quantum correlations. Our proposed compact and rapidly controllable devices pave the way towards new quantum applications as well as improving the current free-space quantum systems.