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arXiv:quant-ph/0503150 · Journal of Optics B Quantum and Semiclassical Optics

Controllability of multi-partite quantum systems and selective excitation of quantum dots

S. G. Schirmer, I. C. H. Pullen, A. I. Solomon

Published Sep 15, 2005• 18 citations
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Abstract

We consider the degrees of controllability of multi-partite quantum systems as well as necessary and sufficient criteria for each case. The results are applied to the problem of simultaneous control of an ensemble of quantum dots with a single laser pulse. Finally, we apply optimal control techniques to demonstrate selective excitation of individual dots for a simultaneously controllable ensemble.

DOI
10.1088/1464-4266/7/10/013

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We consider the degrees of controllability of multi-partite quantum systems as well as necessary and sufficient criteria for each case. The results are applied to the problem of simultaneous control of an ensemble of quantum dots with a single laser pulse. Finally, we apply optimal control techniques to demonstrate selective excitation of individual dots for a simultaneously controllable ensemble.
We investigate the problem of control of quantum systems. Various notions of controllability of quantum systems are discussed and Lie algebraic techniques are employed to derive necessary and sufficient conditions for the resulting degrees of controllability. The results are employed to study the degree of controllability for various model systems. The problem of optimal control is formulated as a problem of maximisation of the expectation value of an observable of the system subject to dynamical constraints and costs. A class of iterative algorithms is discussed, and shown to converge to a solution of the Euler-Lagrange equations, which is a necessary condition for optimality of a solution. A numerical realisation of the algorithm is presented and potential implementation of the resulting control fields in the laboratory is discussed. The algorithm is applied to find optimal control fields for a variety of applications including selective and simultaneous excitation of individual quantum dots in a globally addressed ensemble, creation of superposition states, and selective excitation of certain vibrational modes of a simple molecule such as Hydrogen Fluoride. In each case we systematically explore the parameter space of the algorithm to select solutions with desirable physical features from the multitude of possible choices. As there are many possible optimal control fields which give similar yields the question of whether some are more robust than others is investigated. A number of optimal fields are analysed quantitatively in terms of robustness with regard to temporal and spectral noise affecting the fields, uncertainty in the model parameters and the effect of experimental limitations such as restrictions on the bandwidth of the fields. It is shown that whilst the solutions tend to be sensitive to uncertainty in the energy levels chosen for the model, they appear to be surprisingly tolerant to even severe bandwidth limitations.
Abstract Semiconductor quantum dots are ideal candidates for quantum information applications in solid-state technology. However, advanced theoretical and experimental tools are required to coherently control, for example, the electronic charge in these systems. Here we demonstrate how quantum optimal control theory provides a powerful way to manipulate the electronic structure of coupled quantum dots with an extremely high fidelity. As alternative control fields we apply both laser pulses as well as electric gates, respectively. We focus on double and triple quantum dots containing a single electron or two electrons interacting via Coulomb repulsion. In the two-electron situation we also briefly demonstrate the challenges of timedependent density-functional theory within the adiabatic local-density approximation to produce comparable results with the numerically exact approach.
Full coherent control of quantum systems is a key prerequisite to build a quantum information processing (QIP) system. Spatially selective and ultrafast control of individual qubits in multi-qubit systems, on the other hand, optimally is based on all-optical control techniques using short laser pulses. However, these techniques require optically accessible quantum systems with suitable electronic level configurations to allow for the application of ultrafast and thus broadband pulses. Moreover, to enable good scalability, quantum systems in the solid state are generally preferred. So far, the only quantum systems in the solid state that match all these requirements are semiconductor quantum dots. However, to achieve a suitable level structure in these systems charged dots in strong magnetic fields have to be used.
Coherent single-electron control in a realistic semiconductor double quantum dot is studied theoretically. Using optimal-control theory, we show that the energy spectrum of a two-dimensional double quantum dot has a fully controllable transition line. We find that optimized picosecond laser pulses generate population transfer at significantly higher fidelities (>0.99)(>0.99)(>0.99) than conventional sinusoidal pulses. Finally, we design a robust and fast charge switch driven by optimal pulses that are within reach of terahertz laser technology.
We study the potential for optimal control of a symmetric double quantum-dot structure interacting with a single pulsed electromagnetic field. We first use the rotating wave and resonant approximations and reduce the dynamics of the system to that of a degenerate three-level $\ensuremath{\Lambda}$-type system. We also formulate the optimal control problem in terms of differential equations that have to be fulfilled by the optimal electromagnetic fields. We then obtain general analytical expressions for the optimal pulse shapes that lead to global maximization of the final population of the target state and of the time-averaged population of the target state in the quantum-dot structure.
We analyze the optically driven dynamics of a qubit implemented on a singlet-triplet subspace of two-electron states in a self-assembled quantum dot molecule. We study two possible control schemes based on the coupling to an excited (four-particle) state either by two spectrally separated laser pulses or by a single spectrally broad pulse. We quantitatively characterize the imperfections of the qubit operation resulting from nonadiabatic evolution and from limited spectral selectivity in a real system, as compared to the ideal adiabatic Raman transfer of occupation in the $\mathrm{\ensuremath{\Lambda}}$ system. Next, we study the effects of decoherence induced by the coupling to the phonons of the surrounding crystal lattice and by radiative recombination. As a result, we are able to identify the optimization trade-offs between different sources of errors and indicate the most favorable conditions for quantum control of the singlet-triplet qubit in the two optical control schemes.