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arXiv:quant-ph/0502135 · Physical Review Letters

Enhancing the Capacity and Performance of Collective Atomic Quantum Memory

Tomáš Opatrný, Jaromı́r Fiurášek

Published Jul 28, 2005• 14 citations
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Abstract

Present schemes involving the quantum non-demolition interaction between atomic samples and off-resonant light pulses allow us to store quantum information corresponding to a single harmonic oscillator (mode) in one multi-atomic system. We discuss the possibility of involving several coherences of each atom so that the atomic sample can store information contained in several quantum modes. This is achieved by the coupling of different magnetic sublevels of the relevant hyperfine level by additional Raman pulses. This technique allows us to design not only the quantum non-demolition coupling, but also beam splitter-like and two-mode squeezer-like interactions between light and collective atomic spin.

DOI
10.1103/physrevlett.95.053602

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•Jan 1, 2015•0 citations
Present schemes involving the quantum non-demolition interaction between atomic samples and off-resonant light pulses allow us to store quantum information corresponding to a single harmonic oscillator (mode) in one multi-atomic system. We discuss the possibility of involving several coherences of each atom so that the atomic sample can store information contained in several quantum modes. This is achieved by the coupling of different magnetic sublevels of the relevant hyperfine level by additional Raman pulses. This technique allows us to design not only the quantum non-demolition coupling, but also beam splitter-like and two-mode squeezer-like interactions between light and collective atomic spin.
A scheme for retrieving quantum information stored in collective atomic spin systems onto optical pulses is presented. Two off-resonant light pulses cross the atomic medium in two orthogonal directions and are interferometrically recombined in such a way that one of the outputs carries most of the information stored in the medium. In contrast to previous schemes our approach requires neither multiple passes through the medium nor feedback on the light after passing the sample, which makes the scheme very efficient. The price for that is some added noise which is, however, small enough for the method to beat the classical limits.
We report on the coherent and multi-temporal mode storage of light using the full atomic frequency comb memory scheme. The scheme involves the transfer of optical atomic excitations in Pr 3+ :Y 2 SiO 5 to spin waves in hyperfine levels using strong single-frequency transfer pulses. Using this scheme, a total of five temporal modes are stored and recalled on-demand from the memory. The coherence of the storage and retrieval is characterized using a time-bin interference measurement resulting in visibilities higher than 80%, independent of the storage time. This coherent and multimode spin-wave memory is promising as a quantum memory for light.
In this paper, an optical memory based on an ensemble of cold Cesium atoms interacting with light in the electromagnetically induced transparency (EIT) regime is studied in view of spatially multimode quantum storage. The interfacing protocol involves a control field, generating EIT for the very weak field that carries the quantum signal to be stored and enabling its mapping into the collective hyperfine coherence of the cold atomic ensemble. For the demonstration of multimode storage, the signal pulse at the single photon level is prepared in a mode with (OAM), while the control field is in a TEM00 mode. After the writing process, the information is kept in the memory register. In the retrieval phase, the information is read back from atoms to light and we show that these pulses at the single photon level with OAM can be stored and retrieved with a preserved spatial phase and a good efficiency.
We discuss theoretically quantum interface between light and a spin polarized ensemble of atoms with the spin $\ensuremath{\geqslant}1$ based on an off-resonant Raman scattering. We present the spectral theory of the light--atom interaction and show how particular spectral modes of quantum light couple to spatial modes of the extended atomic ensemble. We show how this interaction can be used for quantum memory storage and retrieval and for deterministic entanglement protocols. The proposed protocols are attractive due to their simplicity since they involve just a single pass of light through atoms without the need for elaborate pulse shaping or quantum feedback. As a practically relevant example we consider the interaction of a light pulse with hyperfine components of D1{D}_{1}D1​ line of 87Rb^{87}\mathrm{Rb}87Rb. The quality of the proposed protocols is verified via analytical and numerical analysis.
We study the coherent storage and retrieval of a very short multimode light pulse in an atomic ensemble. We consider a quantum memory process based on the conversion of a signal pulse into a long-lived spin coherence via light matter interaction in an on-resonant $\ensuremath{\Lambda}$ -type system. In order to study the writing and reading processes we analytically solve the partial differential equations describing the evolution of the field and of the atomic coherence in time as well as in space. We show how to optimize the process for writing as well as for reading. If the medium length is fixed, for each length, there is an optimal value of the pulse duration. We discuss the information capacity of this memory scheme and we estimate the number of transverse modes that can be stored as a quantum hologram.
This thesis presents progress towards two complementary goals. The first part discusses our aim of building high-efficiency quantum memories for quantum optical states and exploring the potential of the memory for performing operations as well as for passive storage. The second part presents our work towards developing a compact source of quantum light by fabricating optical resonators from non-linear optical crystals. Our high-efficiency memories operate by storing the information carried by a weak laser field in the coherence between the hyperfine-split electronic energy levels in a vapour of atomic rubidium. We analyse the performance of a three-level gradient echo memory protocol that is used to store and retrieve optical information from the atomic coherence using an off-resonant Raman transition. Using a warm rubidium vapour, we find that the memory preserves the quantum state of the input light better than any classical means of storage could achieve. We also present results showing that trapped, cold atomic vapours provide an increased storage lifetime and analyse the contribution that four-wave-mixing makes to the retrieved light. Both the warm- and cold-atom implementations of the memory are shown to store and recall light with over 80% efficiency. We also present a number of extensions to the basic memory protocol. We demonstrate that the light-atom coupling can be controlled by the bright coupling field that is used to complete the Raman transition. This control is used to perform a beam-splitting operations between two optical pulses that are separated in time. Using frequency-multiplexed states, we show that beam-splitting operations are also possible between optical modes that are separated in frequency. This operation can be extended to perform arbitrary operations by using a series of memories. Finally, we present a high-fidelity memory for dual-rail q-bits encoded across two frequency modes. The resonators that were fabricated to explore compact sources of quantum light demonstrated many of the properties that are required to obtain the stable operation of a quantum source. We demonstrated that non-linear optical crystals can be machined into monolithic resonators that use total internal reflections to confine light. Two geometries were tested, whispering gallery resonators and square travelling wave cavities. Because both types of resonators use total internal reflection instead of dielectric coatings, they feature very low loss rates. Lithium niobate resonators of both types exhibited cavity decay rates that were dominated by bulk absorption in the crystal. The resonators were shown to be frequency tunable using an applied voltage and could be coupled to free-space modes with a tunable coupling rate. We present preliminary results of non-linear frequency conversion in the resonators. We also investigated calcium fluoride and magnesium fluoride resonators for use as high-finesse reference cavities. We report a finesse of 5000 in a calcium fluoride whispering gallery resonator. A square calcium fluoride monolithic resonator was also produce to have a low insertion loss when coupled to a Gaussian free-space mode. We demonstrate a power coupling efficiency of 94% to that resonator. We also present a proposal to use a square lithium niobate resonator as a tunable coupler for a high-finesse calcium fluoride whispering gallery resonator. The coupled resonator system could be used as a compact high-efficiency optical quantum memory.