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arXiv:quant-ph/0410138 · Physical Review A

Crucial role of quantum entanglement in bulk properties of solids

Časlav Brukner, Vlatko Vedral, Anton Zeilinger

Published Jan 23, 2006• 138 citations
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Abstract

We demonstrate that two well-established experimental techniques of condensed-matter physics, neutron-diffraction scattering and measurement of magnetic susceptibility, can be used to detect and quantify macroscopic entanglement in solids. Specifically, magnetic susceptibility of copper nitrate (CN) measured in 1963 cannot be described without presence of entanglement. A detailed analysis of the spin correlations in CN as obtained from neutron-scattering experiment from 2000 provides microscopic support for this interpretation and gives the value for the amount of entanglement. We present a quantitative analysis resulting in the critical temperature of 5 K in both, completely independent, experiments below which entanglement exists.

DOI
10.1103/physreva.73.012110

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We demonstrate that two well-established experimental techniques of condensed-matter physics, neutron-diffraction scattering and measurement of magnetic susceptibility, can be used to detect and quantify macroscopic entanglement in solids. Specifically, magnetic susceptibility of copper nitrate (CN) measured in 1963 cannot be described without presence of entanglement. A detailed analysis of the spin correlations in CN as obtained from neutron-scattering experiment from 2000 provides microscopic support for this interpretation and gives the value for the amount of entanglement. We present a quantitative analysis resulting in the critical temperature of 5 K in both, completely independent, experiments below which entanglement exists.
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We study the macroscopic entanglement properties of a low-dimensional quantum spin system by investigating its magnetic properties at low temperatures and high magnetic fields. The spin system chosen for this is copper nitrate (Cu(NO 3 ) 2 × 2.5H 2 O), which is a spin chain that exhibits dimerization. The temperature and magnetic field dependence of entanglement from the susceptibility and magnetization data are given, by comparing the experimental results with the theoretical estimates. Extraction of entanglement has been made possible through the macroscopic witness operator, magnetic susceptibility. An explicit comparison of the experimental extraction of entanglement with theoretical estimates is provided. It was found that theory and experiments match over a wide range of temperatures and fields. The spin system studied exhibits quantum phase transition (QPT) at low temperatures when the magnetic field is swept through a critical value. We show explicitly for the first time, using tools used in quantum information processing, that QPT can be captured experimentally using quantum complementary observables, which clearly delineate entangled states from separable ones across the QPT. We have also estimated the partial information sharing in this system from our magnetization and susceptibility data. The complementarity relation has been experimentally verified to hold in this system.
Measuring quantum entanglement in solid state systems has been a long-standing challenge. Here, the authors use three entanglement witnesses borrowed from quantum information theory to directly detect quantum entanglement in the 1D Heisenberg spin chain system KCuF3{}_{3}3​ using inelastic neutron scattering data. The results are validated using density matrix renormalization group calculations and show that model-independent measures of quantum spin entanglement are experimentally possible, as well as reveal which witnesses are more experimentally robust.
We show how entanglement may be quantified in spin and cold atom many-body systems using standard experimental techniques only. The scheme requires no assumptions on the state in the laboratory, and a lower bound to the entanglement can be read off directly from the scattering cross section of neutrons deflected from solid state samples or the time-of-flight distribution of cold atoms in optical lattices, respectively. This removes a major obstacle which so far has prevented the direct and quantitative experimental study of genuine quantum correlations in many-body systems: The need for a full characterization of the state to quantify the entanglement contained in it. Instead, the scheme presented here relies solely on global measurements that are routinely performed and is versatile enough to accommodate systems and measurements different from the ones we exemplify in this work.
We show that magnetic susceptibility can reveal spin entanglement between individual constituents of a solid, while magnetization describes their local properties. We then show that magnetization and its variance (equivalent to magnetic susceptibility for a wide class of systems) satisfy complementary relation in the quantum-mechanical sense. It describes sharing of (quantum) information in the solid between spin entanglement and local properties of its individual constituents. Magnetic susceptibility is shown to be a macroscopic (thermodynamical) spin entanglement witness that can be applied without complete knowledge of the specific model (Hamiltonian) of the solid.
The lack of methods to experimentally detect and quantify entanglement in quantum matter impedes our ability to identify materials hosting highly entangled phases, such as quantum spin liquids. We thus investigate the feasibility of using inelastic neutron scattering (INS) to implement a model-independent measurement protocol for entanglement based on three entanglement witnesses: one-tangle, two-tangle, and quantum Fisher information (QFI). We perform high-resolution INS measurements on Cs_{2}CoCl_{4}, a close realization of the S=1/2 transverse-field XXZ spin chain, where we can control entanglement using the magnetic field, and compare with density-matrix renormalization group calculations for validation. The three witnesses allow us to infer entanglement properties and make deductions about the quantum state in the material. We find QFI to be a particularly robust experimental probe of entanglement, whereas the one and two-tangles require more careful analysis. Our results lay the foundation for a general entanglement detection protocol for quantum spin systems.