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arXiv:quant-ph/0409185 · Physical Review B

Effective boson-spin model for nuclei-ensemble-based universal quantum memory

Z. Song, Peng Zhang, Tao Shi, Chang-Pu Sun

Published May 25, 2005• 21 citations
arXivHTMLPDF

Abstract

We study the collective excitation of a macroscopic ensemble of polarized nuclei fixed in a quantum dot. Under the approximately homogeneous condition that we explicitly present in this paper, this many-particle system behaves as a single-mode boson interacting with the spin of a single conduction-band electron confined in this quantum dot. Within this effective spin-boson system, the quantum information carried by the electronic spin can be coherently transferred into the collective bosonic mode of excitation in the ensemble of nuclei. In this sense, the collective bosonic excitation can serve as a stable quantum memory to store the quantum spin information of the electron.

DOI
10.1103/physrevb.71.205314

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•Jan 1, 2015•0 citations
We study the collective excitation of a macroscopic ensemble of polarized nuclei fixed in a quantum dot. Under the approximately homogeneous condition that we explicitly present in this paper, this many-particle system behaves as a single-mode boson interacting with the spin of a single conduction-band electron confined in this quantum dot. Within this effective spin-boson system, the quantum information carried by the electronic spin can be coherently transferred into the collective bosonic mode of excitation in the ensemble of nuclei. In this sense, the collective bosonic excitation can serve as a stable quantum memory to store the quantum spin information of the electron.
Coupling a qubit coherently to an ensemble is the basis for collective quantum memories. A single driven electron in a quantum dot can deterministically excite low-energy collective modes of a nuclear spin ensemble in the presence of lattice strain. We propose to gate a quantum state transfer between this central electron and these low-energy excitations-spin waves-in the presence of a strong magnetic field, where the nuclear coherence time is long. We develop a microscopic theory capable of calculating the exact time evolution of the strained electron-nuclear system. With this, we evaluate the operation of quantum state storage and show that fidelities up to 90% can be reached with a modest nuclear polarization of only 50%. These findings demonstrate that strain-enabled nuclear spin waves are a highly suitable candidate for quantum memory.
Coherent excitation of an ensemble of quantum objects offers the opportunity to realise robust entanglement generation and information storage in a quantum memory [1]. Thus far, interfacing with such a collective excitation deterministically has remained elusive owing to the difficulty of controlling a probe spin in the midst of a complex many-body system. In the strained atomic lattice of a semiconductor quantum dot, nuclear quadrupole effects generate an electron-nuclear interaction that can be engineered by driving the electron spin (Fig. 1a). By implementing an all-optical approach to access the individual quantised electronic-nuclear spin transitions, we have experimentally demonstrated coherent optical rotations of a single collective nuclear spin excitation corresponding to a spin wave called a nuclear magnon [2] (Fig. 1b).
In this thesis we present protocols for the polarization of nuclear spins in a quantum dot via the hyperfine interaction with a conduction band electron and give a quantitative solution to the master equation we derive. The collective interference effects limiting the polarization are studied in detail, and ways of mitigating them are proposed. At high polarization levels the electron-nuclear interaction is approximated with simple and practical (quantum optical) models, suggesting the possibility of novel coherent manipulation schemes which actively make use of the nuclei. Finally we demonstrate that even completely mixed nuclear spin ensembles can be utilized for the important task of sequentially generating entanglement between electron spins.
We present a mechanism to protect quantum information stored in an ensemble of nuclear spins in a semiconductor quantum dot. When the dot is charged the nuclei interact with the spin of the excess electron through the hyperfine coupling. If this coupling is made off-resonant, it leads to an energy gap between the collective storage states and all other states. We show that the energy gap protects the quantum memory from local spin-flip and spin-dephasing noise. Effects of nonperfect initial spin polarization and inhomogeneous hyperfine coupling are discussed.
We propose a solid state based protocol to implement the universal quantum storage for electronic spin qubit. The quantum memory in this scheme is the spin wave excitation in the ring array of nuclei in a quantum dot. We show that the quantum information carried by an arbitrary state of the electronic spin can be coherently mapped onto the spin wave excitations or the magnon states. With an appropriate external control, the stored quantum state in quantum memory can be read out reversibly. We also explore in detail the quantum decoherence mechanism due to the inhomogeneous couplings between the electronic spin and the nuclear spins.
Electron spins confined in quantum dots (QDs) are among the leading contenders for implementing quantum information processing. In this Thesis we address two of the most significant technological challenges towards developing a scalable quantum information processor based on spins in quantum dots: (i) decoherence of the electronic spin qubit due to the surrounding nuclear spin bath, and (ii) long-range spin-spin coupling between remote qubits. To this end, we develop novel strategies that turn the unavoidable coupling to the solid-state environment (in particular, nuclear spins and phonons) into a valuable asset rather than a liability. In the first part of this Thesis, we investigate electron transport through single and double QDs, with the aim of harnessing the (dissipative) coupling to the electronic degrees of freedom for the creation of coherence in both the transient and steady-state behaviour of the ambient nuclear spins. First, we theoretically show that intriguing features of coherent many-body physics can be observed in electron transport through a single QD. To this end, we first develop a master-equation-based formalism for electron transport in the Coulomb-blockade regime assisted by hyperfine (HF) interaction with the nuclear spin ensemble in the QD. This general tool is then used to study the leakage current through a single QD in a transport setting. When starting from an initially uncorrelated, highly polarized state, the nuclear system experiences a strong correlation buildup, due to the collective nature of the coupling to the central electron spin. We demonstrate that this results in a sudden intensity burst in the electronic tunneling current emitted from the QD system, which exceeds the maximal current of a corresponding classical system by several orders of magnitude. This gives rise to the new paradigm of electronic superradiance. Second, building upon the insight that the nuclear spin dynamics are governed by collective interactions giving rise to coherent effects such as superradiance, we propose a scheme for the deterministic generation of steady-state entanglement between the two nuclear spin ensembles in an electrically defined double quantum dot. Because of quantum interference in the collective coupling to the electronic degrees of freedom, the nuclear system is actively driven into a two-mode squeezedlike target state. The entanglement buildup is accompanied by a self-polarization of the nuclear spins towards large Overhauser field gradients. Moreover, the feedback between the electronic and nuclear dynamics is shown to lead to intriguing effects such as multistability and criticality in the steady-state solutions. In the second part of this Thesis, our focus turns towards the realization of long-range spin-spin coupling between remote qubits. We propose a universal, on-chip quantum transducer based on surface acoustic waves in piezo-active materials. Because of the intrinsic piezoelectric (and/or magnetostrictive) properties of the material, our approach provides a universal platform capable of coherently linking a broad array of qubits, including quantum dots, trapped ions, nitrogen-vacancy centers or superconducting qubits. The quantized modes of surface acoustic waves lie in the gigahertz range, can be strongly confined close to the surface in phononic cavities and guided in acoustic waveguides. We show that this type of surface acoustic excitations can be utilized efficiently as a quantum bus, serving as an on-chip, mechanical cavity-QED equivalent of microwave photons and enabling long-range coupling of a wide range of qubits. In summary, this thesis provides contributions towards developing a scalable quantum information processor based on spins in quantum dots in two different aspects. The first part is dedicated to a deeper understanding of the nuclear spin dynamics in quantum dots. In the second part we put forward a novel sound-based strategy to realize long-range spin-spin coupling between remote qubits. This completes a broad picture of spin-based quantum information processing which integrates different perspectives, ranging from the single-qubit level to a broader quantum network level.