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arXiv:quant-ph/0409003 · Journal of Modern Optics

Causality in propagation of a pulse in a nonlinear dispersive medium

G. S. Agarwal, Tarak Nath Dey

Published Jul 10, 2005• 5 citations
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Abstract

We investigate the causal propagation of the pulse through dispersive media by very precise numerical solution of the coupled Maxwell–Bloch equations without any approximations about the strength of the input field. We study full nonlinear behaviour of the pulse propagation through solid state media like ruby and alexandrite. We have demonstrated that the information carried by the discontinuity, i.e. front of the pulse, moves inside the media with velocity c even though the peak of the pulse can travel either with sub-luminal or with super-luminal velocity. Our numerical demonstration is subject to the condition that the background refractive index of the medium is unity. We extend the argument of Levi-Civita to prove that the discontinuity would travel with velocity c even in a nonlinear medium.

DOI
10.1080/09500340500052572

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We investigate the causal propagation of the pulse through dispersive media by very precise numerical solution of the coupled Maxwell–Bloch equations without any approximations about the strength of the input field. We study full nonlinear behaviour of the pulse propagation through solid state media like ruby and alexandrite. We have demonstrated that the information carried by the discontinuity, i.e. front of the pulse, moves inside the media with velocity c even though the peak of the pulse can travel either with sub-luminal or with super-luminal velocity. Our numerical demonstration is subject to the condition that the background refractive index of the medium is unity. We extend the argument of Levi-Civita to prove that the discontinuity would travel with velocity c even in a nonlinear medium.
The propagation of an optical pulse through a system of two-level atoms embedded in a host medium of constant refractive index n is considered. It is shown that the values of the solutions of the nonlinear system of coupled Maxwell and Schrödinger equations at time t at a point z, in the McCall-Hahn approximation, depend only on data contained in the interval [z - c/nt, z] at t = 0. Thus, information cannot be transmitted through this medium with velocity greater than c/n. Apparent violations of this property in the case of self-induced transparency are explained.
In a causally dispersive medium the signal arrival appears in the dynamical field evolution as an increase in the field amplitude from that of the precursor fields to that of the steady-state signal. The interrelated effects of phase dispersion and frequency dependent attenuation and/or amplification alter the pulse in such a fundamental way that results in the appearance of precursor fields. Although superluminal group velocities have been found in various dispersive media, the pulse "front" and associated precursors will never travel faster than c , and hence these are the vehicles through which relativistic causality is preserved. While many rigorous studies of wave propagation and associated abnormal group velocities in passive Lorentzian media have been performed, the corresponding problem in active media has remained theoretically unexplored. This problem is addressed in the present paper, by employing the steepest descent method for the determination of the response of an active Lorentzian medium to a step modulated pulse. The steepest descent method provides a detailed description of the propagation of the pulse inside the dispersive medium in the time domain. Moreover, the evolution of the saddle points illuminates the relation between the medium parameters and the temporal evolution of the propagating pulse within the medium. Hence, useful physical insights are obtained and the interesting differences between the passive and active case are deduced.
The propagation of pulses through dispersive media was investigated by solving Maxwell's equations without any approximation. We show that the superluminal propagation of pulses through anomalous dispersive media is a result of the interference of different frequency components composed of the pulse. The coherence of the pulse plays an important role for the superluminal propagation. With the decrease of the coherence of the pulse, the propagation changes from superluminal to subluminal. We have shown that the anomalous dispersion (the real part of the susceptibility) not the amplification (the imaginary part of the susceptibility) plays the essential role in the superluminal propagation. Although the superluminality always exists as long as the spectrum of the coherent pulse is within the anomalously dispersive region, both the energy propagation velocity and the frontal velocity never exceed the light speed in the vacuum. The output pulse through the medium is not the original pulse; instead it carries the information of the original pulse and the information of the prepared medium.
Subluminal and superluminal propagation of a light pulse in Kerr materials has been investigated. Group velocities as slow as much less than 1 mm per second to as fast as negative several thousands meters per second can easily be obtained in the Kerr medium, which possesses a large nonlinear refractive index and long relaxation time, such as Cr3+-doped alexandrite, ruby, and GdAlO3. The physical mechanism is the strong highly dispersive coupling between different frequency components of the pulse.
We investigate a light-pulse propagation with negative group velocity in a nonlinear coherent medium. We show that the necessary conditions for nonlinear superluminal effects to be observable are realized in a three-level $\ensuremath{\Lambda}$ system interacting with a linearly polarized laser field in the presence of a static magnetic field. The initially prepared Zeeman coherence cancels the resonant absorption of the medium almost completely, but preserves its dispersion anomalous and very high. In this medium the light pulse propagates superluminally in the sense that the peak of the transmitted pulse exits the medium before the peak of the incident pulse enters. At the same time the pulse group velocity is intensity dependent, which leads to the self-steepening of the pulse trailing edge due to the fact that the more intense parts of the pulse travel slower. This is in contrast with the shock wave generation in a nonlinear medium with normal dispersion. The predicted effect can be easily observed in the well-known schemes employed in the studies of nonlinear magneto-optical rotation. The upper bound of sample length is found from the criterion that the pulse self-steepening and group-advance time are observable without pulse distortion caused by the group-velocity dispersion.
We develop models for the propagation of intense pulses in solid state media which can have either saturated absorption or reverse absorption. We model subluminal propagation in ruby and superluminal propagation in alexandrite as three and four level systems, respectively, coupled to Maxwell's equations. We present results well beyond the traditional pump-probe approach and explain the experiments of Bigelow et al. [Phys. Rev. Lett. 90, 113903 (2003)]Science 301, 200 (2003)]] on solid state materials.