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arXiv:quant-ph/0406040

Macroscopic Thermodynamical Witnesses of Quantum Entanglement

Časlav Brukner, Vlatko Vedral

Published Jun 7, 2004• 15 citations
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Abstract

We show that macroscopic thermodynamical properties - such as functions of internal energy and magnetization - can detect quantum entanglement in solids at nonzero temperatures in the thermodynamical limit. We identify the parameter regions (critical values of magnetic field and temperature) within which entanglement is witnessed by these thermodynamical quantities.

DOI
10.48550/arxiv.quant-ph/0406040

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We show that macroscopic thermodynamical properties - such as functions of internal energy and magnetization - can detect quantum entanglement in solids at nonzero temperatures in the thermodynamical limit. We identify the parameter regions (critical values of magnetic field and temperature) within which entanglement is witnessed by these thermodynamical quantities.
We show that, when measured along orthogonal spatial directions, magnetic susceptibility can reveal entanglement between individual constituents of a solid, while magnetisation describes their local properties. We then show that these two thermodynamical quantities satisfy complementary relation in the quantum-mechanical sense. It describes sharing of (quantum) information in the solid between entanglement and local properties of its individual constituents. Magnetic susceptibility is shown to be universal macroscopic entanglement witness that can be applied independently of the model of the solid (without the knowledge of its Hamiltonian).
We show that magnetic susceptibility can reveal spin entanglement between individual constituents of a solid, while magnetization describes their local properties. We then show that magnetization and its variance (equivalent to magnetic susceptibility for a wide class of systems) satisfy complementary relation in the quantum-mechanical sense. It describes sharing of (quantum) information in the solid between spin entanglement and local properties of its individual constituents. Magnetic susceptibility is shown to be a macroscopic (thermodynamical) spin entanglement witness that can be applied without complete knowledge of the specific model (Hamiltonian) of the solid.
We present a general argument showing that the temperature as well as other thermodynamical state variables can qualify as entanglement witnesses (EWs) for spatial entanglement. This holds for a variety of systems and we exemplify our ideas using a simple free non-interacting bosonic gas. We find that entanglement can exist at arbitrarily high temperatures, provided that we can probe smaller and smaller regions of space. We then discuss the relationship between the occurrence of Bose–Einstein condensation and our conditions for the presence of entanglement and compare the respective critical temperatures. We close with a short discussion of the idea of seeing entanglement as a macroscopic property in thermodynamical systems and its possible relation to phase transitions in general.
This paper summarises the results of our research on macroscopic entanglement in spin systems and free Bosonic gases. We explain how entanglement can be observed using entanglement witnesses which are themselves constructed within the framework of thermodynamics and thus macroscopic observables. These thermodynamical entanglement witnesses result in bounds on macroscopic parameters of the system, such as the temperature, the energy or the susceptibility, below which entanglement must be present. The derived bounds indicate a relationship between the occurrence of entanglement and the establishment of order, possibly resulting in phase transition phenomena. We give a short overview over the concepts developed in condensed matter physics to capture the characteristics of phase transitions in particular in terms of order and correlation functions. Finally we want to ask and speculate whether entanglement could be a generalised order concept by itself, relevant in (quantum induced) phase transitions such as BEC, and that taking this view may help us to understand the underlying process of high-T superconductivity.
This paper summarises the results of our research on macroscopic entanglement in spin systems and free Bosonic gases. We explain how entanglement can be observed using entanglement witnesses which are themselves constructed within the framework of thermodynamics and thus macroscopic observables. These thermodynamical entanglement witnesses result in bounds on macroscopic parameters of the system, such as the temperature, the energy or the susceptibility, below which entanglement must be present. The derived bounds indicate a relationship between the occurrence of entanglement and the establishment of order, possibly resulting in phase transition phenomena. We give a short overview over the concepts developed in condensed matter physics to capture the characteristics of phase transitions in particular in terms of order and correlation functions. Finally we want to ask and speculate whether entanglement could be a generalised order concept by itself, relevant in (quantum induced) phase transitions such as BEC, and that taking this view may help us to understand the underlying process of high-T superconductivity.
Entanglement between individual spins can be detected by using thermodynamics quantities as entanglement witnesses. This applies to collective spins also, provided that their internal degrees of freedom are frozen, as in the limit of weakly coupled nanomagnets. Here, we extend such approach to the detection of entanglement between subsystems of a spin cluster, beyond such weak-coupling limit. The resulting inequalities are violated in spin clusters with different geometries, thus allowing the detection of zero- and finite-temperature entanglement. Under relevant and experimentally verifiable conditions, all the required expectation values can be traced back to correlation functions of individual spins, which are now made selectively available by four-dimensional inelastic neutron scattering.