We demonstrate how spontaneous emission in a cavity can be controlled by the application of a dc field. The method is especially suitable for Rydberg atoms. We present a simple argument based on Stark shifts for the control of emission.
Abstract : Spontaneous emission of an atom is not an immutable property of an atom but can be controlled by modification of the vacuum field fluctuations surrounding the atom. In fact, inhibition and enhancement of spontaneous emission of atoms both at microwave and optical frequencies have been demonstrated experimentally. It has, also, been demonstrated that spontaneous emission from GaAs quantum wells (QWs) is altered by embedding the QWs between AlAs/AlGaAs distributed Bragg reflectors (DBRs). Such an artificial modification of the spontaneous emission in semiconductor micro-structures is very important, particularly from device use point of view. We may, also expect enhancement and inhibition of spontaneous emission induced by tuning of emission wavelength of atoms or active materials embedded in fixed micro-cavities, instead of variation of micro-cavity structures. In this paper, we demonstrate, for the first time, controllable enhancement and inhibition of excitonic spontaneous emission by dc electric fields applied to a GaAs QW embedded in a pair of AlAs/AlGaAs DBRs.
It is well known that spontaneous emission is not an intrinsic atomic property, but rather results from the coupling of the atom to the vacuum modes of the electromagnetic field. As such, it can be modified by tailoring the electromagnetic environment into which the atom can radiate. This was already realized by Purcell, who noted that the spontaneous emission rate can be enhanced if the atom placed inside a cavity is resonant with one of the cavity is resonant with one of the cavity modes, and by Kleppner, who discussed the opposite case of inhibited spontaneous emission. It has also been recognized that spontaneous emission need not be an irreversible process. Indeed, a system consisting of a single atom coupled to a single mode of the electromagnetic field undergoes a periodic exchange of excitation between the atom and the field. This periodic exchange remains dominant as long as the strength of the coupling between the atom and a cavity mode is itself dominant. 23 refs., 6 figs.
Spontaneous emission from an excited atomic state reflects the properties of the surrounding vacuum field. By placing the atom near a metallic surface or in a cavity, one can modify the spectral density of the vacuum modes coupled to it and either enhance1 or inhibit2 spontaneous emission. Large enhancement3 or inhibition effects have been obtained recently in microwave experiments involving either Rydberg atoms4 or a trapped electron5 radiating in cavities whose sizes were of the order of one-tenth of a millimeter to a centimeter.
It has been observed that the spontaneous-emission lifetime of Rydberg atoms is shortened by a large ratio when these atoms are crossing a high-Q superconducting cavity tuned to resonance with a millimeter-wave transition between adjacent Rydberg states.