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arXiv:quant-ph/0312180 · Chinese Physics Letters

Two-Qubit Quantum Logic Gate in Molecular Magnets

Jing-Min Hou, Li-Jun Tian, Mo‐Lin Ge

Published Aug 25, 2005• 7 citations
arXivHTMLPDF

Abstract

We propose a scheme to realize a controlled-NOT quantum logic gate in a dimer of exchange coupled single-molecule magnets, [Mn 4 ] 2 . We chosen the ground state and the three low-lying excited states of a dimer in a finite longitudinal magnetic field as the quantum computing bases and introduced a pulsed transverse magnetic field with a special frequency. The pulsed transverse magnetic field induces the transitions between the quantum computing bases so as to realize a controlled-NOT quantum logic gate. The transition rates between a pair of the four quantum computing bases and between the quantum computing bases and excited states are evaluated and analysed.

DOI
10.1088/0256-307x/22/9/002

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We propose a scheme to realize a controlled-NOT quantum logic gate in a dimer of exchange coupled single-molecule magnets, [Mn 4 ] 2 . We chosen the ground state and the three low-lying excited states of a dimer in a finite longitudinal magnetic field as the quantum computing bases and introduced a pulsed transverse magnetic field with a special frequency. The pulsed transverse magnetic field induces the transitions between the quantum computing bases so as to realize a controlled-NOT quantum logic gate. The transition rates between a pair of the four quantum computing bases and between the quantum computing bases and excited states are evaluated and analysed.
We study the low energy states of one-dimensional spin chain clusters consisting of three spin-1/2 Heisenberg particles. When applying an external magnetic field on the spin chain cluster, the ground state doublet will generate Zeeman splitting. As a two-level quantum system, the split ground state doublet can be defined as a new 'spin cluster qubit'. The cluster quibit is shown to be more robust with a smaller decoherence rate. We realize universal single-qubit gates with the algebraic dynamical method, by applying a time-dependent magnetic field on the spin cluster. We also investigate a two-qubit system made up of two such Heisenberg spin chain clusters which interact through a tunable Heisenberg coupling. In the two-qubit product basis, the controlled quantum phase gates can be generated by applying a magnetic field along the z-axis on the system of the two clusters. One can realize the controlled-NOT gate through a three-step time evolution by adjusting the corresponding physical parameters. Our scheme involves two kinds of dynamically distinct operations, which is much simpler and more feasible.
We propose a method that implements a universal set of one- and two-quantum-bit gates for quantum computation in a system of coupled electron pairs with constant non-diagonal exchange interaction. In our proposal, suppression of the exchange interaction is performed by the continual repetition of single-spin rotations. A small g-factor difference between the electrons allows for addressing qubits and avoiding strong magnetic field pulses. Numerical experiments were performed to show that, to implement the one- and two-qubit operations, it is sufficient to change the strength of the magnetic field by a few Gauss. This introduces one and then the other electron in a resonance. To determine the evolution of the two-qubit system, we use the algorithms of optimal control theory.
Using high-level ab initio many-body theory, we theoretically propose that the Dy and the Ni atoms in the [Dy 2 Ni 2 (L) 4 (NO 3 ) 2 (DMF) 2 ] real molecular magnet as well as in its core, that is, the [Dy 2 Ni 2 O 6 ] system, act as two-level qubit systems. Despite their spatial proximity we can individually control each qubit in this highly correlated real magnetic system through specially designed laser-pulse combinations. This allows us to prepare any desired two-qubit state and to build several classical and quantum logic gates, such as the two-qubit (binary) CNOT gate with three distinct laser pulses. Other quantum logic gates include the single-qubit (unary) quantum X, Y, and Z Pauli gates; the Hadamard gate (which necessitates the coherent quantum superposition of two many-body electronic states); and the SWAP gate (which plays an important role in Shor’s algorithm for integer factorization). Finally, by sequentially using the achieved CNOT and Hadamard gates we are able to obtain the maximally entangled Bell states, for example, ( 1 2 )(|00⟩ + |11⟩).
It is shown theoretically that by the use of two radio-frequency fields of the same resonance frequency but with the different phases and directions the degeneracy of the energy spectrum of a spin system with I = 3/2 is removed. This leads to four non-degenerate spin states which can be used as a platform for quantum computing. The feasibility of quantum computing based on a pure (without DC magnetic fields) nuclear quadrupole resonance technique is investigated in detail. Various quantum logic gates can be constructed by using different excitation techniques allowing different manipulations with the spin system states. Three realizations of quantum logic gates are considered: the application of an additional magnetic field with the resonance frequency, the amplitude modulation of one of the applied RF fields by the resonance frequency field, and the level-crossing method. It is shown that the probabilities of the resonance transitions depend on the method of excitation and on the direction of the excitation field. Feasibility of quantum computing is demonstrated with the examples of constructing a controlled-NOT logic gate using the resonance excitation technique and SWAP and NOT2 logic gates using the level-crossing method.
Abstract We studied the dynamics of a pair of single-electron double quantum dots (DQDs) under longitudinal and transverse static magnetic fields and time-dependent harmonic modulation of their interaction couplings. We propose to modulate the tunnel coupling between the QDs to produce one-qubit gates and the exchange coupling between DQDs to generate entangling gates, the set of operations required for quantum computing. We developed analytical approximations to set the conditions to control the qubits and applied them to numerical calculations to test the accuracy and robustness of the analytical model. The results shows that the unitary evolution of the two-electron state performs the designed operations even under conditions shifted from the ideal ones.
In NMR quantum computing, spin states of spin-1/2 nuclei are called qubits. Quantum logic gates are represented by unitary matrices. As a universal gate, controlled-NOT (CNOT) is a two-qubit gate. For the IS (I = 1/2 and S = 1/2) spin system, two-qubit CNOT gate is represented by a 4 × 4 matrix. SWAP logic gate, which exchanges two quantum states, is constructed by CNOT gates. In this study, first, four-qubit CNOT gates are constructed for the IS (I = 3/2, S = 3/2) spin system. Then, by using these CNOT gates, a four-qubit SWAP logic gate is found. As an application and verification, an obtained SWAP logic gate is applied to the matrix representation of product operators for the IS (I = 3/2, S = 3/2) spin system. SWAP logic gate can also be presented by an NMR pulse sequence. By using the product operator theory, the pulse sequence of the SWAP logic gate is applied to product operators of the IS (I = 3/2, S = 3/2) spin system. The expected exchange results are obtained for both the matrix representation and the pulse sequence of SWAP logic gate.