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arXiv:quant-ph/0309058 · Physical Review A

Tailoring photonic entanglement in high-dimensional Hilbert spaces

Hugues de Riedmatten, I. Marcikic, Valerio Scarani, Wolfgang Tittel, Hugo Zbinden, Nicolas Gisin

Published May 18, 2004• 114 citations
arXivHTMLPDF

Abstract

We present an experiment where two photonic systems of arbitrary dimensions can be entangled. The method is based on spontaneous parametric down-conversion with trains of $d$ pump pulses with a fixed phase relation, generated by a mode-locked laser. This leads to a photon pair created in a coherent superposition of $d$ discrete emission times, given by the successive laser pulses. Entanglement is shown by performing a two-photon interference experiment and by observing the visibility of the interference fringes increasing as a function of the dimension $d$. Factors limiting the visibility, such as the presence of multiple pairs in one train, are discussed.

DOI
10.1103/physreva.69.050304

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We present an experiment where two photonic systems of arbitrary dimensions can be entangled. The method is based on spontaneous parametric down-conversion with trains of ddd pump pulses with a fixed phase relation, generated by a mode-locked laser. This leads to a photon pair created in a coherent superposition of ddd discrete emission times, given by the successive laser pulses. Entanglement is shown by performing a two-photon interference experiment and by observing the visibility of the interference fringes increasing as a function of the dimension ddd. Factors limiting the visibility, such as the presence of multiple pairs in one train, are discussed.
We present a new scheme to generate high dimensional entanglement between two photonic systems. The idea is based on parametric down conversion with a sequence of pump pulses generated by a mode-locked laser. We prove experimentally the feasibility of this scheme by performing a Franson-type Bell test using a 2-way interferometer with path-length difference equal to the distance between 2 pump pulses. With this experiment, we can demonstrate entanglement for a two-photon state of at least dimension D=11. Finally, we propose a feasible experiment to show a Fabry-Perot like effect for a high dimensional two-photon state.
We present a new scheme to generate high dimensional entanglement between two photonic systems. The idea is based on parametric down conversion with a sequence of pump pulses generated by a mode-locked laser. We prove experimentally the feasibility of this scheme by performing a Franson-type Bell test using a 2-way interferometer with path-length difference equal to the distance between 2 pump pulses. With this experiment, we can demonstrate entanglement for a two-photon state of at least dimension d=11. Finally, we propose a feasible experiment to show a Fabry-Perot like effect for a high dimensional two-photon state.
Two spatially separated type-I nonlinear crystals are pumped by femtosecond laser pulses to create entangled photon pairs in the process of spontaneous parametric down-conversion. The two-photon entangled state exhibits high-visibility quantum interference for both polarization and space-time variables without the need of stringent spectral postselection by using narrow-band filters. The visibility is insensitive to the thickness of the crystals, unlike in the case of pulse pumped type-II parametric down-conversion; therefore the intensity can be easily increased by using thick nonlinear crystals. This method will be indispensable in experiments that require a pulsed source of entangled photon pairs, such as generation of multiphoton entangled states, quantum teleportation, and quantum communications.
Multi-particle entangled states are becoming more and more interesting for different applications in quantum information, such as quantum multi-particle teleportation, entangled based cryptography and quantum communication schemes based on multi-particle states, but also for fundamental reasons such as testing local realism by means of the Greenberger-Horne-Zeilinger states (GHZ) arguments . The advantage of multiparticle entanglement versus the most common two particle one lies in the fact that the greater the number of particles involved in the entangled state, the more clearly the quantum effects are exhibited. Our final goal is to exploit the multi-photon entangled states for quantum metrology. By the interaction of those states with nanostructures (mostly nanoholes, but in a future also nanospheres), we expect to reach sub-wavelength sensitivity phase measurements beating the Standard Quantum Limit as well as to detect plasmonic effects. In this thesis we present our work consisting on designing and building an experimental setup for the generation of states of 4-photon entangled in the transverse linear momentum. In the first part we explain some basics in the form of a technical introduction. We then adapt a general theoretical model to our particular case, explaining the physics of the process of generation of entangled states of photons. We proceed explaining the details of our setup, as well as the procedure of measurement. We then present the results of our tests in a "standard" 2-photon regime to show the correct functioning of the setup itself. Some more sophisticated measurements using structured light in the form of a first-order Hermite-Gaussian mode has been performed to generate entanglement in higher spatial modes are also presented. We conclude with theoretical and experimental details regarding the 4-photon experiments feasible with our setup. Our source is based on Spontaneous Parametric Down-Conversion (SPDC). In the last two decades it has been extensively studied for the generation of two-photon entangled states, since Kwiat et al. published in 1995 the new scheme based on polarization entangled photons. Most of the studies regarding entangled states involving more than two photons are indeed based on quantum correlations in the polarization or in the path of the down converted beams. The great advantage of entangling a spatial degree of freedom (as we do) is related to the dimensionality of the Hilbert space in which the state is defined. In the particular case of linear momentum, which is a continuous variable, we are dealing with infinite dimensions. Since in each dimension of the state one quanta of information can be encoded, the advantage of having multidimension entanglement for the field of quantum communication and computing is clear. The specs of our setup include a periodically-poled KTP crystals offering high conversion efficiency and cut for type-0 SPDC. The photons generated are well known to be inherently entangled in different degrees of freedom such as polarization, energy-time, linear momentum, and orbital angular momentum. Since each single SPDC event generates one photon pair, in order to reach four photon we entangle two consecutive SPDC events per each state. Furthermore, it is possible to manipulate (to enhance) the dimensionality of the entanglement by properly tailoring the pump spatial profile. The key point for the generation of four-photon entangled states is that, under some conditions, two consecutive pairs generated via SPDC cannot be described as two independent pairs but necessarily as a four-photon state showing genuine entanglement. This can happen when using a pulsed laser to generate the entangled photons; in particular, in the regime in which the coherence time of the down-converted photons τc is (much) longer than the temporal length of the pumping pulse Δt. In this condition the emission of a second pair is stimulated by the presence of the first one. That effect can be ultimately seen as a constructive multi-particle interference effect, the deep origin of which has to be sought in the boson statistic of photons.
Using angular position–orbital angular momentum entangled photons, we propose an experiment to generate maximally entangled states in D-dimensional quantum systems, the so called qudits, by exploiting correlations of parametric down-converted photons. Angular diffraction masks containing N angular slits in the arms of each twin photon define a qudit space of dimension N2, spanned by the alternative pathways of the photons. Numerical results for N angular slits with N = 2, 4, 5, 10 are reported. We discuss relevant experimental parameters for an experimental implementation of the proposed scheme using Spatial Light Modulators (SLMs), and twin-photons produced by Spontaneous Parametric Down Conversion (SPDC). The entanglement of the qudit state can be quantified in terms of the Concurrence, which can be expressed in terms of the visibility of the interference fringes, or by using Entanglement Witnesses. These results provide an additional means for preparing entangled quantum states in high-dimensions, a fundamental resource for quantum simulation and quantum information protocols.