Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:quant-ph/0307240 · International Journal of Quantum Information

QUANTUM INFORMATION PROCESSING BY NMR: PREPARATION OF PSEUDOPURE STATES AND IMPLEMENTATION OF UNITARY OPERATIONS IN A SINGLE-QUTRIT SYSTEM

Ranabir Das, Avik Mitra, Santosh Kumar, Anil Kumar

Published Sep 1, 2003• 47 citations
arXivHTMLPDF

Abstract

Theoretical Quantum Information Processing (QIP) has matured from the use of qubits to the use of qudits (systems having states >2). Whereas most of the experimental implementations have been performed using qubits, little experimental work has been carried out using qudits as yet. In this paper we demonstrate experimental realization of a qutrit system by nuclear magnetic resonance (NMR), utilizing deuterium (spin-1) nuclei partially oriented in liquid crystalline phase. Preparation of pseudopure states and implementation of unitary operations are demonstrated in this single-qutrit system, using transition selective pulses.

DOI
10.1142/s0219749903000292

Related papers

Quantum Information Processing by NMR using strongly coupled spins

T. S. Mahesh, Neeraj Sinha, Arindam Ghosh +5 more

The enormous theoretical potential of Quantum Information Processing (QIP) is driving the pursuit for its practical realization by various physical techniques. Currently Nuclear Magnetic Resonance (NMR) has been the forerunner by demonstrating a majority of quantum algorithms. In NMR, spin systems consisting of coupled nuclear spins are utilized as qubits. In order to carry out QIP, a spin system has to meet two major requirements: (i) qubit addressability and (ii) mutual coupling among the qubits. It has been demonstrated that the magnitude of the mutual coupling among qubits can be increased by orienting the spin-systems in a liquid crystal matrix and utilizing the residual dipolar couplings. While utilizing residual dipolar couplings may be useful to increase the number of qubits, nuclei of same species (homonuclei) might become strongly coupled. In strongly coupled spin-systems, spins loose their individual identity of being qubits. We propose that even such strongly coupled spin-systems can be used for QIP and the qubit-manipulation can be achieved by transition-selective pulses. We demonstrate experimental preparation of pseudopure states, creation of maximally entangled states, implementation logic gates and implementation of Deutsch-Jozsa (DJ) algorithm in strongly coupled 2,3 and 4 spin systems. The energy levels of the strongly coupled 3 and 4 spin systems were obtained by using a Z-COSY experiment.

arXiv:quant-ph/0212123•Dec 20, 2002•5 citations

Toward quantum information processing by nuclear magnetic resonance: Pseudopure states and logical operations using selective pulses on an oriented spin 3/2 nucleus

Neeraj Sinha, T. S. Mahesh, K. V. Ramanathan +1 more

Nuclear magnetic resonance spectroscopy has demonstrated significant experimental progress toward the development of quantum computations. The developments so far have taken place mainly through the use of spin 12 nuclei. In this paper we describe the use of a spin 32 nucleus, oriented in a liquid crystal matrix for the creation of pseudopure states and the implementation of a complete set of two-qubit reversible logic gates using single-quantum transition-selective pulses, extending the range of practice of NMR toward quantum computation.

The Journal of Chemical Physics•Mar 8, 2001•65 citations

Ensemble quantum-information processing by NMR: Implementation of gates and the creation of pseudopure states using dipolar coupled spins as qubits

T. S. Mahesh, Neeraj Sinha, K. V. Ramanathan +1 more

Quantum-information processing is carried out using dipolar coupled spins and high-resolution nuclear magnetic resonance (NMR). The systems chosen are the dipolar coupled methyl protons of ${\mathrm{CH}}_{3}\mathrm{CN}$ partially oriented in a liquid crystalline matrix yielding a two-qubit system and dipolar coupled ${}^{13}\mathrm{C}$ and methyl protons of ${}^{13}{\mathrm{CH}}_{3}\mathrm{CN}$ also partially oriented in the liquid crystalline matrix, yielding a three-qubit system. The dipolar coupled protons of oriented ${\mathrm{CH}}_{3}$ group are chemically and magnetically identical and their eigenstates can be divided into a set of quartet states (symmetric A) and a pair of doublet (E) states. We describe here a method for selectively retaining the magnetization of the symmetric states, yielding two and three qubit systems. We create pseudopure states using single-quantum-transition selective pulses and implement two- and three-qubit gates using one- and two-dimensional NMR.

Physical Review A•Jan 11, 2002•23 citations

A simple method for the preparation of pseudopure states in nuclear magnetic resonance quantum information processing

B. M. Fung, Vladimir L. Ermakov

The use of nuclear magnetic resonance (NMR) to carry out quantum information processing (QIP) often requires the preparation, transformation, and detection of pseudopure states. In our previous work, it was shown that the use of pairs of pseudopure states (POPS) as a basis for QIP is very convenient because of the simplicity in experimental execution. It is now further demonstrated that the product of the NMR spectra corresponding to two sets of POPS that share a common pseudopure state has the same peak frequencies as those of the common (single) pseudopure state. Examples of applying two different quantum logic gates to a 5-qubit system are given.

arXiv:quant-ph/0407194•The Journal of Chemical Physics•Oct 26, 2004•3 citations

Use of quadrupolar nuclei for quantum-information processing by nuclear magnetic resonance: Implementation of a quantum algorithm

Ranabir Das, Anil Kumar

Physical implementation of quantum-information processing by liquid-state nuclear magnetic resonance, using weakly coupled spin-$\frac{1}{2}$ nuclei of a molecule, is well established. Nuclei with $\mathrm{spin}>1/2$ oriented in liquid-crystalline matrices is another possibility. Such systems have multiple qubits per nuclei and large quadrupolar couplings resulting in well separated lines in the spectrum. So far, creation of pseudopure states and logic gates has been demonstrated in such systems using transition selective radio-frequency pulses. In this paper we report two developments. First, we implement a quantum algorithm that needs coherent superposition of states. Second, we use evolution under quadrupolar coupling to implement multiqubit gates. We implement the Deutsch-Jozsa algorithm on a spin-$\frac{3}{2}$ (2 qubit) system. The controlled-NOT operation needed to implement this algorithm has been implemented here by evolution under the quadrupolar Hamiltonian. To the best of our knowledge, this method has been implemented for the first time in quadrupolar systems. Since the quadrupolar coupling is several orders of magnitude greater than the coupling in weakly coupled spin-$\frac{1}{2}$ nuclei, the gate time decreases, increasing the clock speed of the quantum computer.

arXiv:quant-ph/0306100•Physical Review A•Sep 10, 2003•54 citations

Quantum-information processing by nuclear magnetic resonance: Experimental implementation of half-adder and subtractor operations using an oriented spin-7/2 system

Kota V. R. M. Murali, Neeraj Sinha, T. S. Mahesh +3 more

The advantages of using quantum systems for performing many computational tasks have already been established. Several quantum algorithms have been developed which exploit the inherent property of quantum systems such as superposition of states and entanglement for efficiently performing certain tasks. The experimental implementation has been achieved on many quantum systems, of which nuclear magnetic resonance has shown the largest progress in terms of number of qubits. This paper describes the use of a spin-7/2 as a three-qubit system and experimentally implements the half-adder and subtractor operations. The required qubits are realized by partially orienting ${}^{133}\mathrm{Cs}$ nuclei in a liquid-crystalline medium, yielding a quadrupolar split well-resolved septet. Another feature of this paper is the proposal that labeling of quantum states of system can be suitably chosen to increase the efficiency of a computational task.

Physical Review A•Aug 27, 2002•60 citations
Theoretical Quantum Information Processing (QIP) has matured from the use of qubits to the use of qudits (systems having states >2). Whereas most of the experimental implementations have been performed using qubits, little experimental work has been carried out using qudits as yet. In this paper we demonstrate experimental realization of a qutrit system by nuclear magnetic resonance (NMR), utilizing deuterium (spin-1) nuclei partially oriented in liquid crystalline phase. Preparation of pseudopure states and implementation of unitary operations are demonstrated in this single-qutrit system, using transition selective pulses.
The enormous theoretical potential of Quantum Information Processing (QIP) is driving the pursuit for its practical realization by various physical techniques. Currently Nuclear Magnetic Resonance (NMR) has been the forerunner by demonstrating a majority of quantum algorithms. In NMR, spin systems consisting of coupled nuclear spins are utilized as qubits. In order to carry out QIP, a spin system has to meet two major requirements: (i) qubit addressability and (ii) mutual coupling among the qubits. It has been demonstrated that the magnitude of the mutual coupling among qubits can be increased by orienting the spin-systems in a liquid crystal matrix and utilizing the residual dipolar couplings. While utilizing residual dipolar couplings may be useful to increase the number of qubits, nuclei of same species (homonuclei) might become strongly coupled. In strongly coupled spin-systems, spins loose their individual identity of being qubits. We propose that even such strongly coupled spin-systems can be used for QIP and the qubit-manipulation can be achieved by transition-selective pulses. We demonstrate experimental preparation of pseudopure states, creation of maximally entangled states, implementation logic gates and implementation of Deutsch-Jozsa (DJ) algorithm in strongly coupled 2,3 and 4 spin systems. The energy levels of the strongly coupled 3 and 4 spin systems were obtained by using a Z-COSY experiment.
Nuclear magnetic resonance spectroscopy has demonstrated significant experimental progress toward the development of quantum computations. The developments so far have taken place mainly through the use of spin 12 nuclei. In this paper we describe the use of a spin 32 nucleus, oriented in a liquid crystal matrix for the creation of pseudopure states and the implementation of a complete set of two-qubit reversible logic gates using single-quantum transition-selective pulses, extending the range of practice of NMR toward quantum computation.
Quantum-information processing is carried out using dipolar coupled spins and high-resolution nuclear magnetic resonance (NMR). The systems chosen are the dipolar coupled methyl protons of CH3CN{\mathrm{CH}}_{3}\mathrm{CN}CH3​CN partially oriented in a liquid crystalline matrix yielding a two-qubit system and dipolar coupled 13C{}^{13}\mathrm{C}13C and methyl protons of 13CH3CN{}^{13}{\mathrm{CH}}_{3}\mathrm{CN}13CH3​CN also partially oriented in the liquid crystalline matrix, yielding a three-qubit system. The dipolar coupled protons of oriented CH3{\mathrm{CH}}_{3}CH3​ group are chemically and magnetically identical and their eigenstates can be divided into a set of quartet states (symmetric A) and a pair of doublet (E) states. We describe here a method for selectively retaining the magnetization of the symmetric states, yielding two and three qubit systems. We create pseudopure states using single-quantum-transition selective pulses and implement two- and three-qubit gates using one- and two-dimensional NMR.
The use of nuclear magnetic resonance (NMR) to carry out quantum information processing (QIP) often requires the preparation, transformation, and detection of pseudopure states. In our previous work, it was shown that the use of pairs of pseudopure states (POPS) as a basis for QIP is very convenient because of the simplicity in experimental execution. It is now further demonstrated that the product of the NMR spectra corresponding to two sets of POPS that share a common pseudopure state has the same peak frequencies as those of the common (single) pseudopure state. Examples of applying two different quantum logic gates to a 5-qubit system are given.
Physical implementation of quantum-information processing by liquid-state nuclear magnetic resonance, using weakly coupled spin-12\frac{1}{2}21​ nuclei of a molecule, is well established. Nuclei with spin>1/2\mathrm{spin}>1/2spin>1/2 oriented in liquid-crystalline matrices is another possibility. Such systems have multiple qubits per nuclei and large quadrupolar couplings resulting in well separated lines in the spectrum. So far, creation of pseudopure states and logic gates has been demonstrated in such systems using transition selective radio-frequency pulses. In this paper we report two developments. First, we implement a quantum algorithm that needs coherent superposition of states. Second, we use evolution under quadrupolar coupling to implement multiqubit gates. We implement the Deutsch-Jozsa algorithm on a spin-32\frac{3}{2}23​ (2 qubit) system. The controlled-NOT operation needed to implement this algorithm has been implemented here by evolution under the quadrupolar Hamiltonian. To the best of our knowledge, this method has been implemented for the first time in quadrupolar systems. Since the quadrupolar coupling is several orders of magnitude greater than the coupling in weakly coupled spin-12\frac{1}{2}21​ nuclei, the gate time decreases, increasing the clock speed of the quantum computer.
The advantages of using quantum systems for performing many computational tasks have already been established. Several quantum algorithms have been developed which exploit the inherent property of quantum systems such as superposition of states and entanglement for efficiently performing certain tasks. The experimental implementation has been achieved on many quantum systems, of which nuclear magnetic resonance has shown the largest progress in terms of number of qubits. This paper describes the use of a spin-7/2 as a three-qubit system and experimentally implements the half-adder and subtractor operations. The required qubits are realized by partially orienting 133Cs{}^{133}\mathrm{Cs}133Cs nuclei in a liquid-crystalline medium, yielding a quadrupolar split well-resolved septet. Another feature of this paper is the proposal that labeling of quantum states of system can be suitably chosen to increase the efficiency of a computational task.